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arXiv:2310.11193 · Physical Review Research

Thermally induced localization of dopants in a magnetic spin ladder

K. Knakkergaard Nielsen

Published Jun 25, 2024• 3 citations
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Abstract

I unveil an emergent localization phenomenon pertaining to the motion of a dopant in a thermal spin lattice. This is rendered localized by thermal spin fluctuations, whereby it is in stark constrast to the intrinsic origin of Anderson localization for quenched disorder. The system of interest consists of spin- 1 / 2 particles organized in a two-leg ladder with nearest-neighbor Ising interactions J . The motion of a hole—the dopant—is initialized by suddenly removing a spin from the thermal spin ensemble, which then moves along the ladder via nearest-neighbor hopping t . I find that the hole remains for all values of J / t and for nonzero temperatures. The origin is an effective disorder potential seen by the hole and induced by thermal spin fluctuations. Its length scale is found to match with the underlying spin-spin correlation length at low temperatures. For ferromagnetic couplings ( J < 0 ), the associated localization length of the hole increases with decreasing temperature and becomes proportional to the correlation length at low temperatures, asymptotically delocalizing at low temperatures. For antiferromagnetic couplings ( J > 0 ), there is a smooth crossover between thermal localization at high temperatures to localization driven by the antiferromagnetic order at low temperatures. At infinite temperatures, the dynamics becomes independent of the sign of the spin coupling, whereby the localization length is a universal function of | J | / t , diverging as ( t / J ) 2 for | J | ≪ t . Finally, I analyze a setup with Rydberg-dressed atoms, which naturally realizes finite-range Ising interactions, accessible in current experimental setups. I show that the discovered localization phenomenon can be probed on experimentally accessible length- and timescales, providing a strong testing ground for my predictions. Published by the American Physical Society 2024

DOI
10.1103/physrevresearch.6.023325

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•Jan 1, 2004•0 citations
I unveil an emergent localization phenomenon pertaining to the motion of a dopant in a thermal spin lattice. This is rendered localized by thermal spin fluctuations, whereby it is in stark constrast to the intrinsic origin of Anderson localization for quenched disorder. The system of interest consists of spin- 1 / 2 particles organized in a two-leg ladder with nearest-neighbor Ising interactions J . The motion of a hole—the dopant—is initialized by suddenly removing a spin from the thermal spin ensemble, which then moves along the ladder via nearest-neighbor hopping t . I find that the hole remains for all values of J / t and for nonzero temperatures. The origin is an effective disorder potential seen by the hole and induced by thermal spin fluctuations. Its length scale is found to match with the underlying spin-spin correlation length at low temperatures. For ferromagnetic couplings ( J < 0 ), the associated localization length of the hole increases with decreasing temperature and becomes proportional to the correlation length at low temperatures, asymptotically delocalizing at low temperatures. For antiferromagnetic couplings ( J > 0 ), there is a smooth crossover between thermal localization at high temperatures to localization driven by the antiferromagnetic order at low temperatures. At infinite temperatures, the dynamics becomes independent of the sign of the spin coupling, whereby the localization length is a universal function of | J | / t , diverging as ( t / J ) 2 for | J | ≪ t . Finally, I analyze a setup with Rydberg-dressed atoms, which naturally realizes finite-range Ising interactions, accessible in current experimental setups. I show that the discovered localization phenomenon can be probed on experimentally accessible length- and timescales, providing a strong testing ground for my predictions. Published by the American Physical Society 2024
I investigate the motion of a single hole in 2D spin lattices with square and triangular geometries. While the spins have nearest neighbor Ising spin couplings J J , the hole is allowed to move only in 1D along a single line in the 2D lattice with nearest neighbor hopping amplitude t t . The non-equilibrium hole dynamics is initialized by suddenly removing a single spin from the thermal Ising spin lattice. I find that for any nonzero spin coupling and temperature, the hole is localized. This is an extension of the thermally induced localization phenomenon [Phys. Rev. Res. 6, 023325 (2024)] to the case, where there is a phase transition to a long-range ordered ferromagnetic phase. The dynamics depends only on the ratio of the temperature to the spin coupling, k_BT / |J| k B T / | J | , and on the ratio of the spin coupling to the hopping J/t J / t . I characterize these dependencies in great detail. In particular, I find universal behavior at high temperatures, common features for the square and triangular lattices across the Curie temperatures for ferromagnetic interactions, and highly distinct behaviors for the two geometries in the presence of antiferromagnetic interactions due geometric frustration in the triangular lattice.
The motion of dopants in magnetic spin lattices has received tremendous attention for at least four decades due to its connection to high-temperature superconductivity. Despite these efforts, we lack a complete understanding of their behavior, especially out of the equilibrium and at nonzero temperatures. In this paper, we take a significant step towards a much deeper understanding based on state-of-the-art matrix-product-state calculations. In particular, we investigate the nonequilibrium dynamics of a dopant in two-leg t − J ladders with antiferromagnetic XXZ spin interactions. In the Ising limit, we find that the dopant is for all investigated temperatures due to an emergent disordered potential, with a localization length controlled by the underlying correlation length of the spin lattice, which increases exponentially with decreasing temperature. The dopant, hereby, only delocalizes asymptotically in the zero temperature limit. This greatly generalizes the localization effect discovered recently in Hilbert space fragmented models [, ]. In the presence of spin-exchange processes at rate α , the dopant diffuses with a diffusion coefficient, D h , depending nonmonotonically on α . It initially increases linearly as D h ∝ α for α ≪ 1 before dropping off as α − 1 for α > 1 . Moreover, we show that the underlying spin dynamics at infinite temperature behaves qualitatively the same, albeit with important quantitative differences. We substantiate these findings by showing that the dynamics features self-similar scaling behavior, which strongly deviates from the Gaussian behavior of regular diffusion, especially for weak spin exchange. Finally, we show that the diffusion coefficient D h follows an Arrhenius relation at high temperatures, whereby it is exponentially suppressed upon cooling.
I demonstrate a pairing mechanism of dopants in a magnetic lattice, emerging from the underlying of the spins. The effect is demonstrated in a mixed-dimensional model, where dopants travel along a two-leg ladder, while the spins feature Ising interactions along the rungs and the legs of the ladder. The dynamics following the sudden immersion of two nearest neighbor dopants in an infinite temperature spin lattice shows that thermal spin disorder frustrates the relative motion of the dopants and enforces them to copropagate. The predictions are shown to be realistically testable in quantum simulation experiments.
The fate of a hole injected in an antiferromagnet is an outstanding issue of strongly correlated physics. It provides important insights into doped Mott insulators closely related to high-temperature superconductivity. Here, we report a systematic numerical study of t-J ladder systems based on the density matrix renormalization group. It reveals a surprising result for the single hole's motion in an otherwise well-understood undoped system. Specifically, we find that the common belief of quasiparticle picture is invalidated by the self-localization of the doped hole. In contrast to Anderson localization caused by disorders, the charge localization discovered here is an entirely new phenomenon purely of strong correlation origin. It results from destructive quantum interference of novel signs picked up by the hole, and since the same effect is of a generic feature of doped Mott physics, our findings unveil a new paradigm which may go beyond the single hole doped system.
A long-standing issue in the physics of strongly correlated electronic systems is whether the motion of a single hole in quantum antiferromagnets can be understood in terms of the quasiparticle picture. Very recently, investigations of this issue have been within the experimental reach. Here we perform a large-scale density matrix renormalization group study, and provide the first unambiguous numerical evidence showing that in ladder systems, a single hole doped in the Mott antiferromagnet does not behave as a quasiparticle. Specifically, the injected hole is found to be always localized as long as the leg number is larger than one, with a vanishing quasiparticle weight and a localization length monotonically decreasing with the leg number. In addition, the single hole self-localization is insensitive to the parity (even-odd) of the leg number. Our findings may advance conceptual developments in different fields of condensed matter physics. First of all, the intriguing self-localization phenomenon is of pure strong correlation origin free of extrinsic disorders. Therefore, it is in sharp contrast to the well-known Anderson localization and recently found many-body localization, where extrinsic disordered potentials play crucial roles. Second, they confirm the analytical predictions of the so-called phase string theory, suggesting that the phase string effect lies in the core of the physics of doped Mott antiferromagnets.
A proper theoretical description of doped antiferromagnets is until now an unresolved issue. In this work we study chain and ladder systems, and in particularly we focus on the physically most interesting two leg ladder. Our starting point is the Spin Fermion model in which an antiferromagnetic background of localized spins interacts with mobile holes via a rotation invariant Kondo-like term. The interesting region of the phase diagram is that close to the Mott-insulator transition where the doping delta is zero. At zero doping in fact the system is an insulator and the spins organize themselves in a spin liquid, a rotational invariant state characterized by a finite correlation length and an energy gap (a spin gap) above the ground state. Such a state is also the ground state of a field theory, the non linear sigma model (NLsigmaM) which is recognized as the low energy effective theory for antiferromagnetic spin ladder. The first question we answer is how such a spin state evolves as one moves off from the Mott phase by increasing the doping. Integrating out the fermions in our model we obtain an effective theory for the spins which we are able to evaluate in the continuum limit. The effective theory is again a NLsigmaM with coupling constants which depend on the concentration of dopant holes. In contrast to existing mean field calculation our theory predicts a lowering of the spin gap with doping and a consequent increase in the correlation length. Indeed a lowering of the spin gap due to doping is also observed in numerical simulation and on NMR experiments on $Sr14-xCaxCu24O41 with which we obtain very good agreement. Secondly we concentrated on the behavior of the fermions. The general paradigm of interacting fermions in one dimension is that of the Luttinger Liquid characterized by bosonic excitations and spin charge separation. By generalizing our approach we are able to access the one particle fermion propagator as a quantity averaged over the NLsigmaM which controls the spin background. We see that in the limit of zero doping the quasiparticle weight Z is non-zero in a neighborhood of the Fermi energy. This in turn implies that the Luttinger liquid parameter Krho goes to one as the doping delta goes to zero as was first argued by Schulz. Our stronger result allows us to assert that in the very low doping regime the fermions constitute a Fermi liquid.