Abstract Single-photon sources based on semiconductor quantum dots find several applications in quantum information processing due to their high single-photon indistinguishability, on-demand generation, and low multiphoton emission. In this context, the generation of entangled photons represents a challenging task with a possible solution relying on the interference in probabilistic gates of identical photons emitted at different pulses from the same source. In this work, we implement this approach via a simple and compact design that generates entangled photon pairs in the polarization degree of freedom. We operate the proposed platform with single photons produced through two different pumping schemes, the resonant excited one and the longitudinal-acoustic phonon-assisted configuration. We then characterize the produced entangled two-photon states by developing a complete model taking into account relevant experimental parameters, such as the second-order correlation function, Hong–Ou–Mandel visibility, multiphoton emission and pump laser filtering. Our source shows long-term stability and high quality of the generated entangled states, thus constituting a reliable building block for optical quantum technologies.
Abstract Single-photon sources based on semiconductor quantum dots find several applications in quantum information processing due to their high single-photon indistinguishability, on-demand generation, and low multiphoton emission. In this context, the generation of entangled photons represents a challenging task with a possible solution relying on the interference in probabilistic gates of identical photons emitted at different pulses from the same source. In this work, we implement this approach via a simple and compact design that generates entangled photon pairs in the polarization degree of freedom. We operate the proposed platform with single photons produced through two different pumping schemes, the resonant excited one and the longitudinal-acoustic phonon-assisted configuration. We then characterize the produced entangled two-photon states by developing a complete model taking into account relevant experimental parameters, such as the second-order correlation function, Hong–Ou–Mandel visibility, multiphoton emission and pump laser filtering. Our source shows long-term stability and high quality of the generated entangled states, thus constituting a reliable building block for optical quantum technologies.
During recent years, quantum dots have become an increasingly established source of highly entangled photons 1. The main motivation for the development of this technology has resided in the expectation that a resonantly driven quantum emitter can offer a path towards on-demand photon pair generation 2. In fact, state-of-the-art sources relying on spontaneous parametric down-conversion intrinsically suffer from multipair emission at high pair generation rates, which causes a tradeoff between brightness and degree of entanglement 3. Despite the key importance of this aspect, the experimental study of how multiphoton emission affects the entanglement properties of quantum dot-based sources has received surprisingly little attention. In this paper we report the investigation of the multipair emission of the source under quasi-deterministic resonant two-photon excitation without filtering the excitation laser using polarization suppression. The focus is on measuring the real multipair emission entering in entanglement-based measurements, minimizing measurement artefacts from the setup and in particular from the excitation source. This is investigated by measuring the second-order correlation function at zero-time delay in several measurement conditions, including spectral filtering. Our work confirms that the multipair emission is provided also for entanglement-based measurement conditions and thus helps the design of efficient photon sources for quantum information and communication technologies.
Engineering single-photon states endowed with orbital angular momentum (OAM) is a powerful tool for quantum information photonic implementations. Indeed, due to its unbounded nature, OAM is suitable for encoding qudits, allowing a single carrier to transport a large amount of information. Most of the experimental platforms employ spontaneous parametric down-conversion processes to generate single photons, even if this approach is intrinsically probabilistic, leading to scalability issues for an increasing number of qudits. Semiconductor quantum dots (QDs) have been used to get over these limitations by producing on-demand pure and indistinguishable single-photon states, although only recently they have been exploited to create OAM modes. Our work employs a bright QD single-photon source to generate a complete set of quantum states for information processing with OAM-endowed photons. We first study hybrid intraparticle entanglement between OAM and polarization degrees of freedom of a single photon whose preparation was certified by means of Hong–Ou–Mandel visibility. Then, we investigate hybrid interparticle OAM-based entanglement by exploiting a probabilistic entangling gate. The performance of our approach is assessed by performing quantum state tomography and violating Bell inequalities. Our results pave the way for the use of deterministic sources for the on-demand generation of photonic high-dimensional quantum states.
A standard laser produces a coherent state of light with a Poissonian photon number distribution. Generation of single photons on demand is a key requirement for quantum key distribution and quantum information processing systems based on photonic qubits. One of the generation schemes for single photons is to use a single semiconductor quantum dot embedded in a monolithic microcavity. An optical pump pulse or electrical pump pulse generates more than one electron–hole pairs in a quantum dot. Those electron–hole pairs recombine to generate photons one by one via spontaneous emission. The last photon emitted from a quantum dot has a unique wavelength, differing from the other photons, because the multiparticle interaction inside a quantum dot modulates an emission wavelength. One can selectively extract this last photon by a narrow band optical filter, so that single photons are extracted from the system no matter how many electron–hole pairs are injected into the quantum dot initially.
The characteristics of single photons emitted by columnar microstructures based on epitaxial microcavity heterostructures with distributed Bragg reflectors, which include self-organized InAs/GaAs quantum dots and have a comparatively low Q factor in the range of 2000–3000, have been studied. It has been shown that a state with a given spin configuration—exciton with a certain polarization or trion—can be initialized in a single quantum dot under the coherent resonant linearly polarized optical pumping by a π pulse. The measurement of two-photon interference by the Hong–Ou–Mandel scheme has demonstrated that the degree of indistinguishability of successively emitted single photons is 97 and 93% at a time delay of 2 and 250 ns, respectively. Prospects of application of such sources in optical quantum computing schemes have been discussed.
Semiconductor quantum dots (QDs) coupled with optical microcavities provide an excellent platform for generating high-performance single-photon sources. However, the current microcavity structures are difficult to solve the tradeoff between single-photon purity and indistinguishability without additional filtering, due to challenges in suppressing broad phonon sideband spectrum and two-photon emission in the practical experiments. To address these issues, we have developed a novel asymmetric microcavity that supports two nondegenerate polarized modes, both resonant with a single quantum dot. One cavity mode is broadband and is used for excitation to reduce two-photon emission intensity, while the other is narrowband and is used for collection to enhance the indistinguishability of single-photon sources. This asymmetric microcavity also has the ability to overcome at least half of the photon efficiency loss under polarization filtering. Moreover, our model has employed an excitation pulse that resonates with cavity modes eliminating spectral distortion of intracavity fields, and efficiently achieving deterministic population inversion of QDs compared to an elliptical cavity. Our scheme paves the way to develop the excellent performance single-photon sources with higher brightness, near-unity purity, and indistinguishability without any additional filtering in practical experiments.
In the fields of quantum communications and quantum computing, the transmission of information using single photons guarantees the security of the communication and enables calculations that would be impossible with our "classical" computers. One of the key elements in implementing such protocols is the photon source. It must emit, on demand, one and only one photon with specific quantum properties.The aim of this project is to characterise a source of single and indistinguishable photons, designed and manufactured at CEA-Grenoble, and consisting of an indium arsenide (InAs) semiconductor quantum dot integrated into a gallium arsenide (GaAs) nanocavity. With its low quality factor, the nanocavity enables photons to be extracted efficiently over a wide range of wavelengths (30nm). In addition, thanks to its small mode volume, the spontaneous emission of quantum dots within it can be accelerated by Purcell effect (Purcell factor up to 6).In this manuscript, we first detail the implementation and the optimisation of the experimental setups used to characterise the photons emitted by our sample : microphotoluminescence, radiative lifetime measurement, Hanbury-Brown and Twiss (HBT) experiment and Hong-Ou-Mandel (HOM) experiment. Then, we present the experimental results obtained for photons emitted by two distinct quantum dots : One containing neutral exciton states, and the second, containing a charged exciton state. In order to photo-create these exciton states in the quantum dots, two pulsed optical excitation schemes were implemented: the two-photon resonant excitation of the neutral biexciton, and the phonon-assisted quasi-resonant excitation of the neutral and charged excitons. We present the measurement of the three figures of merit of a single photon source for these two quantum dots : the brightness, the single-photon purity and the indistinguishability of the emitted photons. In a second phase, we will focus on the charged exciton state and measure the profile of its emission line and its autocorrelation function under continuous resonant excitation. These results, achieved within the nano-photonics group of the University of Basel, constitute the first demonstration of continuous excitation on these nanostructures, which is a good surprise given their small size.Finally, we will look at the effects of the application of mechanical stress on the energy separation of the two neutral exciton states, known as the "fine structure splitting" (FSS). During the radiative cascade of the neutral biexciton state, the two photons emitted are entangled in polarisation, and the fidelity of the entanglement depends in particular on the FSS. Here, we will consider a second sample, where the InAs quantum dots are embedded in a GaAs photonic nanowire. By bending the nanowire, mechanical stresses are applied to the quantum dots, which will modify the energy of the exciton states. We will present an experimental study aimed at observing a possible effect on the fine structure splitting.In conclusion, we have developed and optimised various experimental setups for characterising photon sources for applications in the fields of quantum communications and quantum computing. For a first version of these photonic nanostructures, the brightness, the single-photon purity and the indistinguishability of the photons emitted by our quantum dots integrated into nanocavities are very encouraging for the future. The next objectives are to improve the nanocavities and to characterise the decoherence phenomena and the mechanical coupling between the quantum dots and these nanostructures.