Advances in research in fields such as quantum information and quantum chemistry require subtle methods for trapping particles, including ions, neutral atoms, and molecules. Here, we propose a hybrid ion-trapping method that combines a Paul trap with optical tweezers. This trap incorporates both the deep-potential characteristic of the Paul trap and the micromotion-free nature of the optical dipole trap. By modulating the optical dipole trap synchronously with the radio-frequency voltage of the Paul trap, the alternating electrical force in the trap center is fully counteracted, and the micromotion temperature of a cold trapped ion can reach the nanokelvin scale, while the trap depth exceeds 300 K. These features will allow cold collisions between an ion and an atom in the $s$ -wave regime and stably trap the produced molecular ion in the cold hybrid system. This provides a unique platform for probing the interactions between the ions and the surrounding neutral particles and enables the investigation of new reaction pathways and reaction products in the cold regime.Advances in research in fields such as quantum information and quantum chemistry require subtle methods for trapping particles, including ions, neutral atoms, and molecules. Here, we propose a hybrid ion-trapping method that combines a Paul trap with optical tweezers. This trap incorporates both the deep-potential characteristic of the Paul trap and the micromotion-free nature of the optical dipole trap. By modulating the optical dipole trap synchronously with the radio-frequency voltage of the Paul trap, the alternating electrical force in the trap center is fully counteracted, and the micromotion temperature of a cold trapped ion can reach the nanokelvin scale, while the trap depth exceeds 300 K. These features will allow cold collisions between an ion and an atom in the $s$-wave regime and stably trap the produced molecular ion in the cold hybrid system. This provides a unique platform for probing the interactions between the ions and the surrounding neutral particles and enables the investigation of new reaction pathways and reaction products in the cold regime.

arXiv:2306.10366Physical Review AppliedMay 15, 20253 citations

Cold ion–neutral collisions in a hybrid trap

W. W. Smith, Oleg P. Makarov, Jian Lin

A dual hybrid ion–neutral trap has been built to study collisions between a cloud of ultracold atoms and small numbers of co-trapped atomic or molecular ions, in a common volume. Ultracold Na atoms are trapped in a vapour-cell magneto-optical trap (MOT), via a single-mode frequency-stabilized ring-dye laser, with repumping. A linear rf quadrupole Paul ion trap, centred on the MOT, co-traps selected atomic or molecular ions, for example Ca+. Control of the initial ion temperature involves laser cooling Ca+ ions via the resonant Fraunhofer K line at 397 nm. We showed the rf ion trap can operate simultaneously with the MOT without destroying the ultracold atom cloud. The goal is to investigate the physics of ion–neutral sympathetic cooling, the cooling by neutrals of translationally cold and vibrorotationally hot molecular ions (e.g. Na2 +(v*, J*)), and the observation of other ion–neutral processes near 0 K, of potential interest in astrophysics.A dual hybrid ion–neutral trap has been built to study collisions between a cloud of ultracold atoms and small numbers of co-trapped atomic or molecular ions, in a common volume. Ultracold Na atoms are trapped in a vapour-cell magneto-optical trap (MOT), via a single-mode frequency-stabilized ring-dye laser, with repumping. A linear rf quadrupole Paul ion trap, centred on the MOT, co-traps selected atomic or molecular ions, for example Ca+. Control of the initial ion temperature involves laser cooling Ca+ ions via the resonant Fraunhofer K line at 397 nm. We showed the rf ion trap can operate simultaneously with the MOT without destroying the ultracold atom cloud. The goal is to investigate the physics of ion–neutral sympathetic cooling, the cooling by neutrals of translationally cold and vibrorotationally hot molecular ions (e.g. Na2 +(v*, J*)), and the observation of other ion–neutral processes near 0 K, of potential interest in astrophysics.

Journal of Modern OpticsNov 10, 200592 citations

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-wave regime and stably trap the produced molecular ion in the cold hybrid system. This provides a unique platform for probing the interactions between the ions and the surrounding neutral particles and enables the investigation of new reaction pathways and reaction products in the cold regime.