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arXiv:2311.09597 · Physical Review Letters

Evolution Operator Can Always Be Separated into the Product of Holonomy and Dynamic Operators

Xiao‐Dong Yu, D. M. Tong

Published Nov 15, 2023• 11 citations

Abstract

The geometric phase is a fundamental quantity characterizing the holonomic feature of quantum systems. It is well known that the evolution operator of a quantum system undergoing a cyclic evolution can be simply written as the product of holonomic and dynamical components for the three special cases concerning the Berry phase, adiabatic non-Abelian geometric phase, and nonadiabatic Abelian geometric phase. However, for the most general case concerning the nonadiabatic non-Abelian geometric phase, how to separate the evolution operator into holonomic and dynamical components is a long-standing open problem. In this Letter, we solve this open problem. We show that the evolution operator of a quantum system can always be separated into the product of holonomy and dynamic operators. Based on it, we further derive a matrix representation of this separation formula for cyclic evolution, and give a necessary and sufficient condition for a general evolution being purely holonomic. Our finding is not only of theoretical interest itself, but also of vital importance for the application of quantum holonomy. It unifies the representations of all four types of evolution concerning the adiabatic/nonadiabatic Abelian/non-Abelian geometric phase, and provides a general approach to realizing purely holonomic evolution.

DOI: 10.1103/physrevlett.131.200202

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The geometric phase is a fundamental quantity characterizing the holonomic feature of quantum systems. It is well known that the evolution operator of a quantum system undergoing a cyclic evolution can be simply written as the product of holonomic and dynamical components for the three special cases concerning the Berry phase, adiabatic non-Abelian geometric phase, and nonadiabatic Abelian geometric phase. However, for the most general case concerning the nonadiabatic non-Abelian geometric phase, how to separate the evolution operator into holonomic and dynamical components is a long-standing open problem. In this Letter, we solve this open problem. We show that the evolution operator of a quantum system can always be separated into the product of holonomy and dynamic operators. Based on it, we further derive a matrix representation of this separation formula for cyclic evolution, and give a necessary and sufficient condition for a general evolution being purely holonomic. Our finding is not only of theoretical interest itself, but also of vital importance for the application of quantum holonomy. It unifies the representations of all four types of evolution concerning the adiabatic/nonadiabatic Abelian/non-Abelian geometric phase, and provides a general approach to realizing purely holonomic evolution.

Based only on the parallel-transport condition, we present a general method to compute Abelian or non-Abelian geometric phases acquired by the basis states of pure or mixed density operators, which also holds for nonadiabatic and noncyclic evolution. Two interesting features of the non-Abelian geometric phase obtained by our method stand out: i) it is a generalization of Wilczek and Zee's non-Abelian holonomy, in that it describes nonadiabatic evolution where the basis states are parallelly transported between distinct degenerate subspaces, and ii) the non-Abelian character of our geometric phase relies on the transitional evolution of the basis states, even in the nondegenerate case. We apply our formalism to a two-level system evolving nonadiabatically under spontaneous decay to emphasize the non-Abelian nature of the geometric phase induced by the reservoir. We also show, through the generalized invariant theory, that our general approach encompasses previous results in the literature.

The issue of separating Schrödinger-type quantum time evolution into a product of holonomic and dynamical parts in the nonadiabatic non-Abelian case is examined. We identify all special cases in which this kind of separation is possible, and we prove that separability is a gauge-invariant property of quantum time evolution. The general analysis is implemented in a three-level system with Λ -type coupling structures. The typical case where the holonomic and dynamical parts do not separate is illustrated by means of two noncommuting Λ -type Hamiltonians.

We introduce a self-consistent framework for the analysis of both Abelian and non-Abelian geometric phases associated with open quantum systems, undergoing cyclic adiabatic evolution. We derive a general expression for geometric phases, based on an adiabatic approximation developed within an inherently open-systems approach. This expression provides a natural generalization of the analogous one for closed quantum systems, and we prove that it satisfies all the properties one might expect of a good definition of a geometric phase, including gauge invariance. A striking consequence is the emergence of a finite time interval for the observation of geometric phases. The formalism is illustrated via the canonical example of a spin-

1∕2

particle in a time-dependent magnetic field. Remarkably, the geometric phase in this case is immune to dephasing and spontaneous emission in the renormalized Hamiltonian eigenstate basis. This result positively impacts holonomic quantum computing.

Quantum holonomies are investigated in different contexts. A geometric phase is proposed for decomposition dependent evolution, where each component of a given decomposition of a mixed state evolves independently. It is shown that this geometric phase only depends on the path traversed in the space of decompositions. A holonomy is associated to general paths of subspaces of a Hilbert space, both discrete and continuous. This opens up the possibility of constructing quantum holonomic gates in the open path setting. In the discrete case it is shown that it is possible to associate two distinct holonomies to a given path. Interferometric setups for measuring both holonomies are provided. It is further shown that there are cases when the holonomy is only partially defined. This has no counterpart in the Abelian setting. An operational interpretation of amplitudes of density operators is provided. This allows for a direct interferometric realization of Uhlmann's parallelity condition, and the possibility of measuring the Uhlmann holonomy for sequences of density operators. Off-diagonal geometric phases are generalized to the non-Abelian case. These off-diagonal holonomies are undefined for cyclic evolution, but must contain members of non-zero rank if all standard holonomies are undefined. Experimental setups for measuring the off-diagonal holonomies are proposed. The concept of nodal free geometric phases is introduced. These are constructed from gauge invariant quantities, but do not share the nodal point structure of geometric phases and off-diagonal geometric phases. An interferometric setup for measuring nodal free geometric phases is provided, and it is shown that these phases could be useful in geometric quantum computation. A holonomy associated to a sequence of quantum maps is introduced. It is shown that this holonomy is related to the Uhlmann holonomy. Explicit examples are provided to illustrate the general idea.

Non-Abelian quantum holonomies, i.e., unitary state changes solely induced by geometric properties of a quantum system, have been much under focus in the physics community as generalizations of the Abelian Berry phase. Apart from being a general phenomenon displayed in various subfields of quantum physics, the use of holonomies has lately been suggested as a robust technique to obtain quantum gates; the building blocks of quantum computers. Non-Abelian holonomies are usually associated with cyclic changes of quantum systems, but here we consider a generalization to noncyclic evolutions. We argue that this open-path holonomy can be used to construct quantum gates. We also show that a structure of partially defined holonomies emerges from the open-path holonomy. This structure has no counterpart in the Abelian setting. We illustrate the general ideas using an example that may be accessible to tests in various physical systems.