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arXiv:2309.07206 · Nature Communications

Reversibility of quantum resources through probabilistic protocols

Bartosz Regula, Ludovico Lami

Published Apr 17, 2024• 18 citations
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Abstract

Among the most fundamental questions in the manipulation of quantum resources such as entanglement is the possibility of reversibly transforming all resource states. The key consequence of this would be the identification of a unique entropic resource measure that exactly quantifies the limits of achievable transformation rates. Remarkably, previous results claimed that such asymptotic reversibility holds true in very general settings; however, recently those findings have been found to be incomplete, casting doubt on the conjecture. Here we show that it is indeed possible to reversibly interconvert all states in general quantum resource theories, as long as one allows protocols that may only succeed probabilistically. Although such transformations have some chance of failure, we show that their success probability can be ensured to be bounded away from zero, even in the asymptotic limit of infinitely many manipulated copies. As in previously conjectured approaches, the achievability here is realised through operations that are asymptotically resource non-generating, and we show that this choice is optimal: smaller sets of transformations cannot lead to reversibility. Our methods are based on connecting the transformation rates under probabilistic protocols with strong converse rates for deterministic transformations, which we strengthen into an exact equivalence in the case of entanglement distillation.

DOI
10.1038/s41467-024-47243-2

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Among the most fundamental questions in the manipulation of quantum resources such as entanglement is the possibility of reversibly transforming all resource states. The key consequence of this would be the identification of a unique entropic resource measure that exactly quantifies the limits of achievable transformation rates. Remarkably, previous results claimed that such asymptotic reversibility holds true in very general settings; however, recently those findings have been found to be incomplete, casting doubt on the conjecture. Here we show that it is indeed possible to reversibly interconvert all states in general quantum resource theories, as long as one allows protocols that may only succeed probabilistically. Although such transformations have some chance of failure, we show that their success probability can be ensured to be bounded away from zero, even in the asymptotic limit of infinitely many manipulated copies. As in previously conjectured approaches, the achievability here is realised through operations that are asymptotically resource non-generating, and we show that this choice is optimal: smaller sets of transformations cannot lead to reversibility. Our methods are based on connecting the transformation rates under probabilistic protocols with strong converse rates for deterministic transformations, which we strengthen into an exact equivalence in the case of entanglement distillation.
The quantum relative entropy is known to play a key role in determining the asymptotic convertibility of quantum states in general resource-theoretic settings, often constituting the unique monotone that is relevant in the asymptotic regime. We show that this is no longer the case when one allows stochastic protocols that may only succeed with some probability, in which case the quantum relative entropy is insufficient to characterize the rates of asymptotic state transformations, and a new entropic quantity based on a regularization of the Hilbert projective metric comes into play. Such a scenario is motivated by a setting where the cost associated with transformations of quantum states, typically taken to be the number of copies of a given state, is instead identified with the size of the quantum memory needed to realize the protocol. Our approach allows for constructing transformation protocols that achieve strictly higher rates than those imposed by the relative entropy. Focusing on the task of resource distillation, we give broadly applicable strong converse bounds on the asymptotic rates of probabilistic distillation protocols, and show them to be tight in relevant settings such as entanglement distillation with nonentangling operations. This generalizes and extends previously known limitations that are only applicable to deterministic protocols. Our methods are based on recent results for probabilistic one-shot transformations as well as a new asymptotic equipartition property for the projective relative entropy.
We develop two general approaches to characterising the manipulation of quantum states by means of probabilistic protocols constrained by the limitations of some quantum resource theory. First, we give a general necessary condition for the existence of a physical transformation between quantum states, obtained using a recently introduced resource monotone based on the Hilbert projective metric. In all affine quantum resource theories (e.g. coherence, asymmetry, imaginarity) as well as in entanglement distillation, we show that the monotone provides a necessary and sufficient condition for one-shot resource convertibility under resource-non-generating operations, and hence no better restrictions on all probabilistic protocols are possible. We use the monotone to establish improved bounds on the performance of both one-shot and many-copy probabilistic resource distillation protocols. Complementing this approach, we introduce a general method for bounding achievable probabilities in resource transformations under resource-non-generating maps through a family of convex optimisation problems. We show it to tightly characterise single-shot probabilistic distillation in broad types of resource theories, allowing an exact analysis of the trade-offs between the probabilities and errors in distilling maximally resourceful states. We demonstrate the usefulness of both of our approaches in the study of quantum entanglement distillation.
Quantum resource distillation converts imperfect resource states into highly resourceful targets and is a central task in quantum information processing. When distillation is probabilistic, unfavorable outcomes may be discarded and the quality of the output is evaluated conditioned on success, leading to a notion of reliability that differs from the deterministic setting. Here we study the conditional error exponents of probabilistic quantum resource distillation under approximately resource-nongenerating instruments and derive its general connection to the postselected composite quantum hypothesis testing against the corresponding set of free states. This reduction leads naturally to scale-invariant projective distinguishability measures and provides finite-blocklength bounds for a broad class of resource theories. We apply the framework to entanglement, coherence, and magic. For entanglement and magic, we obtain exact zero-rate asymptotic characterizations of the conditional error exponent in terms of regularized projective distinguishability, while for coherence we derive general finite-blocklength and asymptotic bounds. For representative entangled and magic states, the resulting quantities can be evaluated analytically and reveal regimes in which postselection yields a strictly larger conditional error exponent than deterministic distillation. Furthermore, we also show that the conditional error exponents for probabilistic entanglement distillation under a strictly positive success probability constraint are smaller than those with no constraints on the success probability.
Quantum resource theories provide a mathematically rigorous way of understanding the nature of various quantum resources. An important problem in any quantum resource theory is to determine how quantum states can be converted into each other within the physical constraints of the theory. The standard approach to this problem is to study approximate or probabilistic transformations. Here, we investigate the intermediate regime, providing limits on both, the fidelity and the probability of state transformations. We derive limitations on the transformations, which are valid in all quantum resource theories, by providing bounds on the maximal transformation fidelity for a given transformation probability. As an application, we show that these bounds imply an upper bound on the asymptotic rates for various classes of states under probabilistic transformations. We also show that the deterministic version of the single copy bounds can be applied for drawing limitations on the manipulation of quantum channels, which goes beyond the previously known bounds of channel manipulations. Furthermore, we completely solve the question of stochastic-approximate state conversion via local operations and classical communication in the following two cases: (i) Both initial and target states are pure bipartite entangled states of arbitrary dimensions. (ii) The target state is a two-qubit entangled state and the initial state is a pure bipartite state.
The manipulation of quantum entanglement is fundamentally irreversible: some mixed entangled states require pure entanglement for their preparation, although no pure entanglement can be recovered from them by local operations and classical communication. This irreversibility is known to persist even under the maximal class of operations that do not generate entanglement, revealing a fundamental distinction between entanglement theory and thermodynamics. We construct cases for which any attempt to restore reversibility necessarily incurs an error that increases exponentially with the number of copies. Technically, we demonstrate a strict separation between the exponential strong-converse distillable entanglement and the exponential strong-converse entanglement cost. Our result resolves a conjecture posed by Lami and Regula (Nat. Phys. 19, 184-189 (2023)) and strengthens it by showing that the irreversibility of entanglement persists even at the level of polynomially (in the number of copies) growing error. We further derive a semidefinite-programming lower bound on the exponential strong-converse cost under non-entangling operations. Finally, for the class of completely PPT-preserving operations, we construct analytically solvable families of antisymmetric states exhibiting the exponential strong-converse irreversibility. Remarkably, to our knowledge, no analogous separation between exponential strong converse cost and the analogous distillable entanglement is currently known even under the more restrictive class of LOCC operations.