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arXiv:2309.17305 · Physical Review Letters

Precise Photoexcitation Measurement of Tan’s Contact in the Entire BCS-BEC Crossover

Manuel Jäger, Johannes Hecker Denschlag

Published Jun 25, 2024• 9 citations
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Abstract

We study two-body correlations in a spin-balanced ultracold harmonically trapped Fermi gas of ^{6}Li atoms in the crossover from the Bardeen-Cooper-Schrieffer (BCS) to the Bose-Einstein-Condensate (BEC) regime. For this, we precisely measure Tan's contact using a novel method based on photoexcitation of atomic pairs, which was recently proposed by Wang et al. [Photoexcitation measurement of Tan's contact for a strongly interacting Fermi gas, Phys. Rev. A 104, 063309 (2021).PLRAAN2469-992610.1103/PhysRevA.104.063309]. We map out the contact in the entire phase diagram of the BCS-BEC crossover for various temperatures and interaction strengths, probing regions in phase space that have not been investigated yet. Our measurements reach an uncertainty of ≈2% at the lowest temperatures and thus represent a precise quantitative benchmark. By comparison to our data, we localize the regions in phase space where theoretical predictions and interpolations give valid results. In regions where the contact is already well known we find excellent agreement with our measurements. Thus, our results demonstrate that photoinduced loss is a precise probe to measure quantum correlations in a strongly interacting Fermi gas.

DOI
10.1103/physrevlett.132.263401

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We study two-body correlations in a spin-balanced ultracold harmonically trapped Fermi gas of ^{6}Li atoms in the crossover from the Bardeen-Cooper-Schrieffer (BCS) to the Bose-Einstein-Condensate (BEC) regime. For this, we precisely measure Tan's contact using a novel method based on photoexcitation of atomic pairs, which was recently proposed by Wang et al. [Photoexcitation measurement of Tan's contact for a strongly interacting Fermi gas, Phys. Rev. A 104, 063309 (2021).PLRAAN2469-992610.1103/PhysRevA.104.063309]. We map out the contact in the entire phase diagram of the BCS-BEC crossover for various temperatures and interaction strengths, probing regions in phase space that have not been investigated yet. Our measurements reach an uncertainty of ≈2% at the lowest temperatures and thus represent a precise quantitative benchmark. By comparison to our data, we localize the regions in phase space where theoretical predictions and interpolations give valid results. In regions where the contact is already well known we find excellent agreement with our measurements. Thus, our results demonstrate that photoinduced loss is a precise probe to measure quantum correlations in a strongly interacting Fermi gas.
In a parallel publication [Phys. Rev. Lett. 132, 263401 (2024)] we demonstrate that photoinduced two-body loss can be used to measure Tan's contact with high precision in a two-component Fermi gas. Here, in the present companion paper, we provide relevant background information on this work and describe in detail the methodology for both the experiments and the data analysis. We first review various theoretical approaches for calculating the contact and identify areas in phase space of the spin-balanced Fermi gas where Tan's contact has not yet been determined. Next, we provide detailed information on our experimental methods, in particular, explaining the measurement and calibration procedures to achieve a high-precision results for the contact. Afterwards, we study the variation of the decay laws of two-body loss in a Fermi gas in the crossover from the Bardeen-Cooper-Schrieffer (BCS) to the Bose-Einstein-condensate (BEC) regime, verifying previous predictions. Finally, we determine the closed-channel fraction of the Fermi gas and compare it to previous measurements and theoretical calculations.
Ultracold atomic gases are a powerful tool to experimentally study strongly correlated quantum many-body systems. In particular, ultracold Fermi gases with tunable interactions have allowed to realize the famous BEC-BCS crossover from a Bose-Einstein condensate (BEC) of molecules to a Bardeen-Cooper-Schrieffer (BCS) superfluid of weakly bound Cooper pairs. However, large parts of the excitation spectrum of fermionic superfluids in the BEC-BCS crossover are still unexplored. In this work, we use Bragg spectroscopy to measure the full momentum-resolved low-energy excitation spectrum of strongly interacting ultracold Fermi gases. This enables us to directly observe the smooth transformation from a bosonic to a fermionic superfluid that takes place in the BEC-BCS crossover. We also use our spectra to determine the evolution of the superfluid gap and find excellent agreement with previous experiments and self-consistent T-matrix calculations both in the BEC and crossover regime. However, toward the BCS regime a calculation that includes the effects of particle-hole correlations shows better agreement with our data.
The nature of the normal phase of an ultracold Fermi gas in the BCS-BEC crossover regime is an interesting and unresolved question. As interactions increase, while the many-body ground state remains a condensate of paired fermions, the normal state must evolve from a Fermi liquid to a Bose gas of molecules. In this thesis, I present a technique to spatially select a homogeneous sample from the center of a trapped gas to explore this crossover. Combining this technique with RF spectroscopy, we locally measure Tan's contact as a function of temperature and compare to various many-body theories. In another experiment, we measure the distribution of single-particle energies and momenta for a normal gas across the BCS-BEC crossover. We find that the data fit well to a two-part function that includes a peak corresponding to fermionic quasiparticles and an "incoherent background" that is modeled using the dispersion of thermal molecules. I also describe the construction of a new-generation Fermi gas apparatus.
The crossover from weak-coupling Bardeen-Cooper-Schrieffer (BCS) pairing to a Bose-Einstein condensate (BEC) of tightly bound pairs, as a function of the attractive interaction in Fermi systems, has long been of interest to theoretical physicists. The past decade has seen a series of remarkable experimental developments in ultracold Fermi gases that have realized the BCS-BEC crossover in the laboratory, bringing with it fresh new insights into the very strongly interacting unitary regime in the middle of this crossover. In this review, we start with a pedagogical introduction to the crossover and then focus on recent progress in the strongly interacting regime. Although our focus is on new theoretical developments, we also describe three key experiments that probe the thermodynamics, transport, and spectroscopy of the unitary Fermi gas. We discuss connections between the unitary regime and other areas of physics—quark-gluon plasmas, gauge-gravity duality, and high-temperature superconductivity—and conclude with open questions about strongly interacting Fermi gases.
The pairing of fermionic particles is an essential ingredient of superconductivity and of the superfluidity of 3He. While such phenomena are accurately described by BCS theory in the limit of weak pairing strength, a complete understanding remains elusive when pairing strength is increased, such as in high temperature superconductors. We create ultracold gases of trapped fermionic 6Li atoms, through which we directly observe fermionic pairing. In our system, there are no impurities whatsoever, and parameters such as the number and temperature of the trapped atoms are precisely and independently controlled. In addition, a Feshbach resonance enables the continuous tuning of interaction strength and sign between the paired atoms. This control allows us to observe the smooth crossover of a molecular Bose Einstein condensate (MBEC) to a superfluid of weakly interacting Cooper pairs. With these tools, we have performed several fundamental measurements of pairing in fermionic systems.\nWe use optical molecular spectroscopy to precisely measure the closed-channel contribution to the many body state of paired 6Li atoms within a broad Feshbach resonance. The magnitude of this contribution is small, and supports the concept of universality for the description of broad Feshbach resonances. Moreover, the dynamics of the excitation provide clear evidence for pairing across the BEC-BCS crossover, and for the first time, into the weakly interacting BCS regime.\nWe also prepare a polarized Fermi gas with unequal numbers of two spin states of 6Li atoms. The real-space densities of the polarized, strongly-interacting, two-component Fermi gas reveal two low temperature regimes. At the lowest temperatures, the gas separates into a phase with a uniformly paired superfluid core surrounded by a shell of normal, unpaired atoms. This phase separation is accompanied by a spatial deformation of the core. At higher temperatures, the uniformly paired core persists, though it does not deform. This temperature dependence is consistent with a tri-critical point in the phase diagram. These measurements of pairing in a polarized Fermi gas are relevant to predictions of exotic phases of quark matter and magnetized superconductors.
We investigate the crossover from Bardeen-Cooper-Schrieffer (BCS) superfluidity to Bose-Einstein condensation (BEC) in a two-dimensional Fermi gas at T=0 using the fixed-node diffusion Monte Carlo method. We calculate the equation of state and the gap parameter as a function of the interaction strength, observing large deviations compared to mean-field predictions. In the BEC regime our results show the important role of dimer-dimer and atom-dimer interaction effects that are completely neglected in the mean-field picture. Results on Tan's contact parameter associated with short-range physics are also reported along the BCS-BEC crossover.