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arXiv:2312.05641 · Physical Review Letters

Nonclassical Correlations between Photons and Phonons of Center-of-Mass Motion of a Mechanical Oscillator

Ivan Galinskiy, Georg Enzian, Michal P. Parniak, Eugene Simon Polzik

Published Oct 24, 2024• 9 citations
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Abstract

We demonstrate nonclassical correlations between phonons and photons created using opto-mechanical spontaneous parametric down-conversion in a system based on a soft-clamped ultracoherent membrane oscillator inside of a Fabry-Pérot optical resonator. Non-Gaussian quantum features are demonstrated for the center-of-mass motion of a submillimeter nanogram-scale mechanical oscillator. We show that phonons stored in the mechanical oscillator, when subsequently read out, display strong signs of quantum coherence, which we demonstrate by single-photon counting enabled by our state-of-the-art optical filtering system. We observe a violation of the classical two-time Cauchy-Schwarz inequality between a heralding write photon and a stored phonon with a confidence of >92%.

DOI
10.1103/physrevlett.133.173605

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We demonstrate nonclassical correlations between phonons and photons created using opto-mechanical spontaneous parametric down-conversion in a system based on a soft-clamped ultracoherent membrane oscillator inside of a Fabry-Pérot optical resonator. Non-Gaussian quantum features are demonstrated for the center-of-mass motion of a submillimeter nanogram-scale mechanical oscillator. We show that phonons stored in the mechanical oscillator, when subsequently read out, display strong signs of quantum coherence, which we demonstrate by single-photon counting enabled by our state-of-the-art optical filtering system. We observe a violation of the classical two-time Cauchy-Schwarz inequality between a heralding write photon and a stored phonon with a confidence of >92%.
The generation of non-Gaussian quantum states of macroscopic mechanical objects is key to a number of challenges in quantum information science, ranging from fundamental tests of decoherence to quantum communication and sensing. Heralded generation of single-phonon states of mechanical motion is an attractive way toward this goal, as it is, in principle, not limited by the object size. Here we demonstrate a technique that allows for generation and detection of a quantum state of motion by phonon counting measurements near the ground state of a 1.5 MHz micromechanical oscillator. We detect scattered photons from a membrane-in-the-middle optomechanical system using an ultra-narrowband optical filter, and perform Raman-ratio thermometry and second-order intensity interferometry near the motional ground state ( n ¯ = 0.23 ± 0.02 p h o n o n s ). With an effective mass in the nanogram range, our system lends itself for studies of long-lived non-Gaussian motional states with some of the heaviest objects to date.
Adding excitations on a coherent state provides an effective way to observe the nonclassical properties of radiation fields. Here, we describe and analyze how to apply this concept to the motional state of a mechanical oscillator and present a full scheme to prepare non-Gaussian phonon-added coherent states of the mechanical motion in cavity optomechanics. We first generate a mechanical coherent state using electromagnetically induced transparency. We then add a single phonon onto the coherent state via optomechanical parametric down-conversion combined with single-photon detection. We validate this single-phonon-added coherent state by using a red-detuned beam and reading out the state of the optical output field. This approach allows us to verify nonclassical properties of the phonon state, such as sub-Poissonian character and quadrature squeezing. We further show that our scheme can be directly implemented using existing devices, and is generic in nature and hence applicable to a variety of systems in opto- and electromechanics.
We show how to use the radiation pressure optomechanical coupling between a mechanical oscillator and an optical cavity field to generate in a heralded way a single quantum of mechanical motion (a Fock state). Starting with the oscillator close to its ground state, a laser pumping the upper motional sideband produces correlated photon-phonon pairs via optomechanical parametric down-conversion. Subsequent detection of a single scattered Stokes photon projects the macroscopic oscillator into a single-phonon Fock state. The nonclassical nature of this mechanical state can be demonstrated by applying a readout laser on the lower sideband to map the phononic state to a photonic mode and performing an autocorrelation measurement. Our approach proves the relevance of cavity optomechanics as an enabling quantum technology.
A room-temperature mechanical oscillator undergoes thermal Brownian motion with an amplitude much larger than the amplitude associated with a single phonon of excitation. This motion can be read out and manipulated using laser light using a cavity-optomechanical approach. By performing a strong quantum measurement (i.e., counting single photons in the sidebands imparted on a laser), we herald the addition and subtraction of single phonons on the 300 K thermal motional state of a 4 GHz mechanical oscillator. To understand the resulting mechanical state, we implement a tomography scheme and observe highly non-Gaussian phase-space distributions. Using a maximum likelihood method, we infer the density matrix of the oscillator, and we confirm the counterintuitive doubling of the mean phonon number resulting from phonon addition and subtraction.
Destructive interference-based photon-phonon antibunching can lead to violations of classical inequalities in optomechanical cavity systems. In this paper, we explore the violation of the classical Cauchy-Schwarz inequality by examining second-order auto-correlation and cross-correlation functions, as well as Bell's nonlocality, to analyze the quantum correlations of single photon-phonon excitations when the system is driven by two weak probe fields. We propose that the violation of the Cauchy-Schwarz inequality can serve as an indicator for the stronger nonclassical tests associated with Bell's theorem. Our system reveals strong quantum correlations of photon-phonon pairs with distinctive antidiagonal patterns of photon filtering. For numerical analysis, we consider a weak effective optomechanical coupling strength and various optical-to-mechanical field amplitude ratios that enable unconventional photon (phonon) blockades at resonance. The findings are significant for producing sub-Poissonian signals under optimal conditions and have potential applications in hybrid systems for generating on-demand single photon-phonon pairs.
The preparation of pure quantum states with high degrees of macroscopicity is a central goal of ongoing experimental efforts to control quantum systems. We present a state preparation protocol which renders a mechanical oscillator with an arbitrarily large coherent amplitude in a manifestly nonclassical state. The protocol relies on coherent-state preparation followed by a projective measurement of a single Raman scattered photon, making it particularly suitable for cavity optomechanics. The nonclassicality of the state is reflected by sub-Poissonian phonon statistics, which can be accessed by measuring the statistics of subsequently emitted Raman sideband photons. The proposed protocol would facilitate the observation of nonclassicality of a mechanical oscillator that moves macroscopically relative to motion at the single-phonon level.