Quantum gas microscopes are versatile and powerful tools for fundamental science as well as promising candidates for enticing applications such as in quantum simulation or quantum computation. Here we present a quantum gas microscopy setup for experiments with highly magnetic atoms of the lanthanoid elements erbium and dysprosium. Our setup features a non-magnetic, non-conducting, large-working-distance, high-numerical-aperture, in-vacuum microscope objective, mounted inside a glue-free quartz glass cell. The quartz glass cell is enclosed by a compact multi-shell ferromagnetic shield that passively suppresses external magnetic field noise by a factor of more than a thousand. Our setup will enable direct manipulation and probing of the rich quantum many-body physics of dipolar atoms in optical lattices, and bears the potential to put exciting theory proposals - including exotic magnetic phases and quantum phase transitions - to an experimental test.
Quantum gas microscopes are versatile and powerful tools for fundamental science as well as promising candidates for enticing applications such as in quantum simulation or quantum computation. Here we present a quantum gas microscopy setup for experiments with highly magnetic atoms of the lanthanoid elements erbium and dysprosium. Our setup features a non-magnetic, non-conducting, large-working-distance, high-numerical-aperture, in-vacuum microscope objective, mounted inside a glue-free quartz glass cell. The quartz glass cell is enclosed by a compact multi-shell ferromagnetic shield that passively suppresses external magnetic field noise by a factor of more than a thousand. Our setup will enable direct manipulation and probing of the rich quantum many-body physics of dipolar atoms in optical lattices, and bears the potential to put exciting theory proposals - including exotic magnetic phases and quantum phase transitions - to an experimental test.
Long-range interactions are important to complex physical systems. Specifically in quantum mechanical many-body systems, long-range interactions promote spatial structures, give rise to quantum frustration, and generate quantum entanglement. Nevertheless, quantum simulations of lattice systems have largely not been able to realize long-range interactions. Many efforts are underway to explore long-range interacting lattice systems using polar molecules, Rydberg atoms, and magnetic atoms. In this thesis, I present the realization of long-range interacting itinerant systems using magnetic erbium atoms. I start by discussing the construction of the Erbium quantum gas microscope, including the installation of an in-vacuum high-numerical-aperture objective, various optical lattices, and potential projection through the objective. Then, I present emerging quantum phases with half-filling and directly probe the spatial structures of dipolar quantum solids using site-resolved imaging. A kaleidoscope of phases emerges as we tune the dipolar interaction, demonstrating the great tunability of this experimental platform. The dipolar interactions can be tuned slowly to study first-order quantum phase transitions between different solids. Next, I discuss topological phases that emerge with unity filling. With a zoo of Fano-Feshbach resonances, erbium atoms are gifted with the flexibility of widely tunable on-site interaction, allowing continuous probing of the quantum phase transitions between topologically trivial and non-trivial phases. We explore average symmetry protected topological phases as an instance of the mixed state quantum order. Finally, I briefly discuss the observation of spin squeezing with itinerant systems and super- and sub-radiance in a sub-wavelength optical lattice.
Quantum gas microscopy of dipolar atoms is a promising opportunity to expand upon previous quantum simulations of neutral atoms in optical lattices. Erbium atoms interact via the long-range magnetic dipole-dipole interaction, which leads to a variety of new many-body effects and strongly correlated phases that are currently unexplored in microscopes with only short-range interactions. In this thesis I will detail progress toward the construction of an erbium quantum gas microscope as well as the techniques we implemented to produce a Bose-Einstein condensate of 8×104 atoms in under a second. These include the installation of a dual-stage magneto-optical trap, a stroboscopic optical dipole trap, as well as a tunable crossed optical dipole trap that allows for efficient evaporation of both bosonic and fermionic isotopes. I will also discuss the frequency stabilization systems we have implemented to produce laser linewidths of less than 1 kHz for near-resonant laser cooling on narrow transitions and a custom, high NA reflective objective to be used as part of a high resolution imaging system. Finally, I will discuss the noise properties of charge-coupled devices and the photon counting techniques that are needed for having high fidelities while using fast imaging schemes.
Quantum gas microscopy provides an exciting platform for the study of in situ atom-atom interactions. Recent advances in quantum gas microscopy have allowed the probing of the Bose-Hubbard and Fermi-Hubbard Hamiltonian with a variety of atomic species. In this thesis, we are currently extending these platforms with the introduction of an Erbium Dipolar Quantum Gas Microscope which will allow us to study dipole-dipole interactions in a lattice. Erbium has several exciting properties, which increase the control and flexibility of these systems. These include stable bosonic and fermionic isotopes, a large magnetic dipole moment (7uB), a large spin value (J=6 and F=19/2 for bosonic and fermionic isotopes), a rich Feshbach spectrum, and several useful broad and narrow atomic transitions. A broad 401 nm transition can be used for imaging, which in combination with a 266 nm lattice spacing will provide fast time scales and access to a dipole-dipole interaction of approximately 30 Hz. This thesis will document the progress toward an Erbium Quantum Gas Microscope and include a variety of systems which have been developed. It will also show the first ever 841nm, red-detuned Magneto-Optical Trap with temperatures as low as 400 nK and a phase space density up to 0.05. This, in combination with other improvements, will allow for faster cycle times and more control over the system. These developments will allow us to benefit from the long-range interaction of Erbium and probe the Extended Bose-Hubbard and Extended Fermi-Hubbard Hamiltonian to an unprecedented degree.
Quantum gas microscopy provides single-shot access to many-body configurations, yet has so far relied on pinning atoms to a discrete lattice during fluorescence readout. Here, we realize ultrafast atom-resolved fluorescence microscopy of an ultracold 162Dy gas directly in free space, with all external confinement removed during imaging. Exploiting the large mass and broad optical transition of dysprosium together with a high numerical aperture in-vacuum objective, we detect single atoms within 4μs while maintaining an effective point-spread function with a full width at half maximum of 254.8(3)nm. We achieve a single-atom conditional classification fidelity of 99.72(3)% for identified fluorescence candidates. We use the measured single-atom response to construct a statistical configuration-inference model that recovers atomic positions and multiplicities, coming from overlapping atoms, directly from single fluorescence snapshots. We further benchmark our reconstruction algorithm through end-to-end Monte Carlo simulations with known ground-truth atomic configurations, obtaining a reconstruction fidelity of 98.7%. Our approach, applicable to a wide variety of atomic species, extends quantum gas microscopy beyond predefined detection lattices, enabling atom-resolved measurements of counting statistics and higher-order spatial correlations directly on the intrinsic length scales of continuum many-body systems.
In this thesis, I present single-site detection of neutral atoms stored in a three-dimensional optical lattice using a numerical aperture objective lens (NAdesign = 0.92). The combination of high-resolution imaging with state-dependent trapping along two-direction of the lattice opens up the path towards quantum simulations via quantum walks. Suppressing the interactions of a quantum system with the environment is essential for all quantum simulation experiments. It demands a precise control of both the external magnetic (stray) fields and the polarization properties of laser beams inside the vacuum chamber. I designed a metal shielding to reduce magnetic field fluctuations and designed, assembled and characterized a novel ultra-high vacuum glass cell. The glass cell consists of special glass material and exhibits an ultra-low birefringence Δn of a few times 10^-8 to highly suppress polarization disturbances originating from stress birefringence in vacuum windows. Furthermore, anti-reflection coatings avoid reflections on all window surfaces. The cell hosts the assembled vacuum-compatible objective, that exhibits a diffraction limited resolution of up to 453 nm and allows to optically resolve the spacing of the optical lattice. Fluorescence images of single trapped atoms are used to characterize the imaging system. The filling, orientation and geometry of the optical lattice is precisely reconstructed using positions of atoms that can be determined from fluorescence images. Furthermore, I present a scheme to realize state-dependent transport and discuss its robustness against experimental imperfections in a technical implementation. This transport scheme enable the realization of discrete-time quantum walks with neutral atoms in two dimensions. These quantum walks pave the way towards the simulation of artificial magnetic fields and topologically protected edge states.
A system of ultracold atoms in an optical lattice provides a powerful platform for quantum simulation. In our laboratory, we use a quantum gas microscope to tune lattice parameters not only in a global scale but also at the level of individual sites. This allows us to control and detect the quantum state of interacting many-body systems as well as to engineer a broad class of Hamiltonians with high fidelity. Leveraging this versatility, we can realize several types of strongly correlated bosonic systems, which present intriguing behaviors and implement novel phases of matter. Analyzing snapshots of the atomic distribution with single-site resolution, we measure correlations and entanglement within these systems to reveal their main features, including non-equilibrium dynamics and quantum phase transitions. In this thesis, I present the works performed by our team for four different types of systems. First of all, I briefly introduce the behavior of a 1D disordered system in the critical regime between the thermal and the many-body-localized phases. In particular, we discuss what happens when a disordered and a non-disordered region are coupled via a single site. We find evidence for accelerated transport of thermal inclusion into the localized region, which shows the existence of a quantum avalanche, i.e. thermalization via accelerated transport throughout the localized system. In the second part, we realize a fractional quantum Hall state using an artificial gauge field, by implementing an adiabatic preparation protocol. We identify a topological phase transition in our system and characterize several key physical features expected for a Laughlin state by measuring density correlations and Hall conductivity. The next topic of this thesis relates to quantum magnetism. Mapping nearest hopping in a tilted optical lattice to spin flips, we realize a finite one-dimensional chain of 1/2-spins with closed boundary conditions. We perform an in-depth investigation on behaviors shown across the quantum phase transition between paramagnetic and antiferromagnetic ground states, including the evolution of the magnetization and Néel order parameter. Also, we find evidence for quantum superposition at the many-body level as a result of geometric frustration. In the last chapter, I report the experimental realization of a novel dipolar Bose-Hubbard Hamiltonian, based on a strongly tilted lattice system. When the tilt becomes the dominant energy scale, the Hamiltonian is fragmented, and the system behaves in a way that conserves dipole moment. Starting from a 1D chain of unity filled sites, we generate individual dipolar and anti-dipolar excitations at desired pinpoints. We observe quantum walks of these dipolar quasi-particles as well as their scattering dynamics, which allows us to study this new type of Hamiltonian using a bottom-up approach.