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arXiv:2307.01801 · Journal of Statistical Mechanics Theory and Experiment

Stretched exponential to power-law: crossover of relaxation in a kinetically constrained model

Sukanta Mukherjee, Puneet Pareek, Mustansir Barma, Saroj Kumar Nandi

Published Feb 9, 2024• 2 citations
arXivHTMLPDF

Abstract

Abstract The autocorrelation function in many complex systems shows a crossover in the form of its decay: from a stretched exponential relaxation (SER) at short times to a power law at long times. Studies of the mechanisms leading to such multiple relaxation patterns are rare. Additionally, the inherent complexity of these systems makes it hard to understand the underlying mechanism leading to the crossover. Here we develop a simple one-dimensional spin model, which we call a domain wall (DW) to doublon model, that shows such a crossover as the nature of the excitations governing the relaxation dynamics changes with temperature and time. The relevant excitations are DWs and bound pairs of DWs, which we term ‘doublons’. The diffusive motion of the DWs governs the relaxation at short times, whereas the diffusive motion of the doublons yields the long-time decay. This change of excitations and their relaxation leads to a crossover from SER to a power law in the decay pattern of the autocorrelation function. We augment our numerical results with simple physical arguments and analytic derivations.

DOI
10.1088/1742-5468/ad1f55

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Abstract The autocorrelation function in many complex systems shows a crossover in the form of its decay: from a stretched exponential relaxation (SER) at short times to a power law at long times. Studies of the mechanisms leading to such multiple relaxation patterns are rare. Additionally, the inherent complexity of these systems makes it hard to understand the underlying mechanism leading to the crossover. Here we develop a simple one-dimensional spin model, which we call a domain wall (DW) to doublon model, that shows such a crossover as the nature of the excitations governing the relaxation dynamics changes with temperature and time. The relevant excitations are DWs and bound pairs of DWs, which we term ‘doublons’. The diffusive motion of the DWs governs the relaxation at short times, whereas the diffusive motion of the doublons yields the long-time decay. This change of excitations and their relaxation leads to a crossover from SER to a power law in the decay pattern of the autocorrelation function. We augment our numerical results with simple physical arguments and analytic derivations.
The Kohlrausch(-Williams-Watts) law of stretched exponential relaxation has been observed for over a century and a half in diverse complex classical systems. Here we show that this law describes relaxation quite generically in closed (executing Schrödinger dynamics), interacting disordered many-body systems, using interaction range and disorder strength as primary tuning parameters. This we observe for both time-independent and periodically driven (Floquet) systems. Finite-size analysis indicates the persistence of this nonthermal relaxation regime in the thermodynamic limit thus defining a distinct dynamical regime. This regime exhibits a peak in the time scale of the long-time relaxation (following a transient), upon crossing over from weak to strong disorder. We provide a simple picture of this behavior, which naturally accounts for its generic occurrence. Formation of spin-glass — one of the possible mechanisms for stretched relaxation appears incidental to the occurrence of Kohlrausch law in our context. Finally, we provide a simple non-Hermitian Hamiltonian formulation for the dynamics of a single spin embedded in the disordered chain. This provides an analytical formula that captures not only the Kohlrausch relaxation of the disorder averaged autocorrelation but also captures the largely diverse dynamics of an arbitrary target spin in the system. Our work hence also provides a concrete quantification of the “prethermal slowness” in many-body disordered system.
Assuming that hierarchical procedure governs the evolution from one to the next step of Kadanoff's renormalization in the presence of some disorder one finds that the dynamic response is described by a log-normal distribution of the relaxation times. There are two natural limits to the model which restitute either the dynamic scaling or the activated dynamic hypotheses. This provides the basis for a simple justification to the success of the usual fits by a stretched exponential or by a Cole-Cole law which are commonly made to the non-exponential responses observed in the time or in the frequency domains in spin glasses. We provide expressions for the temperature dependences of the parameters which control these laws. We also propose a model for freezing which is based on the idea that ∂\partial∂ ln τ/∂(1/T)\tau/\partial(1/T)τ/∂(1/T) should be continuous at the freezing point. We discuss available data in spin glasses but our conclusions should be very general.
Dynamic spin correlation functions 〈Six{\mathit{S}}_{\mathit{i}}^{\mathit{x}}Six​(t)Sjx{\mathit{S}}_{\mathit{j}}^{\mathit{x}}Sjx​〉 for the one-dimensional S=1/2 XX model H=-Jtsumi{\mathit{Jtsum}}_{\mathit{i}}Jtsumi​{Six{\mathit{S}}_{\mathit{i}}^{\mathit{x}}Six​Si+1x{\mathit{S}}_{\mathit{i}+1}^{\mathit{x}}Si+1x​+Siy{\mathit{S}}_{\mathit{i}}^{\mathit{y}}Siy​Si{\mathit{S}}_{\mathit{i}}Si​ $_{+1}^{\mathit{y}}\mathrm{}}$ are calculated exactly for finite open chains with up to N=10 000 spins. Over a certain time range the results are free of finite-size effects and thus represent correlation functions of an infinite chain (bulk regime) or a semi-infinite chain (boundary regime). In the bulk regime, the long-time asymptotic decay as inferred by extrapolation is Gaussian at T=\ensuremath{\infty}, exponential at 0T\ensuremath{\infty}, and power law (\ensuremath{\sim}${\mathit{t}}^{\mathrm{\ensuremath{-}}1/2}$) at T=0, in agreement with exact results. In the boundary regime, a power-law decay is obtained at all temperatures; the characteristic exponent is universal at T=0 (\ensuremath{\sim}${\mathit{t}}^{\mathrm{\ensuremath{-}}1}$) and at 0T\ensuremath{\infty}(\ensuremath{\sim}${\mathit{t}}^{\mathrm{\ensuremath{-}}3/2}$), but is site dependent at T=\ensuremath{\infty}. In the high-temperature regime (T/J\ensuremath{\gg}1) and in the low-temperature regime (T/J\ensuremath{\ll}1), crossovers between different decay laws can be observed in 〈Six{\mathit{S}}_{\mathit{i}}^{\mathit{x}}Six​(t)Sjx{\mathit{S}}_{\mathit{j}}^{\mathit{x}}Sjx​〉. Additional crossovers are found between bulk-tpe and boundary-type decay for i=j near the boundary, and between spacelike and timelike behavior for i\ensuremath{\ne}j.
We investigate nonequilibrium relaxations of Ising models at the critical point by using a cluster update. While preceding studies imply that nonequilibrium cluster-flip dynamics at the critical point are universally described by the stretched-exponential function, we find that the dynamics changes from the stretched exponential to the power function as the dimensionality is increased: The two-, three-, four-, and infinite-dimensional Ising models are numerically studied, and the four- and infinite-dimensional Ising models exhibit the power-law relaxation. We also show that the finite-size scaling analysis using the normalized correlation length is markedly effective for the analysis of relaxational processes rather than the direct use of the Monte Carlo step.
We study numerically the nonequilibrium dynamical behavior of an Ising model with mixed two-spin and four-spin interactions after a sudden quench from the high-temperature phase to the first-order phase transition point. The autocorrelation function is shown to approach its limiting value, given by the magnetization in the ordered phase at the transition point, m c , through a stretched exponential decay. On the other hand relaxation of the magnetization starting with an uncorrelated initial state with magnetization, m i , approaches either m c , for m i > 0.5, or zero, for m i < 0.5. For small m i and for m i slightly larger than 0.5 the relaxation of the magnetization shows an asymptotic power law time dependence, thus from a nonequilibrium point of view the transition is continuous.
Aging phenomena of short-range Ising spin glass models have been investigated using Monte Carlo simulations. It is found that in the low-temperature spin-glass phase the mean domain size exhibits a crossover from a power-law growth associated with the critical fluctuation at the transition temperature to slower growth inherent in the low-temperature phase. The temperature dependence of the growth law of the domain size can be almost explained by this crossover. We also find that the spin-autocorrelation function in the quasi-equilibrium regime follows the expected scaling behavior from the droplet theory expressed in terms of the mean domain size and a characteristic length scale of droplet excitations. Spin glasses (SG) exhibit characteristic slow dynamics below the SG transition temperature. 1)-3) Recently such slow dynamics, in particular aging phenomena, has been much attractive both in experimental and theoretical studies. Several attempts have been made so far to explain the slow dynamics. There are mainly two distinct