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arXiv:2312.00649 · Nature Communications

Robustness of quantum chaos and anomalous relaxation in open quantum circuits

Takato Yoshimura, Lucas Sá

Published Nov 12, 2024• 18 citations
arXivHTMLPDF

Abstract

Dissipation is a ubiquitous phenomenon that affects the fate of chaotic quantum many-body dynamics. Here, we show that chaos can be robust against dissipation but can also assist and anomalously enhance relaxation. We compute exactly the dissipative form factor of a generic Floquet quantum circuit with arbitrary on-site dissipation modeled by quantum channels and find that, for long enough times, the system always relaxes with two distinctive regimes characterized by the presence or absence of gap-closing. While the system can sustain a robust ramp for a long (but finite) time interval in the gap-closing regime, relaxation is "assisted" by quantum chaos in the regime where the gap remains nonzero. In the latter regime, we prove that, if the thermodynamic limit is taken first, the gap does not close even in the dissipationless limit. We complement our analytical findings with numerical results for quantum qubit circuits.

DOI
10.1038/s41467-024-54164-7

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Dissipation is a ubiquitous phenomenon that affects the fate of chaotic quantum many-body dynamics. Here, we show that chaos can be robust against dissipation but can also assist and anomalously enhance relaxation. We compute exactly the dissipative form factor of a generic Floquet quantum circuit with arbitrary on-site dissipation modeled by quantum channels and find that, for long enough times, the system always relaxes with two distinctive regimes characterized by the presence or absence of gap-closing. While the system can sustain a robust ramp for a long (but finite) time interval in the gap-closing regime, relaxation is "assisted" by quantum chaos in the regime where the gap remains nonzero. In the latter regime, we prove that, if the thermodynamic limit is taken first, the gap does not close even in the dissipationless limit. We complement our analytical findings with numerical results for quantum qubit circuits.
We consider the dynamics of generic chaotic quantum many-body systems with no conservation laws, subject to weak bulk dissipation. It was recently observed [T. Mori, Phys. Rev. B 109, 064311 (2024)] that the generator of these dissipative dynamics, a quantum channel E\mathcal{E}E, retains a nonzero gap as the dissipation strength $\ensuremath{\gamma}\ensuremath{\rightarrow}0$ if the thermodynamic limit is taken first. We use a hydrodynamic description of operator spreading in the presence of dissipation to estimate the gap of E\mathcal{E}E as $\ensuremath{\gamma}\ensuremath{\rightarrow}0$, to calculate the operator-size distribution of the slowest eigenmodes of E\mathcal{E}E, and to relate the gap to the long-time decay rates of autocorrelation functions under unitary Floquet dynamics. We provide a microscopic derivation of this hydrodynamic perspective for random unitary circuits. We argue that the gap in the $\ensuremath{\gamma}\ensuremath{\rightarrow}0$ limit can change nonanalytically as one tunes the parameters of the unitary dynamics.
We address the longstanding challenge in quantum many-body theory of reconciling unitary dynamics with irreversible relaxation. In classical chaos, the unitary evolution operator develops Ruelle-Pollicott (RP) resonances inside the unit circle in the continuum limit, leading to mixing. In the semiclassical limit, chaotic single-particle quantum systems relax with the same RP resonances. In contrast, the theory of quantum many-body RP resonances and their link to irreversibility remain underdeveloped. Here, we relate the spectral form factor to the sum of autocorrelation functions and, in generic many-body lattice systems without conservation laws, we argue that all quantum many-body RP resonances converge inside the unit disk, highlighting the role of nonunitary and the thermodynamic limit. While we conjecture this picture to be general, we analytically prove the emergence of irreversibility in the random phase model (RPM), a paradigmatic Floquet quantum circuit model, in the limit of large local Hilbert space dimension. To this end, we couple it to local environments and compute the exact time evolution of autocorrelation functions, the dissipative form factor, and out-of-time-order correlation functions (OTOCs). Although valid for any dissipation strength, we then focus on weak dissipation to clarify the origin of irreversibility in unitary systems. When the dissipationless limit is taken after the thermodynamic limit, the unitary quantum map develops an infinite tower of decaying RP resonances-chaotic systems display so-called anomalous relaxation. We identify the exact RP resonances in the RPM and prove that the same RP resonances are obtained from operator truncation. We also show that the OTOC in the RPM can undergo a two-stage relaxation, and that during the second stage, the approach to the stationary value is again controlled by the leading RP resonance. Finally, we demonstrate how conservation laws, many-body localization, and nonlocal interactions merge the leading RP resonance into the unit circle, thereby suppressing anomalous relaxation. Our findings clarify the microscopic origin of macroscopic relaxation in quantum systems and emphasize the role of RP resonances as a largely unexplored signature of many-body quantum chaos.
Phenomena in quantum chaotic systems such as spectral fluctuations are known to be described remarkably well by the random matrix theory (RMT) in small energy intervals and over large time scales. However, in exchange for analytical tractability, RMT has been constructed to leave out an important element of realistic physical systems { the notion of locality. Since quantum information propagates at a finite speed in a spatially-extended quantum chaotic system, there exists time scales before which RMT is effective. How do we describe the non-equilibrium quantum dynamics at intermediate timescales which are much longer than the local relaxation time but too short for RMT to apply? What are the signatures of many-body quantum chaotic systems beyond the description of RMT? In this thesis, we address these questions by analysing minimal models that incorporate a notion of locality and at the same time retain some analytical tractability of RMT. More specifically, we study Floquet quantum circuits that are random in space but periodic in time. These circuits consist of local and random quantum gates that act on a q-state `spin' at each site. After a brief review of classical chaos, quantum chaos, and quantum circuits in Chapter 1, we present three main results. In Chapter 2, we formulate a diagrammatical approach for computing ensemble averages of observables over random unitary circuits, and derive exact results on spectral statistics and dynamical observables for a Floquet circuit in the large-q limit. In Chapter 3, we further investigate the spectral statistics in spatiallyextended many-body quantum chaotic systems by computing the spectral form factor K(t) analytically and numerically. We show that K(t) follows the RMT description at times longer than the Thouless time tTh and identify the scaling of tTh at the large-q limit of a Floquet circuit. In Chapter 4, we discuss eigenstate correlations for spatially-extended many-body quantum chaotic systems, in terms of the statistical properties of matrix elements of local observables. While the eigenstate thermalization hypothesis (ETH) is known to give an excellent description of these quantities, the phenomenon of scrambling and the butterfly effect imply structure beyond ETH. We determine analytically and verify numerically the universal form of this structure at long distances and small eigenvalue separations for Floquet systems.
In interacting quantum many-body systems, relaxation toward equilibrium reflects a competition between internal chaotic dynamics and environmental dissipation. While conventional Markovian baths typically produce exponential decay, non-Markovian dissipation can give rise to more intricate behavior, including algebraic relaxation. We study an open Sachdev-Ye-Kitaev (SYK) model coupled to a pseudogapped fermionic bath, using the Keldysh formalism to compute steady-state correlations in the large-NNN limit. Our results uncover a rich dynamical phase diagram, with regimes of bath-driven power-law relaxation, chaos-driven exponential decay, and an intermediate pre-relaxation phase where exponential decay crosses over to algebraic decay. These findings demonstrate that non-Markovian environments can qualitatively reshape relaxation mechanisms in strongly correlated quantum many-body systems.
We define quantum chaos and integrability in open quantum many-body systems as a dynamical property of single stochastic realizations, referred to as quantum trajectories. This definition relies on the predictions of random matrix theory applied to the subset of the Liouvillian eigenspectrum involved in each quantum trajectory. Our approach, which we name (SSQT), enables a natural distinction between transient and steady-state quantum chaos as general phenomena in open setups. We test the generality and reliability of the SSQT criterion on several dissipative systems, further showing that an open system with a chaotic structure can evolve towards either a chaotic or integrable steady state. We apply our theoretical framework to two driven-dissipative bosonic systems. First, we study the driven-dissipative Bose-Hubbard model, a paradigmatic example of a quantum simulator, clarifying the interplay of integrability, transient, and steady-state chaos across its phase diagram. Our analysis shows the existence of an emergent dissipative quantum chaotic phase, whereas the classical and semiclassical limits display an integrable behavior. In this regime, chaos arises from the quantum and classical fluctuations associated with the dissipation mechanisms. Second, we investigate dissipative quantum chaos in the dispersive readout of a transmon qubit: a measurement technique ubiquitous in superconducting-based quantum hardware. Through the SSQT, we distinguish several regimes where the performance of the measurement instrument can be connected to the integrable or chaotic nature of the underlying driven-dissipative bosonic system. Our work offers a general understanding of the integrable and chaotic dynamics of open quantum systems and paves the way for the investigation of dissipative quantum chaos and its consequences on state-of-the-art noisy intermediate-scale quantum devices.
Digital quantum simulation (DQS) is one of the most promising applications of quantum computing. Trotterised DQS models quantum dynamics by decomposing the evolution into a sequence of gate-based Trotter steps. Using larger Trotter steps reduces the required gate count, but it is now understood that the Trotterisation step size cannot be increased beyond a certain threshold value, beyond which there is a sudden breakdown in simulation accuracy, due to the onset of quantum chaos. To date, this behaviour has only been studied for closed systems not subjected to the environmental noise and decoherence to which real-world quantum computers are highly sensitive. In this work, we study a range of experimentally relevant open-system quantum simulator models and show that Trotterisation thresholds persist even when open-system effects are included, even in the long-time, steady-state limit, once all coherence has been lost. We show that open DQS can accurately reproduce the dynamics of open target systems prior to the threshold, but still exhibits a sudden performance breakdown beyond it. We introduce new, statistical techniques to rigorously characterise the onset of quantum chaos beyond the Trotterisation threshold for both approximately unitary and genuine dissipative quantum chaos, based on random matrix theory (RMT), building on techniques developed for closed systems. Finally, we demonstrate that dissipative quantum chaos emerges when the dissipation is in balance with the presence of underlying unitary quantum chaos; the dissipation must be strong enough to induce genuinely dissipative behaviour, yet not so strong as to suppress the underlying chaotic structure.