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arXiv:2305.13273 · Applied Physics Letters

Robust excitation of C-band quantum dots for quantum communication

Michal Vyvlečka, Lennart Jehle, Cornelius Nawrath, Francesco Giorgino, Mathieu Bozzio, Robert Sittig, Michael Jetter, Simone Luca Portalupi, Peter Michler, Philip John Walther

Published Oct 23, 2023• 13 citations
arXivHTMLPDF

Abstract

Building a quantum internet requires efficient and reliable quantum hardware, from photonic sources to quantum repeaters and detectors, ideally operating at telecommunication wavelengths. Thanks to their high brightness and single-photon purity, quantum dot (QD) sources hold the promise to achieve high communication rates for quantum-secured network applications. Furthermore, it was recently shown that excitation schemes such as longitudinal acoustic phonon-assisted (LA) pumping provide security benefits by scrambling the coherence between the emitted photon-number states. In this work, we investigate further advantages of LA-pumped quantum dots with emission in the telecom C-band as a core hardware component of the quantum internet. We experimentally demonstrate how varying the pump power and spectral detuning with respect to the excitonic transition can improve quantum-secured communication rates and provide stable emission statistics regardless of network-environment fluctuations. These findings have significant implications for general implementations of QD single-photon sources in practical quantum communication networks.

DOI
10.1063/5.0166285

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Building a quantum internet requires efficient and reliable quantum hardware, from photonic sources to quantum repeaters and detectors, ideally operating at telecommunication wavelengths. Thanks to their high brightness and single-photon purity, quantum dot (QD) sources hold the promise to achieve high communication rates for quantum-secured network applications. Furthermore, it was recently shown that excitation schemes such as longitudinal acoustic phonon-assisted (LA) pumping provide security benefits by scrambling the coherence between the emitted photon-number states. In this work, we investigate further advantages of LA-pumped quantum dots with emission in the telecom C-band as a core hardware component of the quantum internet. We experimentally demonstrate how varying the pump power and spectral detuning with respect to the excitonic transition can improve quantum-secured communication rates and provide stable emission statistics regardless of network-environment fluctuations. These findings have significant implications for general implementations of QD single-photon sources in practical quantum communication networks.
Long-range, terrestrial quantum networks require high-brightness single-photon sources emitting in the telecom C-band for maximum transmission rates. For solid-state quantum emitters, the underlying pumping process, i.e., coherent or incoherent excitation schemes, impacts several photon properties such as photon indistinguishability, single-photon purity, and photon number coherence. These properties play a major role in quantum communication applications, the latter in particular for quantum cryptography. Here, we present a versatile telecom C-band single-photon source that is operated coherently and incoherently using two complementary pumping schemes. The source is based on a quantum dot coupled to a circular Bragg grating cavity, whereas coherent (incoherent) operation is performed via the novel SUPER scheme (phonon-assisted excitation). In this way, high end-to-end-efficiencies (η end ) of 5.36% (6.09%) are achieved simultaneously with a small multiphoton contribution g (2) (0) of 0.076 ± 0.001 [ g (2) (0) of 0.069 ± 0.001] for coherent (incoherent) operation.
Semiconductor quantum dots emitting in the telecommunication O- and C-bands are promising candidates as single-photon sources for fiber-based quantum communication. In this work, we show how coherent quasi-resonant and phonon-assisted excitation help reveal the intrinsic optical properties of InAs quantum dots embedded in relaxed InGaAs matrices on top of metamorphic InGaAs layers for achieving emission in the telecom bands. By systematically comparing excitation schemes, we separate excitation-induced effects from intrinsic emitter properties. This allows us to observe linewidths as narrow as 21 μμμeV, the disappearance of slow decay channels, and single-photon purity reaching second-order autocorrelation values in the order of 10−210^{-2}10−2. Photoluminescence excitation reveals higher excited states, enabling coherent control of trion transitions and the observation of Rabi-like oscillations in both telecom bands. These results confirm the promising potential of these quantum dots for applications in quantum technologies.
For quantum light sources in everyday telecommunication networks, quantum science needs to be fully transformed into quantum technology. The first necessary step to move outside a well-controlled lab environment requires the use of quantum light sources operating in the technologically relevant telecom O- and C-band. This can be provided using epitaxial quantum dots as deterministic sources of quantum light. Particularly intriguing is that emitters operating at telecom wavelengths are rapidly catching up with their short wavelength counterparts in terms of performances. Here, we make a decisive step forward in the development of quantum communication networks: a state-of-the-art source of quantum light, a semiconductor quantum dot (QD), with record coincidence rate for entangled photon emission in the telecom C-band, is operated inside an optimized rack-based setup. This setup includes a tunable pulsed laser for the QD excitation (from quasi- to fully resonant excitation), all optics for the excitation filtering, and QD signal coupling into single-mode fibers. Overall, the setup allows for above 50%50\%50% transmission for both exciton and biexciton photons. These results show that quantum dots-based telecom light sources can now be transported and integrated into existing fiber infrastructures, an important step to demonstrate the feasibility of the upcoming quantum internet.
Long-range, terrestrial quantum networks will require high brightness single-photon sources emitting in the telecom C-band for maximum transmission rate. Many applications additionally demand triggered operation with high indistinguishability and narrow spectral linewidth. This would enable the efficient implementation of photonic gate operations and photon storage in quantum memories, as for instance required for a quantum repeater. Especially, semiconductor quantum dots (QDs) have shown these properties in the near-infrared regime. However, the simultaneous demonstration of all these properties in the telecom C-band has been elusive. Here, we present a coherently (incoherently) optically-pumped narrow-band (0.8 GHz) triggered single-photon source in the telecom C-band. The source shows simultaneously high single-photon purity with g(2)(0)=0.026g^{(2)}(0) = 0.026g(2)(0)=0.026 (g(2)(0)=0.014g^{(2)}(0) = 0.014g(2)(0)=0.014), high two-photon interference visibility of 0.508 (0.664) and high application-ready rates of 0.75 MHz (1.45 MHz) of polarized photons. The source is based on a QD coupled to a circular Bragg grating cavity combined with spectral filtering. Coherent (incoherent) operation is performed via the novel SUPER scheme (phonon-assisted excitation).
Abstract Quantum cryptography harnesses quantum light, in particular single photons, to provide security guarantees that cannot be reached by classical means. For each cryptographic task, the security feature of interest is directly related to the photons’ non-classical properties. Quantum dot-based single-photon sources are remarkable candidates, as they can in principle emit deterministically, with high brightness and low multiphoton contribution. Here, we show that these sources provide additional security benefits, thanks to the tunability of coherence in the emitted photon-number states. We identify the optimal optical pumping scheme for the main quantum-cryptographic primitives, and benchmark their performance with respect to Poisson-distributed sources such as attenuated laser states and down-conversion sources. In particular, we elaborate on the advantage of using phonon-assisted and two-photon excitation rather than resonant excitation for quantum key distribution and other primitives. The presented results will guide future developments in solid-state and quantum information science for photon sources that are tailored to quantum communication tasks.
On-demand sources of entangled photons for the transmission of quantum information in the telecom C-band are required to realize fiber-based quantum networks. So far, non-deterministic sources of quantum states of light were used for long distance entanglement distribution in this lowest loss wavelength range. However, they are fundamentally limited in either efficiency or security due to their Poissonian emission statistics. Here, we show on-demand generation of entangled photon pairs in the telecom C-band by an InAs/GaAs semiconductor quantum dot. Using a robust phonon-assisted excitation scheme we measure a concurrence of 91.4 %91.4\,\%91.4% and a fidelity of 95.2 %95.2\,\%95.2% to Φ+Φ^+Φ+. On-demand generation of polarization entangled photons will enable secure quantum communication in fiber-based networks. Furthermore, applying this excitation scheme to several remote quantum dots tuned into resonance will enable first on-demand entanglement distribution over large distances for scalable real-life quantum applications.