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arXiv:2311.18616 · Physical Review A

Quantum dynamics of a fully blockaded Rydberg atom ensemble

Dominik S. Wild, Sabina Drăgoi, Corbin McElhanney, Jonathan Wurtz, Sheng-Tao Wang

Published Apr 16, 2024• 4 citations
arXivHTMLPDF

Abstract

Classical simulation of quantum systems plays an important role in the study of many-body phenomena and in the benchmarking and verification of quantum technologies. Exact simulation is often limited to small systems because the dimension of the Hilbert space increases exponentially with the size of the system. For systems that possess a high degree of symmetry, however, classical simulation can reach much larger sizes. Here we consider an ensemble of strongly interacting atoms with permutation symmetry, enabling the computation of certain collective observables for hundreds of atoms at arbitrarily long evolution times. The system is realized by an ensemble of three-level atoms, where one of the levels corresponds to a highly excited Rydberg state. In the limit of all-to-all Rydberg blockade, the Hamiltonian is invariant under permutation of the atoms. Using techniques from representation theory, we construct a block-diagonal form of the Hamiltonian, where the size of the largest block increases only linearly with the system size. We apply this formalism to derive efficient pulse sequences to prepare arbitrary permutation-invariant quantum states. Moreover, we study the quantum dynamics following a quench, uncovering a parameter regime in which the system thermalizes slowly and exhibits pronounced revivals. Our results create opportunities for the experimental and theoretical study of large interacting and nonintegrable quantum systems. Published by the American Physical Society 2024

DOI
10.1103/physreva.109.043111

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Classical simulation of quantum systems plays an important role in the study of many-body phenomena and in the benchmarking and verification of quantum technologies. Exact simulation is often limited to small systems because the dimension of the Hilbert space increases exponentially with the size of the system. For systems that possess a high degree of symmetry, however, classical simulation can reach much larger sizes. Here we consider an ensemble of strongly interacting atoms with permutation symmetry, enabling the computation of certain collective observables for hundreds of atoms at arbitrarily long evolution times. The system is realized by an ensemble of three-level atoms, where one of the levels corresponds to a highly excited Rydberg state. In the limit of all-to-all Rydberg blockade, the Hamiltonian is invariant under permutation of the atoms. Using techniques from representation theory, we construct a block-diagonal form of the Hamiltonian, where the size of the largest block increases only linearly with the system size. We apply this formalism to derive efficient pulse sequences to prepare arbitrary permutation-invariant quantum states. Moreover, we study the quantum dynamics following a quench, uncovering a parameter regime in which the system thermalizes slowly and exhibits pronounced revivals. Our results create opportunities for the experimental and theoretical study of large interacting and nonintegrable quantum systems. Published by the American Physical Society 2024
A frontier challenge in quantum science and technology is the construction of scalable quantum systems which can operate in regimes beyond classical simulatability. Such systems can be used as tools for simulating and exploring complex phenomena in quantum physics; they can also be used to benchmark and test quantum algorithms. Several experimental platforms, based on a variety of quantum mechanical building blocks, are currently being pursued with these goals in mind, with state-of-the-art systems capable of controlling up to around fifty particles. In this thesis, we present the development of a new platform based on individually controlled neutral atoms. In this approach, hundreds of individual atoms are trapped in an array of optical tweezers, and they are sorted in real-time into programmable geometries in one and two dimensions. After initialization of an array, atom interactions are switched on by coherent excitation to highly excited Rydberg states, resulting in a rich spin Hamiltonian. We experimentally advance several key aspects of this platform, developing new tools for controlling strongly interacting atom arrays and probing novel quantum phases and non-equilibrium dynamics. We additionally utilize Rydberg interactions to entangle atoms, demonstrating high fidelity universal quantum logic gates as well as the preparation of fully entangled Schrödinger cat states. This work highlights the prospects for scalable quantum simulation and quantum information processing beyond the limit of classical computation using neutral atom arrays.
Abstract Strongly Rydberg-blockaded two-level atoms form a Rydberg superatom which is excited only to a collective symmetrical Dicke state. However, emerging often in the alkali-earth atoms, spontaneous decay from the Rydberg state to an additional pooling state renders the ensemble no longer a closed superatom. Herein we present a computationally efficient model to characterize the interaction between a fully Rydberg-blockaded ensemble of N Λ-type three-level atoms and a strong probe light field in a coherent state. The model enables us to achieve a decomposition of the coupled dynamics in the strong field limit, which significantly reduces the complexity of computing the N -body system evolution and paves the way for practical analysis in experiments. A quasi-steady-state power spectrum with multiple sidebands is found in the scattered field. The relative heights of the sidebands show a time-dependence determined by the atomic relaxation, which illuminates potential applications of using the system in information transfer of quantum networks. With negligible dissipative flipping to the unsymmetrical states, the atomic relaxation time, indicating a linearly increasing pooling state fraction, is derived analytically as a function of the number of atoms.
We study the Rydberg blockade in a system of three atoms arranged in different two-dimensional geometries (linear and triangular configurations). In the strong blockade regime, we observe high-contrast, coherent collective oscillations of the single excitation probability and an almost perfect van der Waals blockade. Our data are consistent with a total population in doubly and triply excited states below 2%. In the partial blockade regime, we directly observe the anisotropy of the van der Waals interactions between |nD> Rydberg states in the triangular configuration. A simple model that only uses independently measured two-body van der Waals interactions fully reproduces the dynamics of the system without any adjustable parameter. These results are extremely promising for scalable quantum information processing and quantum simulation with neutral atoms.
Recent achievements in ultra-cold experiments have made quantum simulation of interacting many-body systems possible in a well controllable environment. Of many candidates as quantum simulators, Rydberg atoms have been extensively utilised due to its exaggerated and fascinating atomic properties. Example includes high susceptibility to electric fields and relatively long life time in comparison to atoms in low-lying states. The tunable interaction between Rydberg atoms have made them even more versatile in simulating quantum many-body systems, e.g. interacting spin-1/2 particles. We will start the thesis by reviewing these properties of Rydberg atoms and explain how they lead to the Rydberg lattice gases that of interest. Following the review of the essential knowledge of Rydberg atoms, we first study the ground states of interacting Rydberg lattice gases in both one-dimension and two-dimensions. The many-body system we are interested in is initially prepared in a Mott-insulator state, with each lattice site containing one atom that is laser coupled to its highly excited Rydberg state. The extremely huge van der Waals interactions between Rydberg atoms at close distance leads to an interesting Rydberg blockade effect. As we shall show, these strong interactions lead to rich phases and critical behaviours in the ground states of the many-body Hamiltonians that describes the systems. The aim of the first three chapters is to analyse these ground states in detail. Having investigated the static properties, we then move on to study the dynamical behaviour of a class of generic spin models which can in principal be realised by Rydberg lattice gases with tunable blockade radius. By deriving an effective master equation, and comparing it to the exact calculation, we will demonstrate how different pure initial states eventually evolve to the same equilibrium state and analysed in detail the time evolution and the steady state.
Rydberg atom arrays are powerful platforms for studying quantum many-body systems. We consider the Rydberg-Ising Hamiltonian in a ring geometry and numerically study ensembles of states generated by random global pulse sequences subject to hardware constraints and fixed evolution times. We compare the statistical properties of such states with those of Haar-random states within the relevant lattice symmetry sector. In the strong-interaction regime (short interatomic distance), the dynamics is governed by an effective blockade that restricts Hilbert-space exploration and limits entanglement growth. In this regime, level-spacing statistics of the entanglement spectrum are close to random-matrix predictions, while the distribution of measurement probabilities deviates from Porter-Thomas behavior. For weaker interactions (larger interatomic distance), the system approaches Haar-like statistics at long times, as reflected in entanglement entropy, entanglement-spectrum statistics, and the distribution of measurement probabilities. At intermediate interactions, this behavior is observed on experimentally relevant timescales. Motivated by this observation, we investigate whether individual target states can be efficiently prepared using quantum optimal control in this regime. Employing target states drawn from an ensemble with a broad entropy distribution, we observe high fidelities (infidelities between 10^-5 and 3 x 10^-2 for nine spins). Within this ensemble, the fidelity decreases with the entanglement entropy of the target state, indicating that highly entangled targets are more difficult to prepare under the considered finite-time control constraints.
Ultracold atoms confined in microtrap array is a highly versatile platform for quantum many-body physics, quantum simulation and quantum computation because of the easy scalability, long coherence time, single site addressability and controllable interactions, e.g. using Rydberg states. Here, we demonstrate an novel method to prepare versatile arrays of atomic ensembles by transferring them from a pancake shaped optical reservoir to an array of optical tweezers produced via direct projection of light patterns produced via a digital micromirror device. The size of each ensemble is smaller than the Rydberg blockade radius, such that each one can carry either 0 or 1 (collective) excitations which can then strongly interact with the neighbouring ensembles. Finally I will discuss a recent proposal to use such Rydberg arrays to realise programmable quantum systems in the form of quantum cellular automata (QCA). This opens a path to study many-body quantum dynamics in quantum and classical regimes, to engineer highly entangled quantum states and toward an inherently scalable approach to quantum information processing and computing.