The nature of pseudogap lies at the heart of strongly-interacting superconductivity and superfluidity. With known pairing interactions, unitary Fermi gases provide an ideal testbed to verify whether a pseudogap can arise from many-body pairing. Here we report the observation of the long-sought pair-fluctuation-driven pseudogap in homogeneous unitary Fermi gases of lithium-6 atoms, by precisely measuring the spectral function through momentum-resolved microwave spectroscopy without the serious effects of final-state effect. We find a large pseudogap above the superfluid transition. The inverse pair lifetime exhibits a thermally-activated exponential behavior, uncovering the microscopic virtual pair breaking and recombination mechanism. The obtained large, T-independent single-particle scattering rate is comparable with that set by the Planckian limit. Our findings quantitatively characterize the pseudogap in strongly-interacting Fermi gases, highlighting the role of preformed pairing as a precursor to superfluidity.
The nature of pseudogap lies at the heart of strongly-interacting superconductivity and superfluidity. With known pairing interactions, unitary Fermi gases provide an ideal testbed to verify whether a pseudogap can arise from many-body pairing. Here we report the observation of the long-sought pair-fluctuation-driven pseudogap in homogeneous unitary Fermi gases of lithium-6 atoms, by precisely measuring the spectral function through momentum-resolved microwave spectroscopy without the serious effects of final-state effect. We find a large pseudogap above the superfluid transition. The inverse pair lifetime exhibits a thermally-activated exponential behavior, uncovering the microscopic virtual pair breaking and recombination mechanism. The obtained large, T-independent single-particle scattering rate is comparable with that set by the Planckian limit. Our findings quantitatively characterize the pseudogap in strongly-interacting Fermi gases, highlighting the role of preformed pairing as a precursor to superfluidity.
The existence of a pseudogap in unitary Fermi gases has recently been established and measured experimentally [Li et al., Nature 626, 288 (2024)]. This lends strong support for the pairing origin as the mechanism of the pseudogap in Fermi superfluids. Here we present a spectral study of unitary Fermi gases, and show how the data can be understood quantitatively, when compared with theoretically calculated momentum-resolved rf or microwave spectra, and the pseudogap extracted from the spectra. We use an iterative treatment of the fermion self energy and hence the spectral function, beyond previous pseudogap approximation, based on a pairing fluctuation theory that incorporates both particle-particle and particle-hole T matrices, with self-consistent self energy feedback. Our results not only provide a microscopic explanation of the experimental data but also strengthen the support for both the pairing-induced pseudogap physics and the pairing fluctuation theory of Fermi superfluidity.
Interacting Fermi systems in two dimensions display intriguing phenomena such as high temperature superfluidity and pseudogap physics. These features emerge from the collective behavior of the constituent particles but are extremely hard to predict from microscopic theory. I will report on experiments that realize microscopic two-dimensional systems with ultracold fermionic lithium atoms. With the ability to deterministically prepare few-body ground states and to observe individual particles in momentum space, they enable a microscopic view of strongly interacting two-dimensional Fermi systems. Surprisingly, we find that characteristic features of many-body Fermi gases can already be found in systems of no more than a dozen particles: In spectroscopy, we observe collective excitations that are the few-body precursor of the Higgs amplitude mode of a superfluid. Moreover, in spin-resolved momentum space probes, we can directly image individual ‘Cooper pairs’ and show the presence of fermionic pairing even in a microscopic setting. These findings may broaden our understanding of finite-size Fermi systems, such as atomic nuclei and superconducting grains.
The pseudogap phenomenon is a hallmark of strongly interacting Fermi systems, from high-temperature superconductors to ultracold atomic gases, yet its precise origin remains debated. Here we calculate the spectral function and rf spectra of ultracold atomic gases across the BCS-BEC crossover to quantitatively investigate the pairing mechanism of the pseudogap. We advance our pairing fluctuation theory by incorporating particle-hole fluctuations, which renormalize the effective interaction in the particle-particle channel. To achieve quantitative accuracy, we employ a full numerical convolution for the pair susceptibility and self-energy, moving beyond previous analytic pseudogap approximations. This convolution approach automatically captures two critical effects: (i) the full spectral broadening of fermions due to finite pair lifetime, and (ii) the previously neglected pair-hole scattering effect, which manifests as a substantial Hartree energy. We calculate the spectral function, and use rf spectral intensity maps and energy distribution curves to determine the quasiparticle dispersion. From these, we extract the pseudogap Δ, Hartree energy, and chemical potential, mapping their evolution across the crossover. Our results show that the pseudogap emerges continuously as the system moves from the BCS regime toward BEC. Furthermore, the pair spectral function reveals that pairs become diffusive at energies above 2Δ, indicating that the pair lifetime is governed by virtual binding and unbinding processes. Our calculations achieve quantitative agreement with recent experiments across the BCS-BEC crossover, including at unitarity, providing strong support for a pairing-based origin of the pseudogap as described by our pairing fluctuation theory.
The Bose-Einstein condensate to Bardeen-Cooper-Schrieffer crossover in ultracold Fermi gases creates an ideal environment to enrich our knowledge of many-body systems. It is relevant to a wide range of fields from condensed matter to astrophysics. The nature of pairing in strongly interacting Fermi gases can be readily studied. This aids our understanding of related problems in high-Tc superconductors, whose mechanism is still under debate due to the large interaction parameter. Here, we calculate the dynamical properties of a normal, trapped strongly correlated Fermi gas, by developing a quantum cluster expansion. Our calculations for the single-particle spectral function agree with recent rf spectroscopy measurements, and clearly demonstrate pseudogap pairing in the strongly interacting regime.
The physics of the pseudogap state is intimately linked with the pairing mechanism that gives rise to superfluidity in quantum gases and to superconductivity in high- T c cuprates, and therefore, both in quantum gases and in superconductors, the pseudogap state and preformed pairs have been under intensive experimental scrutiny. Here, we develop a path integral treatment that provides a divergence-free description of the paired state in two-dimensional Fermi gases. Within this formalism, we derive the pseudogap temperature and the pair fluctuation spectral function, and compare these results with a recent experimental measurement of the pairing in the two-dimensional Fermi gas. The removal of the infrared divergence in the number equations is shown both numerically and analytically, through a study of the long-wavelength and low-energy limit of the pair fluctuation density. Besides the pseudogap temperature, the pair formation temperature and the critical temperature for superfluidity are also derived. The latter corresponds to the Berezinski–Kosterlitz–Thouless (BKT) temperature. The pseudogap temperature, which coincides with the pair formation temperature in the mean field, is found to be suppressed with respect to the pair formation temperature by fluctuations. This suppression is strongest for large binding energies of the pairs. Finally, we investigate how the pair formation temperature, the pseudogap temperature and the BKT temperature behave as a function of both binding energy and imbalance between the pairing partners in the Fermi gas. This allows us to set up phase diagrams for the two-dimensional Fermi gas, in which the superfluid phase, the phase-fluctuating quasicondensate and the normal state can be identified.
We investigate single-particle properties of a one-component Fermi gas with a tunable p-wave interaction. Including pairing fluctuations associated with this anisotropic interaction within a T-matrix theory, we calculate the single-particle density of states, as well as the spectral weight, above the superfluid transition temperature Tc. Starting from the weak-coupling regime, we show that the so-called pseudogap first develops in these quantities with increasing the interaction strength. However, when the interaction becomes strong to some extent, the pseudogap becomes obscure to eventually disappear in the intermediate coupling regime. In the strong-coupling regime, the excitation gap associated with the formation of tightly bound molecules again opens. This nonmonotonic interaction dependence of the excitation gap is quite different from the case of an s-wave interaction, where the pseudogap simply develops with increasing the interaction strength, which continuously changes into the molecular excitation gap. The difference between the two cases is shown to originate from the momentum dependence of the p-wave interaction, which vanishes in the low momentum limit. We also identify the pseudogap regime in the phase diagram with respect to the temperature and the p-wave interaction strength. Since the pseudogap is a precursor phenomenon of the superfluid phase transition, our results would be useful for the research toward the realization of p-wave superfluid Fermi gases.