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arXiv:2307.04342 · Physical Review X

Realization of an Extremely Anisotropic Heisenberg Magnet in Rydberg Atom Arrays

Kangheun Kim, Fan Yang, Klaus Mølmer, Jaewook Ahn

Published Feb 21, 2024• 38 citations
arXivHTMLPDF

Abstract

Strong mutual interaction which correlates elementary excitations of quantum matter plays a key role in a range of emergent phenomena, from binding and condensation to quantum thermalization and many-body localization. Here, we employ a Rydberg quantum simulator to experimentally demonstrate strongly correlated spin transport in anisotropic Heisenberg magnets, where the magnon-magnon interaction can be tuned 2 orders of magnitude larger than the magnon hopping strength. In our approach, the motion of magnons is controlled by an induced spin-exchange interaction through far off-resonant driving, which enables coherent transport of a single Rydberg excitation across a chain of ground-state atoms. As the most prominent signature of a giant anisotropy, we show that nearby Rydberg excitations form distinct types of magnon-bound states, where a tightly bound pair exhibits frozen dynamics in a fragmented Hilbert space, while a loosely bound pair propagates and establishes correlations beyond a single lattice site. Our scheme complements studies using resonant dipole-dipole interactions between Rydberg states and opens the door to exploring quantum thermodynamics with ultrastrong interactions and kinetic constraints. Published by the American Physical Society 2024

DOI
10.1103/physrevx.14.011025

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Strong mutual interaction which correlates elementary excitations of quantum matter plays a key role in a range of emergent phenomena, from binding and condensation to quantum thermalization and many-body localization. Here, we employ a Rydberg quantum simulator to experimentally demonstrate strongly correlated spin transport in anisotropic Heisenberg magnets, where the magnon-magnon interaction can be tuned 2 orders of magnitude larger than the magnon hopping strength. In our approach, the motion of magnons is controlled by an induced spin-exchange interaction through far off-resonant driving, which enables coherent transport of a single Rydberg excitation across a chain of ground-state atoms. As the most prominent signature of a giant anisotropy, we show that nearby Rydberg excitations form distinct types of magnon-bound states, where a tightly bound pair exhibits frozen dynamics in a fragmented Hilbert space, while a loosely bound pair propagates and establishes correlations beyond a single lattice site. Our scheme complements studies using resonant dipole-dipole interactions between Rydberg states and opens the door to exploring quantum thermodynamics with ultrastrong interactions and kinetic constraints. Published by the American Physical Society 2024
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Neutral atoms become strongly interacting when their electrons are excited to loosely bound Rydberg states. We investigate the strongly correlated quantum phases of matter that emerge in two-dimensional atom arrays where three Rydberg levels are used to encode an effective spin-1 degree of freedom. Dipolar exchange between such spin-1 Rydberg atoms naturally yields two distinct models: (i) a two-species hardcore boson model, and (ii) upon tuning near a Förster resonance, a dipolar spin-1 XY model. Through extensive, large-scale infinite density matrix renormalization group calculations, we provide a broad roadmap predicting the quantum phases that emerge from these models on a variety of lattice geometries: square, triangular, kagome, and ruby. We identify a wealth of correlated states, including lattice supersolids and simplex phases, all of which can be naturally realized in near-term experiments.
Spectroscopic measurements of single-particle spectral functions provide crucial insight into strongly correlated quantum matter by resolving the energy and spatial structure of elementary excitations. Here we introduce a spectroscopic protocol for single-charge injection with simultaneous spatial and energy resolution in a Rydberg tweezer array, effectively emulating scanning tunneling microscopy. By combining this protocol with single-atom-resolved imaging, we go beyond conventional spectroscopy by not only measuring the single-particle spectral function but also directly imaging the microscopic structure of the excitations underlying spectral resonances in frustrated tJtJtJ Hamiltonians. We reveal resonances associated with the formation of bound magnetic polarons -- composite quasiparticles consisting of a mobile hole bound to a magnon -- and directly extract their binding energy, spatial extent, and spin character. Finally, by exploiting the spatial tunability of our platform, we measure the local density of states across different lattice geometries. Our work establishes Rydberg tweezer arrays as a powerful platform for spectroscopic studies of strongly correlated models, offering microscopic control and direct real-space access to emergent quasiparticles in engineered quantum matter.
A system of ultracold atoms in an optical lattice provides a powerful platform for quantum simulation. In our laboratory, we use a quantum gas microscope to tune lattice parameters not only in a global scale but also at the level of individual sites. This allows us to control and detect the quantum state of interacting many-body systems as well as to engineer a broad class of Hamiltonians with high fidelity. Leveraging this versatility, we can realize several types of strongly correlated bosonic systems, which present intriguing behaviors and implement novel phases of matter. Analyzing snapshots of the atomic distribution with single-site resolution, we measure correlations and entanglement within these systems to reveal their main features, including non-equilibrium dynamics and quantum phase transitions. In this thesis, I present the works performed by our team for four different types of systems. First of all, I briefly introduce the behavior of a 1D disordered system in the critical regime between the thermal and the many-body-localized phases. In particular, we discuss what happens when a disordered and a non-disordered region are coupled via a single site. We find evidence for accelerated transport of thermal inclusion into the localized region, which shows the existence of a quantum avalanche, i.e. thermalization via accelerated transport throughout the localized system. In the second part, we realize a fractional quantum Hall state using an artificial gauge field, by implementing an adiabatic preparation protocol. We identify a topological phase transition in our system and characterize several key physical features expected for a Laughlin state by measuring density correlations and Hall conductivity. The next topic of this thesis relates to quantum magnetism. Mapping nearest hopping in a tilted optical lattice to spin flips, we realize a finite one-dimensional chain of 1/2-spins with closed boundary conditions. We perform an in-depth investigation on behaviors shown across the quantum phase transition between paramagnetic and antiferromagnetic ground states, including the evolution of the magnetization and Néel order parameter. Also, we find evidence for quantum superposition at the many-body level as a result of geometric frustration. In the last chapter, I report the experimental realization of a novel dipolar Bose-Hubbard Hamiltonian, based on a strongly tilted lattice system. When the tilt becomes the dominant energy scale, the Hamiltonian is fragmented, and the system behaves in a way that conserves dipole moment. Starting from a 1D chain of unity filled sites, we generate individual dipolar and anti-dipolar excitations at desired pinpoints. We observe quantum walks of these dipolar quasi-particles as well as their scattering dynamics, which allows us to study this new type of Hamiltonian using a bottom-up approach.