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arXiv:2312.05336

Beyond-mean-field effects in mixtures: few-body and many-body aspects

Dmitry S. Petrov

Published Dec 8, 2023• 1 citation
arXivHTMLPDF

Abstract

The discovery of ultracold dilute liquids has significantly elevated our interest in various phenomena which go under the name of beyond-mean-field (BMF) physics. In these lecture notes we give an elementary introduction to the quantum stabilization and liquefaction of a collapsing weakly interacting Bose-Bose mixture. A detailed derivation of the leading BMF correction, also known as the Lee-Huang-Yang (LHY) term, in this system is presented in a manner suitable for further generalizations and extensions. Although the LHY term is a nonanalytic function of the density $n$, under certain conditions the leading BMF correction becomes analytic and can be expanded in integer powers of $n$, effectively introducing three-body and higher-order interactions. We discuss why and how well the Bogoliubov approach can predict these few-body observables.

DOI
10.48550/arxiv.2312.05336

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The discovery of ultracold dilute liquids has significantly elevated our interest in various phenomena which go under the name of beyond-mean-field (BMF) physics. In these lecture notes we give an elementary introduction to the quantum stabilization and liquefaction of a collapsing weakly interacting Bose-Bose mixture. A detailed derivation of the leading BMF correction, also known as the Lee-Huang-Yang (LHY) term, in this system is presented in a manner suitable for further generalizations and extensions. Although the LHY term is a nonanalytic function of the density nnn, under certain conditions the leading BMF correction becomes analytic and can be expanded in integer powers of nnn, effectively introducing three-body and higher-order interactions. We discuss why and how well the Bogoliubov approach can predict these few-body observables.
We observe monopole oscillations in a mixture of Bose-Einstein condensates, where the usually dominant mean-field interactions are canceled. In this case, the system is governed by the next-order Lee-Huang-Yang (LHY) correction to the ground state energy, which describes the effect of quantum fluctuations. Experimentally such a LHY fluid is realized by controlling the atom numbers and interaction strengths in a ^{39}K spin mixture confined in a spherical trap potential. We measure the monopole oscillation frequency as a function of the LHY interaction strength as proposed recently by Jrgensen et al. [Phys. Rev. Lett. 121, 173403 (2018)PRLTAO0031-900710.1103/PhysRevLett.121.173403] and find excellent agreement with simulations of the complete experiment including the excitation procedure and inelastic losses. This confirms that the system and its collective behavior are initially dominated by LHY interactions. Moreover, the monopole oscillation frequency is found to be stable against variations of the involved scattering lengths in a broad region around the ideal values, confirming the stabilizing effect of the LHY interaction. These results pave the way for using the nonlinearity provided by the LHY term in quantum simulation experiments and for investigations beyond the LHY regime.
We demonstrate how the beyond-mean-field Lee-Huang-Yang (LHY) corrections and its related physics can be naturally incorporated into the representation of an ultracold Bose gas using the truncated Wigner approach without invoking effective energy terms or local density approximation. By generating a Bogoliubov ground-state representation with appropriately tailored bare interaction strength g0g_0g0​ and condensate density n0n_0n0​, the expected initial energy and densities are obtained while retaining access to quantum effects beyond the reach of the extended Gross-Pitaevskii equation (EGPE) formulation. This approach enables the study of correlations, coherence decay, single realisations, and the onset of quantum fluctuation effects with growing interaction strength. Numerical demonstrations for a weakly interacting single-component Bose gas show that observables deviate significantly from both the plain GPE and the EGPE incorporating LHY corrections. In regimes of strong interaction, many of the interference effects predicted by the GPE and EGPE are suppressed, and the EGPE offers no improvement over the plain GPE compared to the full Wigner model. In the weakly interaction limit, the EGPE appears accurate but resolving its deviation from mean-field results requires extensive ensemble averaging.
Quantum fluctuations play a pivotal role in determining the ground state properties and phase transitions of ultra-cold bosonic systems. This study presents a comprehensive theoretical investigation of fluctuation effects beyond mean-field theory in dilute Bose gases, examining their impact on the superfluid–Mott insulator transition, quantum droplet formation, and critical phenomena. Beginning with the Gross–Pitaevskii mean-field framework , we systematically incorporate quantum corrections through Bogoliubov theory, yielding the Lee–Huang–Yang (LHY) energy correction scaling as . The quantum depletion quantifies the fraction of atoms driven from the condensate by zero-point fluctuations. For the Bose–Hubbard model , quantum Monte Carlo simulations establish the superfluid–Mott insulator critical point at , shifted 15% from the mean-field prediction. Critical exponents and confirm 3D XY universality. Quantum droplets in binary mixtures are stabilized by the repulsive LHY correction against mean-field collapse, with equilibrium densities matching experimental observations in K mixtures. Finite-size scaling analysis and the Ginzburg criterion delineate regimes where fluctuation effects dominate. All theoretical predictions are validated against precision measurements in ultracold atomic gases.
The miscibility of quantum liquids is an interesting topic in many-body physics, which has been intensively investigated in 3He-4He superfluids and the mixtures of ultracold atoms. In the context of dual species Bose-Einstein condensates, the mean-field description has been well established, according to which, the miscibility condition is density independent and determined only by the ratio of inter- and intra-species interaction strength. Recently, Nadion and Petrov proposed that [ Phys. Rev. Lett. 126 115301 ], in the vicinity of the mixing-demixing threshold, quantum fluctuations play an important role to affect the equilibrium stability, and as a result, the partially miscible state emerges. This new phase of quantum matter opens up new perspectives to explore the beyond mean-field effect in ultracold atomic gases. In this work, according to the equation of state taking the Lee-Huang-Yang correction into consideration, we investigate the ground state phase diagram of repulsive binary Bose mixtures in the interacting regime suffering a weak mean-field instability. Under the thermodynamic balance conditions, the phase boundaries between the immiscible state, partially miscible state and the homogenous state are determined. For the equal-mass case, these phase transitions only take place on condition that intra-species interactions are in an asymmetric form. In terms of interaction parameters, we explicitly derive analytical expressions of the phase boundaries, which are appropriate to describe the transitions in sufficiently dilute atomic gases. At the quantum critical point, where the partially miscible state terminates, the susceptibility tensor of the density response exhibits a divergent behavior. For the unequal-mass case, the beyond-mean-field equation of state cannot be written in a compact form, thus the determination of the phase boundaries is more involved. By expanding the Lee-Huang-Yang energy expression to the terms linear in the concentration of the minority species, we analytically obtain the threshold density for the partially miscible transition. We also propose a discriminant function, from which the configuration of the partially miscible state can be identified for the given mass ratio and interaction strength. Applications of these theoretical results to experimental systems, such as sodium, potassium, and rubidium gases, are presented.
We investigate the properties of self-bound ultradilute Bose-Bose mixtures, beyond the Lee-Huang-Yang description. Our approach is based on the determination of the beyond mean-field corrections to the phonon modes of the mixture in a self-consistent way and calculation of the associated equation of state. The newly obtained ground state energies show excellent agreement with recent quantum Monte Carlo calculations, providing a simple and accurate description of the self-bound mixtures with contact type interaction. We further show numerical results for the equilibrium properties of the finite size droplet, by adjusting the Gross-Pitaevskii equation. Our analysis is extended to the one-dimensional mixtures where an excellent agreement with quantum Monte Carlo predictions is found for the equilibrium densities. Finally, we discuss the effects of temperature on the stability of the liquid phase.
Abstract The static and dynamic properties of self-bound quantum droplets in a one-dimensional Bose-Bose mixture are discussed in the spirit of the Hartree–Fock-Bogoliubov theory. This latter enables us to provide beyond the Lee-Huang-Yang (LHY) quantum corrections to the equation of state at both zero and finite temperatures. In the uniform case our results for the ground-state energy and the critical temperature are confirmed through comparison with Quantum Monte-Carlo simulation and with available theoretical results. The density profiles are supported by numerical simulations of the generalized Gross-Pitaevskii equation which selfconsistently includes higher-order terms originating from the normal and anomalous fluctuations under the local density approximation. We show that the density exhibits a dip near its center in the flat-top plateau region for large interspecies interactions. We exemplify the impact of the beyond LHY corrections on the spatiotemporal evolution of the self-bound droplet in the presence of excitation induced by periodic density modulation. It is found that higher-order corrections may lead to the formation of a train of small droplets. We then extend our study for the case of inhomogeneous droplets in quasi one-dimensional Bose mixtures.