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arXiv:2312.01503 · Physical Review Research

Impact of temporal correlations, coherence, and postselection on two-photon interference

Fernando Redivo Cardoso, Jaewon Lee, Riccardo Checchinato, Jan-Heinrich Littmann, Marco De Gregorio, Sven Höfling, Christian Schneider, Celso J. Villas-Bôas, Ana Predojević

Published Feb 21, 2025• 4 citations
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Abstract

Two-photon interference is an indispensable resource in quantum photonics, but it is not straightforward to achieve. The cascaded generation of photon pairs contains intrinsic temporal correlations that negatively affect the ability of such sources to perform two-photon interference, thus hindering applications. We report on how such correlation interplays with decoherence and temporal postselection, and under which conditions temporal postselection could improve two-photon interference visibility. Our study identifies crucial parameters and points the way to a source with optimal performance.

DOI
10.1103/physrevresearch.7.013190

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Two-photon interference is an indispensable resource in quantum photonics, but it is not straightforward to achieve. The cascaded generation of photon pairs contains intrinsic temporal correlations that negatively affect the ability of such sources to perform two-photon interference, thus hindering applications. We report on how such correlation interplays with decoherence and temporal postselection, and under which conditions temporal postselection could improve two-photon interference visibility. Our study identifies crucial parameters and points the way to a source with optimal performance.
Two-photon interference (TPI) is a fundamental phenomenon in quantum optics and plays a crucial role in optical quantum technologies. TPI is commonly considered as quantum interference with an upper bound of 100% for both the TPI and the beat visibility in contrast to its classical counterpart with a maximum visibility of 50%. However, this is not always the case. Here, we report a simultaneous observation of quantum and classical TPI of single photons with ultralong coherence time, which is five orders of magnitude longer than the photon correlation time. We observe a TPI visibility of 94.3% ± 0.2% well above the 50% classical limit indicating the quantum feature, and a beat visibility of 50% reflecting the classical feature. In addition an anti-bunching central dip due to single-photon anti-correlation, we also observe two bunching side peaks in cross correlation curves for indistinguishable photons. Using the general wave superposition theory and the quantum field approach, we derive the same cross correlation functions, which fully reproduce and explain the experiments. Our results reveal that the quantum and classical features of TPI result from the same interference, as the fourth-order temporal interference arises from the second-order temporal interference between two photons on the timescale of the photon coherence time.
Quantum emitters such as semiconductor quantum dots can provide entangled photon pairs emitting from a system of cascaded states. However, the resulting temporal correlation between the two photons from the three-level ladder system has been shown to set a limit on the achievable two-photon interference. In this work, we show that such limitation, for photons emitted by the second transition, is only due to reduced temporal overlap at the interference beam splitter. We investigate this theoretically and experimentally by determining time-resolved four-photon coincidences between two successively emitted photon pairs. Post-emission synchronization shows the recovery of maximum interference visibility; in prospective quantum networks this could be achieved via deterministic quantum memories.
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We experimentally demonstrate shaping of the two-photon wave function of entangled-photon pairs, utilizing coherent pulse-shaping techniques. By performing spectral-phase manipulations we tailor the second-order correlation function of the photons exactly like a coherent ultrashort pulse. To observe the shaping we perform sum-frequency generation with an ultrahigh flux of entangled photons. At the appropriate conditions, sum-frequency generation performs as a coincidence detector with an ultrashort response time (approximately 100 fs), enabling a direct observation of the two-photon wave function. This property also enables us to demonstrate background-free, high-visibility two-photon interference oscillations.
In classical optics, interference occurs between two optical fields when they are indistinguishable from one another. The same holds true in quantum optics, where a particular experiment, the Franson interferometer, involves the interference of a photon pair with a time-delayed version of itself. The canonical version of this interferometer requires that the time delay be much shorter than the coherence length of the pump used to generate the photon pair, so as to guarantee indistinguishability. However, when this time delay is comparable to the coherence length, conventional wisdom suggests that interference visibility degrades significantly. In this work, though, we show that the interference visibility can be restored through judicious temporal post-selection. Utilizing correlated photon pairs generated by a pump whose pulsewidth (460 ps) is shorter than the interferometer’s time delay (500 ps), we are able to observe a fringe visibility of 97.4±4.3%. We believe this new method can be used for the encoding of high-dimensional quantum information in the temporal domain.