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arXiv:2307.01799 · Physical review. E

Multiparameter universality and intrinsic diversity of critical phenomena in weakly anisotropic systems

V. Dohm

Published Oct 30, 2023• 5 citations
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Abstract

Recently a unified hypothesis of multiparameter universality for the critical behavior of bulk and confined anisotropic systems has been formulated [V. Dohm, Phys. Rev. E 97, 062128 (2018)2470-004510.1103/PhysRevE.97.062128]. We prove the validity of this hypothesis in d≥2 dimensions on the basis of the principle of two-scale-factor universality for isotropic systems at vanishing external field. We introduce an angular-dependent correlation vector and a generalized shear transformation that transforms weakly anisotropic systems to isotropic systems. As examples we consider the O(n)-symmetric φ^{4} model, Gaussian model, and n-vector model. By means of the inverse of the shear transformation we determine the general structure of the bulk order-parameter correlation function, of the singular bulk part of the critical free energy, and of critical bulk amplitude relations of anisotropic systems at and away from T_{c}. It is shown that weakly anisotropic systems exhibit a high degree of intrinsic diversity due to d(d+1)/2-1 independent parameters that cannot be determined by thermodynamic measurements. Exact results are derived for the d=2 Ising universality class and for the spherical and Gaussian universality classes in d≥2 dimensions. For the d=3 Ising universality class we identify the universal scaling function of the isotropic bulk correlation function from the nonuniversal result of the functional renormalization group. A proof is presented for the validity of multiparameter universality of the exact critical free energy and critical Casimir amplitude in a finite rectangular geometry of weakly anisotropic systems with periodic boundary conditions in the Ising universality class. This confirms the validity of recent predictions of self-similar structures of finite-size effects in the (d=2,n=1) universality class at T=T_{c} derived from conformal field theory [V. Dohm and S. Wessel, Phys. Rev. Lett. 126, 060601 (2021)PRLTAO0031-900710.1103/PhysRevLett.126.060601]. This also substantiates the previous notion of an effective shear transformation for anisotropic two-dimensional Ising models. Our theory paves the way for a quantitative theory of nonuniversal critical Casimir forces in anisotropic superconductors for which experiments have been proposed by G. A. Williams [Phys. Rev. Lett. 92, 197003 (2004)PRLTAO0031-900710.1103/PhysRevLett.92.197003].

DOI
10.1103/physreve.108.044149

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Recently a unified hypothesis of multiparameter universality for the critical behavior of bulk and confined anisotropic systems has been formulated [V. Dohm, Phys. Rev. E 97, 062128 (2018)2470-004510.1103/PhysRevE.97.062128]. We prove the validity of this hypothesis in d≥2 dimensions on the basis of the principle of two-scale-factor universality for isotropic systems at vanishing external field. We introduce an angular-dependent correlation vector and a generalized shear transformation that transforms weakly anisotropic systems to isotropic systems. As examples we consider the O(n)-symmetric φ^{4} model, Gaussian model, and n-vector model. By means of the inverse of the shear transformation we determine the general structure of the bulk order-parameter correlation function, of the singular bulk part of the critical free energy, and of critical bulk amplitude relations of anisotropic systems at and away from T_{c}. It is shown that weakly anisotropic systems exhibit a high degree of intrinsic diversity due to d(d+1)/2-1 independent parameters that cannot be determined by thermodynamic measurements. Exact results are derived for the d=2 Ising universality class and for the spherical and Gaussian universality classes in d≥2 dimensions. For the d=3 Ising universality class we identify the universal scaling function of the isotropic bulk correlation function from the nonuniversal result of the functional renormalization group. A proof is presented for the validity of multiparameter universality of the exact critical free energy and critical Casimir amplitude in a finite rectangular geometry of weakly anisotropic systems with periodic boundary conditions in the Ising universality class. This confirms the validity of recent predictions of self-similar structures of finite-size effects in the (d=2,n=1) universality class at T=T_{c} derived from conformal field theory [V. Dohm and S. Wessel, Phys. Rev. Lett. 126, 060601 (2021)PRLTAO0031-900710.1103/PhysRevLett.126.060601]. This also substantiates the previous notion of an effective shear transformation for anisotropic two-dimensional Ising models. Our theory paves the way for a quantitative theory of nonuniversal critical Casimir forces in anisotropic superconductors for which experiments have been proposed by G. A. Williams [Phys. Rev. Lett. 92, 197003 (2004)PRLTAO0031-900710.1103/PhysRevLett.92.197003].
Abstract Analytic predictions have been derived recently by Dohm and Wessel (2021 Phys. Rev. Lett. 126 060601) from anisotropic φ 4 theory and conformal field theory for the amplitude F c of the critical free energy of finite anisotropic systems in the two-dimensional Ising universality class. These predictions employ the hypothesis of multiparameter universality. We test these predictions by means of high-precision Monte Carlo (MC) simulations for F c of the Ising model on a square lattice with isotropic ferromagnetic couplings between nearest neighbors and with an anisotropic coupling between next-nearest neighbors along one diagonal. We find remarkable agreement between the MC data and the analytical prediction. This agreement supports the validity of multiparameter universality and invalidates two-scale-factor universality as F c is found to exhibit a nonuniversal dependence on the microscopic couplings of the scalar φ 4 model and the Ising model. Our results are compared with the exact result for F c in the three-dimensional φ 4 model with a planar anisotropy in the spherical limit. The critical Casimir amplitude is briefly discussed.
The exact critical Casimir amplitude is derived for anisotropic systems within the d=2 Ising universality class by combining conformal field theory with anisotropic φ^{4} theory. Explicit results are presented for the general anisotropic scalar φ^{4} model and for the fully anisotropic triangular-lattice Ising model in finite rectangular and infinite strip geometries with periodic boundary conditions. These results demonstrate the validity of multiparameter universality for confined anisotropic systems and the nonuniversality of the critical Casimir amplitude. We find an unexpected complex form of self-similarity of the anisotropy effects near the instability where weak anisotropy breaks down. This can be traced back to the property of modular invariance of isotropic conformal field theory for d=2. More generally, for d>2 we predict the existence of self-similar structures of the finite-size scaling functions of O(n)-symmetric systems with planar anisotropies and periodic boundary conditions both in the critical region for n≥1 as well as in the Goldstone-dominated low-temperature region for n≥2.
We prove the validity of multiparameter universality for the exact critical bulk correlation functions of the anisotropic square-lattice and triangular-lattice Ising models on the basis of the exact scaling structure of the correlation function of the two-dimensional anisotropic scalar φ^{4} model with four nonuniversal parameters. The correlation functions exhibit a directional nonuniversality due to principal axes whose orientation depends on microscopic details. We determine the exact anisotropy matrices governing the bulk and finite-size critical behavior of the φ^{4} and Ising models. We also prove the validity of multiparameter universality for an exact critical bulk amplitude relation.
We study spatial anisotropy effects on the bulk and finite-size critical behavior of the O(n) symmetric anisotropic phi;{4} lattice model with periodic boundary conditions in a d -dimensional hypercubic geometry above, at, and below Tc. The absence of two-scale factor universality is discussed for the bulk order-parameter correlation function, the bulk scattering intensity, and for several universal bulk amplitude relations. The anisotropy parameters are observable by scattering experiments at Tc. For the confined system, renormalization-group theory within the minimal subtraction scheme at fixed dimension d for 2<d<4 is employed. In contrast to the epsilon=4-d expansion, the fixed- d finite-size approach keeps the exponential form of the order-parameter distribution function unexpanded. For the case of cubic symmetry and for n=1 , our perturbation approach yields excellent agreement with the Monte Carlo (MC) data for the finite-size amplitude of the free energy of the three-dimensional Ising model at Tc by Mon [Phys. Rev. Lett. 54, 2671 (1985)]. The epsilon expansion result is in less good agreement. Below Tc, a minimum of the scaling function of the excess free energy is found. We predict a measurable dependence of this minimum on the anisotropy parameters. The relative anisotropy effect on the free energy is predicted to be significantly larger than that on the Binder cumulant. Our theory agrees quantitatively with the nonmonotonic dependence of the Binder cumulant on the ferromagnetic next-nearest-neighbor (NNN) coupling of the two-dimensional Ising model found by MC simulations of Selke and Shchur [J. Phys. A 38, L739 (2005)]. Our theory also predicts a nonmonotonic dependence for small values of the antiferromagnetic NNN coupling and the existence of a Lifshitz point at a larger value of this coupling. The nonuniversal anisotropy effects in the finite-size scaling regime are predicted to satisfy a kind of restricted universality. The tails of the large- L behavior at T++Tc violate both finite-size scaling and universality even for isotropic systems as they depend on the bare four-point coupling of the phi4 theory, on the cutoff procedure, and on subleading long-range interactions.
We study the bulk and finite-size critical behavior of the O(n) symmetric phi4 theory with spatially anisotropic interactions of noncubic symmetry in d<4 dimensions. In such systems of a given (d,n) universality class, two-scale factor universality is absent in bulk correlation functions, and finite-size scaling functions including the Privman-Fisher scaling form of the free energy, the Binder cumulant ratio, and the Casimir amplitude are shown to be nonuniversal. In particular it is shown that, for anisotropic confined systems, isotropy cannot be restored by an anisotropic scale transformation.
Anisotropy effects on the finite-size critical behavior of a two-dimensional Ising model on a general triangular lattice in an infinite-strip geometry with periodic, antiperiodic, and free boundary conditions (bc) in the finite direction are investigated. Exact results are obtained for the scaling functions of the finite-size contributions to the free energy density. With ξ(>) the largest and ξ(<) the smallest bulk correlation length at a given temperature near criticality, we find that the dependence of these functions on the ratio ξ(<)/ξ(>) and on the angle parametrizing the orientation of the correlation volume is of geometric nature. Since the scaling functions are independent of the particular microscopic realization of the anisotropy within the two-dimensional Ising model, our results provide a limited verification of universality. We explain our observations by considering finite-size scaling of free energy densities of general weakly anisotropic models on a d-dimensional film (i.e., in an L×∞(d-1) geometry) with bc in the finite direction that are invariant under a shear transformation relating the anisotropic and isotropic cases. This allows us to relate free energy scaling functions in the presence of an anisotropy to those of the corresponding isotropic system. We interpret our results as a simple and transparent case of anisotropic universality, where, compared to the isotropic case, scaling functions depend additionally on the shape and orientation of the correlation volume. We conjecture that this universality extends to cases where the geometry and/or the bc are not invariant under the shear transformation and argue in favor of validity of two-scale factor universality for weakly anisotropic systems.