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arXiv:2306.14804

Quantum circuits to measure scalar spin chirality

L. I. Reascos, Bruno Murta, Ernesto F. Galvão, Joaquín Fernández-Rossier

Published Jun 26, 2023• 1 citation
arXivHTMLPDF

Abstract

The scalar spin chirality is a three-body physical observable that plays an outstanding role both in classical magnetism, characterizing non-coplanar spin textures, and in quantum magnetism, as an order parameter for chiral spin liquids. In quantum information, the scalar spin chirality is a witness of genuine tripartite entanglement. Here we propose an indirect measurement scheme, based on the Hadamard test, to estimate the scalar spin chirality for general quantum states. We apply our method to study chirality in two types of quantum states: generic one-magnon states of a ferromagnet, and the ground state of a model with competing symmetric and antisymmetric exchange. We show a single-shot determination of the scalar chirality is possible for chirality eigenstates, via quantum phase estimation with a single auxiliary qutrit. Our approach provides a unified theory of chirality in classical and quantum magnetism.

DOI
10.48550/arxiv.2306.14804

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The scalar spin chirality is a three-body physical observable that plays an outstanding role both in classical magnetism, characterizing non-coplanar spin textures, and in quantum magnetism, as an order parameter for chiral spin liquids. In quantum information, the scalar spin chirality is a witness of genuine tripartite entanglement. Here we propose an indirect measurement scheme, based on the Hadamard test, to estimate the scalar spin chirality for general quantum states. We apply our method to study chirality in two types of quantum states: generic one-magnon states of a ferromagnet, and the ground state of a model with competing symmetric and antisymmetric exchange. We show a single-shot determination of the scalar chirality is possible for chirality eigenstates, via quantum phase estimation with a single auxiliary qutrit. Our approach provides a unified theory of chirality in classical and quantum magnetism.
The scalar spin chirality is a three-body physical observable that plays an outstanding role both in classical magnetism, characterizing non-co-planar spin textures, and in quantum magnetism, as an order parameter for chiral spin liquids. In quantum information, the scalar spin chirality is a witness of genuine tripartite entanglement. Here we propose an indirect measurement scheme, based on the Hadamard test, to estimate the scalar spin chirality for general quantum states. We apply our method to study chirality in two types of quantum states: generic one-magnon states of a ferromagnet, and the ground state of a model with competing symmetric and antisymmetric exchange. We show a single-shot determination of the scalar chirality is possible for chirality eigenstates, via quantum phase estimation with a single auxiliary qutrit. Our approach provides a unified theory of chirality in classical and quantum magnetism.
The scalar spin chirality (SSC), whose nonzero value ⟨Si⋅(Sj×Sk)⟩≠0\langle {\bf S}_i \cdot ({\bf S}_j \times {\bf S}_k) \rangle \neq 0⟨Si​⋅(Sj​×Sk​)⟩=0 implies the breaking of time-reversal and certain point-group symmetries in the ground state, is a key quantity characterizing chiral magnetism in both classical and quantum settings. The classical SSC is manifested, for instance, in skyrmion crystal phase, while the quantum SSC is still highly sought after in various frustrated spin-1/2 models. An interesting possibility that has not been explored so far is the case in which SSC is symmetry-wise allowed, yet remains zero classically due to the collinear or coplanar arrangement of spins, but is generated by virtue of quantum fluctuation. We demonstrate the existence of precisely such a phase in a spin-1/2 triangular-lattice model with XXZ interaction, spin-orbit-induced exchange interactions, and an external magnetic field. Using iDMRG, we thoroughly map out the phase diagram of the model and identify several phases with coexisting magnetic order and SSC. The nonzero SSC arises despite the classical magnetic order being collinear or coplanar. We provide detailed magnon analysis to ascribe its origin to quantum fluctuations around classical magnetic order. The estimate of SSC from magnon analysis agrees with iDMRG results quantitatively. We map out the magnon spectrum and its Berry curvature, culminating in the prediction of finite thermal Hall conductivity in these phases with SSC.
Bosons and fermions are defined by their exchange properties and the underlying symmetries determine the structure of the corresponding state spaces. For two particles there are two possible exchange symmetries, resulting in symmetric or antisymmetric behaviour, but when exploring multiparticle systems also quantum states with chiral symmetries appear. In this work we demonstrate that chiral symmetries lead to extremal forms of quantum entanglement. More precisely, we show that subspaces with this symmetry are highly entangled with respect to the geometric measure of entanglement, leading to observables which can be useful for entanglement characterization. Along the way, we develop a simple method to solve the problem of genuine multiparticle entanglement for unitarily invariant three-particle states and use it to identify genuine multipartite entangled states whose partial transposes with respect to all bipartitions are positive. Finally, we consider generalizations with less symmetry and discuss potential applications.
Quantum circuits have been shown to be a fertile ground for realizing long-range entangled phases of matter. While various quantum double models with non-chiral topological order have been theoretically investigated and experimentally implemented, the realization and characterization of chiral topological phases have remained less explored. Here we show that chiral topological phases in spin systems, i.e., chiral spin liquids, can be prepared in quantum circuits using the variational quantum eigensolver (VQE) framework. On top of the VQE ground state, signatures of the chiral topological order are revealed using the recently proposed tangent space excitation ansatz for quantum circuits. We show that, both topological ground state degeneracy and the chiral edge mode can be faithfully captured by this approach. We demonstrate our approach using the Kitaev honeycomb model, finding excellent agreement of low-energy excitation spectrum on quantum circuits with exact solution in all topological sectors. Further applying this approach to a non-exactly solvable chiral spin liquid model on square lattice, the results suggest this approach works well even when the topological sectors are not exactly known.
Since strong quantum fluctuations are essential for the emergence of quantum spin liquids, there have been extensive exploration and identification of spin liquid candidates in spin-12\frac{1}{2}21​ systems, while such activities are rare in higher spin systems. Here we report an example of non-Abelian chiral spin liquid emerging in a spin-32\frac{3}{2}23​ Heisenberg model on a square lattice. By tuning Heisenberg exchange interaction and scalar chirality interaction, we map out a quantum phase diagram enclosing three conventional magnetic orders and a chiral spin liquid based on density-matrix renormalization group studies. The nature of the spin liquid is identified as a long-sought bosonic version of the Read-Rezayi state that supports non-Abelian Fibonacci anyonic statistics, identified by the ground state entanglement spectrum. Significantly, we establish that the non-Abelian chiral spin liquid emerges through the enlarged local degrees of freedom and enhanced quantum fluctuations near the classical phase boundaries of competing magnetic orders. Our numerical discovery of an exotic quantum spin liquid in a spin-32\frac{3}{2}23​ system suggests a route for discovering fractionalized quantum phases in frustrated higher spin magnetic compounds.
Quantum circuits have been shown to be a fertile ground for realizing long-range entangled phases of matter. While various quantum double models with non-chiral topological order have been theoretically investigated and experimentally implemented, the realization and characterization of chiral topological phases have remained less explored. Here we show that chiral topological phases in spin systems, i.e., chiral spin liquids, can be prepared in quantum circuits using the variational quantum eigensolver (VQE) framework. On top of the VQE ground state, signatures of the chiral topological order are revealed using the recently proposed tangent space excitation ansatz for quantum circuits. We show that, both topological ground state degeneracy and the chiral edge mode can be faithfully captured by this approach.We demonstrate our approach using the Kitaev honeycomb model, finding excellent agreement of low-energy excitation spectrum on quantum circuits with exact solution in all topological sectors. Further applying this approach to a non-exactly solvable chiral spin liquid model on square lattice, the results suggest this approach works well even when the topological sectors are not exactly known.