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arXiv:2312.03679

Single-ion optical autocorrelator

Mahmood Irtiza Hussain, Milena Guevara-Bertsch, E. Torrontegui, Juan José García‐Ripoll, R. Blatt, Christian F. Roos

Published Dec 6, 2023• 0 citations
arXivHTMLPDF

Abstract

Well isolated quantum systems are exquisite sensors of electromagnetic fields. In this work, we use a single trapped ion for characterizing chirped ultraviolet (UV) picosecond laser pulses. The frequency swept pulses resonantly drive a strong dipole transition via rapid adiabatic passage, resulting in near deterministic population exchange caused by absorption or stimulated emission of photons. When subjecting an ion to counterpropagating pulse pairs, we observe the loss and revival of atomic coherence as a function of the pulse pair spatial overlap enabling quantification of the temporal pulse broadening caused by a frequency chirp in shaped UV pulses with a very low peak power. We find good agreement between measured and applied chirp. The ultrafast population exchange imparts an impulsive force where the estimated change in the mean phonon numbers of 0.5 is measured for two pairs of pulses. The resonant ultrafast kicks could be applied to matter wave interferometry experiments and present a step towards ultrafast entanglement operations in trapped ions.

DOI
10.48550/arxiv.2312.03679

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Well isolated quantum systems are exquisite sensors of electromagnetic fields. In this work, we use a single trapped ion for characterizing chirped ultraviolet (UV) picosecond laser pulses. The frequency swept pulses resonantly drive a strong dipole transition via rapid adiabatic passage, resulting in near deterministic population exchange caused by absorption or stimulated emission of photons. When subjecting an ion to counterpropagating pulse pairs, we observe the loss and revival of atomic coherence as a function of the pulse pair spatial overlap enabling quantification of the temporal pulse broadening caused by a frequency chirp in shaped UV pulses with a very low peak power. We find good agreement between measured and applied chirp. The ultrafast population exchange imparts an impulsive force where the estimated change in the mean phonon numbers of 0.5 is measured for two pairs of pulses. The resonant ultrafast kicks could be applied to matter wave interferometry experiments and present a step towards ultrafast entanglement operations in trapped ions.
Experimental realizations of two qubit entangling gates with trapped ions typically rely on addressing spectroscopically resolved motional sidebands, limiting gate speed to the secular frequency. Fast entangling gates using ultrafast pulsed lasers overcome this speed limit. This approach is based on state-dependent photon recoil kicks from a sequence of counter-propagating, resonant, ultrafast pulse pairs, which can allow sub-microsecond gate speeds. Here, we demonstrate a key component of the ultrafast gate protocol, the coherent excitation of a 171Yb+ ion across the 2S1∕2-2P1∕2 transition with a single near-resonant short optical pulse at 369.53 nm. We achieve a maximum population transfer of 94(1)% using a picosecond pulsed laser that can be tuned across the 2S1∕2-2P1∕2 transition and 42.5(9)% with 190(7) GHz detuning.
Trapped atomic ions are a promising medium for quantum computing, due to their long coherence times and potential for scalability. Current methods of en-tangling ions rely on addressing individual modes of motion within the trap and applying qubit state dependent forces with external fields. This approach can limit the speed of entangling gates and make them vulnerable to decoherence due to coupling to unwanted modes or ion heating. This thesis is directed towards demon-strating novel entanglement schemes which are not limited by the trap frequency, and can be made almost arbitrarily fast. Towards this goal, I report here on the first experiments using ultrafast laser pulses to control the internal and external states of a single trapped ion. I begin with experiments in ultrafast spin control, showing how a single laser pulse can be used to completely control both spin degrees of freedom of the ion qubit in tens of picoseconds. I also show how a train of weak pulses can be used to drive Raman transitions based on a frequency comb. I then discuss exper-iments using pulses to rapidly entangle the spin with the motion, and how careful spectral redistribution allows a single pulse to execute a spin-dependent momentum kick. Finally, I explain how these spin-dependent momentum kicks can be used in the future to create an ultrafast entangling gate. I go over how such a gate would work, and present experimentally realizable timing sequences which would create a maximally entangled state of two ions in a time faster than the period of motion in the trap.
Trapped atomic ions are a promising medium for quantum computing, due to their long coherence times and potential for scalability. Current methods of entangling ions rely on addressing individual modes of motion within the trap and applying qubit state dependent forces with external fields. This approach can limit the speed of entangling gates and make them vulnerable to decoherence due to coupling to unwanted modes or ion heating. This thesis is directed towards demonstrating novel entanglement schemes which are not limited by the trap frequency, and can be made almost arbitrarily fast. Towards this goal, I report here on the first experiments using ultrafast laser pulses to control the internal and external states of a single trapped ion. I begin with experiments in ultrafast spin control, showing how a single laser pulse can be used to completely control both spin degrees of freedom of the ion qubit in tens of picoseconds. I also show how a train of weak pulses can be used to drive Raman transitions based on a frequency comb. I then discuss experiments using pulses to rapidly entangle the spin with the motion, and how careful spectral redistribution allows a single pulse to execute a spin-dependent momentum kick. Finally, I explain how these spin-dependent momentum kicks can be used in the future to create an ultrafast entangling gate. I go over how such a gate would work, and present experimentally realizable timing sequences which would create a maximally entangled state of two ions in a time faster than the period of motion in the trap.
Coherent excitation and stimulated emission from optical transitions has been proposed as a mechanism to generate strong coherent forces in atomic systems and as the basis for fast quantum gates in trapped ions. We have demonstrated driving coherent oscillations between the 2S1/2 and 2P1/2 states in trapped 171Yb+ with 2.5 ps pulses straddling the resonance at 369.5nm. At higher powers nearly full extinction was observed, demonstrating coherence, however residual detuning issues have precluded full coherent population transfer.
Scalable quantum gates remain a central challenge for trapped-ion quantum computing. Ultrafast gates driven by spin-dependent kicks (SDKs) provide a promising approach. However, current protocols rely on mode-locked lasers, suffering from inflexible timing control and limited single-SDK fidelity. To overcome this, we propose a scheme using rapid adiabatic passage (RAP) pulses modulated from a continuous-wave laser. We demonstrate that this RAP-based approach suppresses the sensitivity of SDKs to fluctuations in optical intensity, thereby enabling the construction of robust entangling gates. Furthermore, the programmable nature of these modulated pulses allows for precise control over pulse sequences, further optimizing gate performance.