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arXiv:2307.05776 · Physical Review A

Probabilistic unitary formulation of open quantum system dynamics

Le Hu, Andrew N. Jordan

Published Dec 5, 2024• 1 citation
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Abstract

We show that all nonrelativistic quantum processes, whether open or closed, are either unitary or probabilistic unitary, i.e., probabilistic combinations of unitary evolutions. This means that, for open quantum systems, their continuous dynamics can always be described by the Lindblad master equation with all jump operators being unitary. We call this formalism the probabilistic unitary formulation of open quantum system dynamics. This formalism is shown to be exact under all cases, and does not rely on any assumptions other than the continuity and differentiability of the density matrix. Moreover, it requires as few as $d\ensuremath{-}1$ jump operators, instead of ${d}^{2}\ensuremath{-}1$, to describe the open dynamics in the most general case, where $d$ is the dimension of Hilbert space of the system. Importantly, different from the conventional Lindblad master equation, this formalism is state dependent, meaning that the Hamiltonian, jump operators, and rates in general all depend on the current state of the density matrix. Hence one needs to know the explicit expression of the density matrix in order to write down the probabilistic unitary master equation explicitly. Experimentally, the formalism provides a scheme to control a quantum state to evolve along designed nonunitary quantum trajectories, and can be potentially useful in quantum computing and quantum control scenes since only unitary resources are needed for implementation.

DOI
10.1103/physreva.110.062205

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We show that all nonrelativistic quantum processes, whether open or closed, are either unitary or probabilistic unitary, i.e., probabilistic combinations of unitary evolutions. This means that, for open quantum systems, their continuous dynamics can always be described by the Lindblad master equation with all jump operators being unitary. We call this formalism the probabilistic unitary formulation of open quantum system dynamics. This formalism is shown to be exact under all cases, and does not rely on any assumptions other than the continuity and differentiability of the density matrix. Moreover, it requires as few as d\ensuremath−1d\ensuremath{-}1d\ensuremath−1 jump operators, instead of d2\ensuremath−1{d}^{2}\ensuremath{-}1d2\ensuremath−1, to describe the open dynamics in the most general case, where ddd is the dimension of Hilbert space of the system. Importantly, different from the conventional Lindblad master equation, this formalism is state dependent, meaning that the Hamiltonian, jump operators, and rates in general all depend on the current state of the density matrix. Hence one needs to know the explicit expression of the density matrix in order to write down the probabilistic unitary master equation explicitly. Experimentally, the formalism provides a scheme to control a quantum state to evolve along designed nonunitary quantum trajectories, and can be potentially useful in quantum computing and quantum control scenes since only unitary resources are needed for implementation.
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Quantum stochastic master equations of jump type are formulated in a general way and connections with quantum/classical hybrid systems and quantum filtering theory are discussed. By introducing the notion of ``typical trajectory", we show how to recursively construct the solution of the non-linear stochastic master equation (the conditional state). Moreover, by the notion of ``exclusive probability densities" we can describe all the probabilities related to the jumps, in particular, the waiting times of the jumps and their probability distributions. This general formulation and the idea of hybrid system allow to unify and generalize different fields: evolutions under non-Hermitian Hamiltonians, unitary dynamics interspersed by quantum channels at random times, quantum renewal processes, continuous time open quantum walks, Lindblad rate equation, ...
By exploiting the peculiarities of a recently introduced formalism for describing open quantum systems (the parametric representation with environmental coherent states) we derive an equation of motion for the reduced density operator of an open quantum system that has the same structure of the celebrated Gorini–Kossakowski–Sudarshan–Lindblad equation, but holds regardless of Markovianity being assumed. The operators in our result have explicit expressions in terms of the Hamiltonian describing the interactions with the environment, and can be computed once a specific model is considered. We find that, instead of a single set of Lindblad operators, in the general (non-Markovian) case there one set of Lindblad-like operators for each and every point of a symplectic manifold associated to the environment. This intricacy disappears under some assumptions (which are related to Markovianity and the classical limit of the environment), under which it is possible to recover the usual master-equation formalism. Finally, we find such Lindblad-like operators for two different models of a qubit in a bosonic environment, and show that in the classical limit of the environment their renown master equations are recovered.
Stochastic unravelings provide a useful way to represent open quantum system dynamics in terms of pure state realizations, and have been widely studied both from a fundamental and from a computational point of view. They were initially formulated for Markovian dynamics described by the Gorini-Kossakowski-Sudarshan-Lindblad master equation. However, due to recent technological and experimental development, most physical relevant dynamics present temporal correlations beyond the Markov approximation. Such correlations cause decay rates to turn temporarily negative, thus requiring the generalization of stochastic unravelings from Markovian to non-Markovian scenarios. Indeed, many unraveling techniques have been introduced in this regime, and a comprehensive review of the different jump methods is currently missing. In this work, we provide an overview of widely used quantum jump unraveling techniques for non-Markovian systems and also discuss them in terms of their numerical efficiency, divisibility requirements, Hilbert space extension, and measurement interpretation.
Abstract If an open quantum system is initially uncorrelated from its environment, then its dynamics can be written in terms of a Lindblad-form master equation. The master equation is divided into a unitary piece, represented by an effective Hamiltonian, and a dissipative piece, represented by a hermiticity-preserving superoperator; however, the division of open system dynamics into unitary and dissipative pieces is non-unique. For finite-dimensional quantum systems, we resolve this non-uniqueness by specifying a norm on the space of dissipative superoperators and defining the canonical Hamiltonian to be the one whose dissipator is minimal. We show that the canonical Hamiltonian thus defined is equivalent to the Hamiltonian initially defined by Lindblad, and that it is uniquely specified by requiring the dissipator’s jump operators to be traceless, extending a uniqueness result known previously in the special case of Markovian master equations. For a system weakly coupled to its environment, we give a recursive formula for computing the canonical effective Hamiltonian to arbitrary orders in perturbation theory, which we can think of as a perturbative scheme for renormalizing the system’s bare Hamiltonian.
Every open-system dynamics can be associated to infinitely many stochastic pictures, called unravelings, which have proved to be extremely useful in several contexts, both from the conceptual and the practical point of view. Here, focusing on quantum-jump unravelings, we demonstrate that there exists inherent freedom in how to assign the terms of the underlying master equation to the deterministic and jump parts of the stochastic description, which leads to a number of qualitatively different unravelings. As relevant examples, we show that a fixed basis of post-jump states can be selected under some definite conditions, or that the deterministic evolution can be set by a chosen time-independent non-Hermitian Hamiltonian, even in the presence of external driving. Our approach relies on the definition of rate operators, whose positivity equips each unraveling with a continuous-measurement scheme and is related to a long known but so far not widely used property to classify quantum dynamics, known as dissipativity. Starting from formal mathematical concepts, our results allow us to get fundamental insights into open quantum system dynamics and to enrich their numerical simulations.