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arXiv:2311.10390 · Chinese Physics Letters

Relative-Intensity Squeezing of High-Order Harmonic Twin Beams

Shicheng Jiang, Konstantin E. Dorfman

Published Apr 13, 2026• 2 citations
arXivHTMLPDF

Abstract

Abstract Relative intensity squeezing (RIS) is emerging as a promising technique for performing high-precision measurements beyond the shot-noise limit. A commonly used way to produce RIS in the visible/infrared range is generating correlated “twin beams” through four-wave mixing by driving atomic resonances with weak laser beams. Here, we propose an all-optical strong-field scheme to produce a series of relative-intensity-squeezed high-order harmonic “twin beams”. Due to the nature of high-harmonic generation, the frequencies of the “twin beams” can cover a broad range of photon energy. Our proposal paves the way for the development of non-classical XUV sources and high precision spectroscopy tools in the strong-field regime.

DOI
10.1088/0256-307x/43/5/050401

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Abstract Relative intensity squeezing (RIS) is emerging as a promising technique for performing high-precision measurements beyond the shot-noise limit. A commonly used way to produce RIS in the visible/infrared range is generating correlated “twin beams” through four-wave mixing by driving atomic resonances with weak laser beams. Here, we propose an all-optical strong-field scheme to produce a series of relative-intensity-squeezed high-order harmonic “twin beams”. Due to the nature of high-harmonic generation, the frequencies of the “twin beams” can cover a broad range of photon energy. Our proposal paves the way for the development of non-classical XUV sources and high precision spectroscopy tools in the strong-field regime.
Using a nondegenerate four-wave mixing process based on a double-$\mathrm{\ensuremath{\Lambda}}$ scheme in hot cesium vapor, we generate quantum correlated twin beams with a maximum intensity-difference squeezing of 6.5 dB. The substantially improved squeezing can be mainly attributed to very good frequency and phase-difference stability between the pump and probe beams in our experiment. Intensity-difference squeezing can be observed within a wide experimental parameter range, which guarantees its robust generation. Since this scheme produces multi-spatial-mode twin beams at the Cs D1{D}_{1}D1​ line, it is of interest for experiments involving quantum imaging and coherent interfaces between atomic and solid-state systems.
We report the generation of strong, bright-beam intensity-difference squeezing down to measurement frequencies below 10 Hz. We generate two-mode squeezing in a four-wave mixing (4WM) process in Rb vapor, where the single-pass-gain nonlinear process does not require cavity locking and only relies on passive stability. We use diode laser technology and several techniques, including dual seeding, to remove the noise introduced by seeding the 4WM process as well as the background noise. Twin-beam intensity-difference squeezing down to frequencies limited only by the mechanical and atmospheric stability of the lab is achieved. These results should enable important low-frequency applications such as direct intensity-difference imaging with bright beams on integrating detectors.
Squeezed optical fields are a powerful resource for a variety of investigations in basic research and technology. However, the generation of intense squeezed light is challenging. Here, we show that intense squeezed light can be produced using strongly laser driven atoms and the so far unrelated process of high harmonic generation. We demonstrate that when the intensity of the driving field significantly depletes the ground state of the atoms, leading to dipole moment correlations, the quantum state of the driving field and the generated high harmonics are entangled and squeezed. Furthermore, we analyze how the resulting quadrature squeezing of the fundamental laser mode after the interaction can be controlled. The findings open the way for the generation of high intensity squeezed light states for a wide range of applications.
High-harmonic generation is a light up-conversion process occurring in a strong laser field, leading to coherent bursts of extreme ultrashort broadband radiation [1]. As a new perspective, we propose that ultrafast strong-field electronic or photonic processes such as high-harmonic generation can potentially generate non-classical states of light well before the decoherence of the system occurs [2, 3]. This could address fundamental challenges in quantum technology such as scalability, decoherence or the generation of massively entangled states [4]. Here, we report experimental evidence of the non-classical nature of the harmonic emission in several semiconductors excited by a femtosecond infrared laser. By investigating single- and double beam intensity cross-correlation [5], we measure characteristic, non-classical features in the single photon statistics. We observe two-mode squeezing in the generated harmonic radiation, which depends on the laser intensity that governs the transition from Super-Poissonian to Poissonian photon statistics. The measured violation of the Cauchy-Schwarz inequality realizes a direct test of multipartite entanglement in high-harmonic generation [6]. This result is supported by the theory of multimodal detection and the Hamiltonian from which the effective squeezing modes of the harmonics can be derived [7, 8]. With this work, we show experimentally that high-harmonic generation is a new quantum bosonic platform that intrinsically produces non-classical states of light with unique features such as multipartite broadband entanglement or multimode squeezing. The source operates at room temperature using standard semiconductors and a standard commercial fiber laser, opening new routes for the quantum industry, such as optical quantum computing, communication and imaging.
Abstract High-harmonic generation has been driving the development of attosecond science and sources. More recently, high-harmonic generation in solids has been adopted by other communities as a method to study material properties. However, so far high-harmonic generation has only been driven by classical light, despite theoretical proposals to do so with quantum states of light. Here we observe non-perturbative high-harmonic generation in solids driven by a macroscopic quantum state of light, a bright squeezed vacuum, which we generate in a single spatiotemporal mode. The process driven by a bright squeezed vacuum is considerably more efficient in the generation of high harmonics than classical light of the same mean intensity. Due to its broad photon-number distribution, covering states from 0 to 2 × 10 13 photons per pulse, and strong subcycle electric field fluctuations, a bright squeezed vacuum gives access to free carrier dynamics within a much broader range of peak intensities than accessible with classical light.
We analytically describe the strong-field light-electron interaction using a quantized coherent laser state with arbitrary photon number. We obtain a light-electron wave function which is a closed-form solution of the time-dependent Schrödinger equation (TDSE). This wave function provides information about the quantum optical features of the interaction not accessible by semi-classical theories. With this approach we can reveal the quantum optical properties of high harmonic generation (HHG) process in gases by measuring the photon statistics of the transmitted infrared (IR) laser radiation. This work can lead to novel experiments in high-resolution spectroscopy in extreme-ultraviolet (XUV) and attosecond science without the need to measure the XUV light, while it can pave the way for the development of intense non-classical light sources.