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arXiv:2312.04115 · Physical Review Letters

Quantum Slush State in Rydberg Atom Arrays

Tengzhou Zhang, Zi Cai

Published May 17, 2024• 15 citations
arXivHTMLPDF

Abstract

In this Letter, we propose an exotic quantum state that does not order at zero temperature in a Rydberg atom array with antiblockade mechanism. By performing an unbiased large-scale quantum Monte Carlo simulation, we investigate a minimal model with facilitated excitation in a disorder-free system. At zero temperature, this model exhibits a heterogeneous structure of liquid and glass mixture. This state, dubbed quantum slush state, features a quasi-long-range order with an algebraic decay for its correlation function, and is different from most well-established quantum phases of matter.

DOI
10.1103/physrevlett.132.206503

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In this Letter, we propose an exotic quantum state that does not order at zero temperature in a Rydberg atom array with antiblockade mechanism. By performing an unbiased large-scale quantum Monte Carlo simulation, we investigate a minimal model with facilitated excitation in a disorder-free system. At zero temperature, this model exhibits a heterogeneous structure of liquid and glass mixture. This state, dubbed quantum slush state, features a quasi-long-range order with an algebraic decay for its correlation function, and is different from most well-established quantum phases of matter.
We investigate the nonequilibrium dynamics of a kinetic slush state realized via facilitated excitations in a two-dimensional dissipative Rydberg atom array. Utilizing kinetic Monte Carlo simulations in the strong dephasing regime, we show that tuning the laser detuning to compensate for nearest-neighbor interactions enables facilitated dynamics, while residual next-nearest-neighbor interactions induce kinetic frustration. This competition gives rise to an emergent slush phase characterized by pronounced dynamical heterogeneity and the coexistence of liquid- and solid-like configurations. By probing its nonequilibrium real-time evolution, we uncover a dynamical crossover from isotropic spreading to one-dimensional constrained growth, which can be continuously tuned by the frustration strength. Within this crossover regime, the slush dynamics generate fractal cluster geometries and generalized Ornstein-Zernike spatial correlations. Finite-size scaling analysis supports the system's proximity to criticality. Our findings establish driven-dissipative Rydberg systems as a highly controllable platform for engineering complex nonequilibrium soft-matter phenomena.
A programmable quantum simulator using Rydberg-atom array provides a promising route to demystifying quantum many-body physics in strongly correlated systems. Motivated by the recent realization of various quantum magnetic phases on the frustrated Rydberg-atom array, we perform numerically exact quantum Monte Carlo simulations to investigate the exotic states of matter emerging in the model describing the Rydberg atom on a triangular lattice. Our state-of-the-art simulation unveils the $\sqrt{3}\ifmmode\times\else\texttimes\fi{}\sqrt{3}$ triangular antiferromagnetic order exists at 1/31/31/3 or 2/32/32/3-Rydberg filling, consistent with the observation in experiments. Remarkably, $\sqrt{3}\ifmmode\times\else\texttimes\fi{}\sqrt{3}$ long-range order arising from order-by-disorder mechanism emerges at 1/21/21/2 filling. At finite temperature, U(1)\mathrm{U}(1)U(1) symmetry is emergent at 1/21/21/2 filling and a Kosterlitz-Thouless phase transition occurs with increasing temperature. These intriguing phenomena are potentially detected in future Rydberg-atom experiments.
Motivated by recent experimental realizations of exotic phases of matter on programmable quantum simulators, we carry out a comprehensive theoretical study of quantum phase transitions in a Rydberg atom array on a square lattice, with both open and periodic boundary conditions. In the bulk, we identify several first-order and continuous phase transitions by performing large-scale quantum Monte Carlo simulations and develop an analytical understanding of the nature of these transitions using the framework of Landau-Ginzburg-Wilson theory. Remarkably, we find that under open boundary conditions, the boundary itself undergoes a second-order quantum phase transition, independent of the bulk. These results explain recent experimental observations and provide important insights into both the adiabatic state preparation of novel quantum phases and quantum optimization using Rydberg atom array platforms.
Recent advances in Rydberg tweezer arrays bring novel opportunities for programmable quantum simulations beyond previous capabilities. In this Letter, we investigate a bosonic t-J-V model currently realized with Rydberg atoms. Through large-scale quantum Monte Carlo simulations, we uncover an emergent double supersolid (DSS) phase with the coexistence of two superfluids and crystalline order. Tunable long-range tunneling and repulsive hole-hole interactions enable a rich phase diagram featuring a double superfluid phase, a DSS phase, and an antiferromagnetic insulator. Intriguingly, within the DSS regime we observe an unconventional thermal enhancement of crystalline order. Our results establish the bosonic t-J-V model as a promising and experimentally accessible platform for exploring exotic quantum phases in Rydberg atom arrays.
Rydberg atom arrays have recently emerged to be a promising platform for the exploration of exotic quantum phases of matter and quantum phenomena. In this work, we map out the ground-state phase diagram of Rydberg atoms on a honeycomb lattice as a function of the Rydberg blockade radius and the laser detuning by performing large-scale finite-size density matrix renormalization group simulations. Apart from a featureless disordered phase, we find five other intricate long-range density-wave-ordered phases within a relatively wide parameter space. The properties of these quantum phases are analyzed by calculating their Rydberg excitation profiles and static structure factors. In addition, a continuous quantum phase transition belonging to the (2+1)-dimensional Ising universality class is explored by a standard finite-size scaling analysis. Our work implies some different physics, such as the possible nontrivial quantum phase transitions and a highly degenerate string ordered phase, that a honeycomb geometry could bring to the Rydberg system and serves as a numerical guide for possible real experiments.
Deterministic quasiperiodicity in quantum systems has long been associated with localization, criticality, or glassy behavior, and has therefore been believed to suppress long-range order rather than stabilize it. Here we demonstrate the opposite: quasiperiodicity in interactions--without any quasiperiodic potential, disorder, or geometric modulation--can generate coherent, ordered quantum phases. We study hard-core bosons in one dimension with quasiperiodic long-range interactions, V_{ij}=V_0 \cos(παi)\cos(παj), where n=α=(\sqrt{5}-1)/2 is the inverse golden ratio. Using large-scale path-integral quantum Monte Carlo simulations, we uncover thermodynamically stable incompressible plateaus at irrational densities tied to Fibonacci ratios. These plateaus exhibit sharp incommensurate Bragg peaks, signaling an emergent quasi-solid with long-range quasicrystalline density order. More strikingly, at nearby fillings and interaction strengths, we identify a quasi-supersolid phase that supports both Fibonacci density ordering and finite superfluid density--demonstrating that interaction-induced quasiperiodicity can stabilize supersolid coherence. Our results establish a new mechanism for realizing ordered quasicrystalline quantum matter, and provide realistic guidance for implementation in Rydberg atom arrays, multimode cavity-QED systems, and trapped-ion quantum simulators.