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arXiv:2309.10261 · Physics Letters B

Visualizing quantum coherence and decoherence in nuclear reactions

K. Hagino, Takuya Yoda

Published Nov 15, 2023• 5 citations
arXivHTMLPDF

Abstract

Differential cross sections of nuclear reactions often exhibit characteristic oscillations in the angular distribution originated from an interference of two indistinguishable processes. Here we propose a novel method to visualize origins of such oscillations. This is achieved by taking Fourier transform of scattering amplitudes, following the idea in wave optics. We apply this method to elastic scattering of 16O+16O and 18O+18O at energies above the Coulomb barrier. The former system shows strong oscillations in the angular distribution due to the nearside-farside interferences, while the oscillations are largely suppressed in the latter system due to a stronger absorption. We show that the image of the former and the latter systems corresponds to a double-slit and a single-slit problems in quantum mechanics, respectively.

DOI
10.1016/j.physletb.2023.138326

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Differential cross sections of nuclear reactions often exhibit characteristic oscillations in the angular distribution originated from an interference of two indistinguishable processes. Here we propose a novel method to visualize origins of such oscillations. This is achieved by taking Fourier transform of scattering amplitudes, following the idea in wave optics. We apply this method to elastic scattering of 16O+16O and 18O+18O at energies above the Coulomb barrier. The former system shows strong oscillations in the angular distribution due to the nearside-farside interferences, while the oscillations are largely suppressed in the latter system due to a stronger absorption. We show that the image of the former and the latter systems corresponds to a double-slit and a single-slit problems in quantum mechanics, respectively.
In quantum mechanics the Young-type double-slit experiment can be performed with electrons either traveling through a double slit or being coherently emitted from two inversion symmetric molecular sites. In the latter one the valence photoionization cross sections of homonuclear diatomic molecules were predicted to oscillate over kinetic energy almost 50 years ago. Beyond the direct proof of the oscillatory behavior of these photoionization cross sections σ, we show that the angular distribution of the emitted electrons reveals hitherto unexplored information on the relative phase shift between the corresponding partial waves through two-center interference patterns.
We describe a method for obtaining the scattering matrix for nuclear or chemical reactions on a finite lattice. Aside from the preparation of the initial and final states as wave packets, the only other operation required is unitary time evolution, making this approach ideal for simulations on quantum hardware. The central quantity is a time-dependent overlap between incoming and outgoing wave packets whose Fourier transform corresponds to the scattering matrix at fixed energy, from which one can calculate elastic and inelastic cross sections for reactions involving two interacting clusters. Working in Cartesian coordinates enables an efficient encoding of the problem on quantum hardware via the first quantization mapping, with favorable qubit scaling for describing asymptotic scattering states. Within this framework, we describe a quantum algorithm for probing the scattering amplitude through different angles, including the forward direction, which provides access to the total cross section via the optical theorem. We demonstrate our methods through a series of numerical examples, for both elastic and inelastic processes, comparing against exact calculations. The techniques we describe can more readily be extended to a large number of constituent particles than other existing approaches, once fault-tolerant quantum hardware becomes available.
We include the dynamics of the angular straggling process in the angular distributions of Mott scattering of heavy ions. We model the passage of an incoming nucleus through a target as a diffusion process. It is then possible to derive a simple and physically transparent expression for the angular dispersion due to the straggling. The angular dispersion should be folded with the theoretical Mott cross section to see its effect on the amplitude of the Mott oscillations. Our results agree very well with data of 208{}^{208}208Pb + 208{}^{208}208Pb scattering. We define the ``classical'' limit as the limit when the angular dispersion due to straggling becomes comparable with the Mott oscillation period and get the disappearance of quantum interference occurring at the limit $0.050\sqrt{\ensuremath{\xi}}\frac{{Z}^{4}}{{E}^{3/2}}\ensuremath{\ge}1$, where $\ensuremath{\xi}$ stands for the target thickness, ZZZ is the system's charge, and EEE is the center-of-mass energy. The experiments on lead are very close to this limit. We show that the kinematical correlations due to the identity of the particles is maintained, as it should be, and the action of the environment is to reduce the fringe visibility.
Young's classic double-slit experiment demonstrates the reality of interference when waves and particles travel simultaneously along two different spatial paths. Here, we propose a double-slit experiment in momentum space, realized in the free-space elastic scattering of vortex electrons. We show that this process proceeds along two paths in momentum space, which are well localized and well separated from each other. For such vortex beams, the (plane-wave) amplitudes along the two paths acquire adjustable phase shifts and produce interference fringes in the final angular distribution. We argue that this experiment can be realized with the present-day technology. We show that it gives experimental access to the Coulomb phase, a quantity which plays an important role in all charged particle scattering but which usual scattering experiments are insensitive to.
Atomic nuclei are complex, quantum many-body systems whose structure manifests itself through intrinsic quantum states associated with different excitation modes or degrees of freedom.Collective modes (vibration and/or rotation) dominate at low energy (near the ground-state).The associated states are usually employed, within a truncated model space, as a basis in (coherent) coupled channels approaches to low-energy reaction dynamics.However, excluded non-collective states can be essential, and their effects on the open (nuclear) system dynamics are usually treated through complex potentials.Is this a complete description of open system dynamics?Does it include effects of quantum decoherence?Can decoherence be manifested in reaction observables?This paper discusses these issues and the main ideas of a coupled-channels density-matrix approach that makes it possible to quantify the role and importance of quantum decoherence in low-energy nuclear reaction dynamics.Some topical applications are highlighted.