Mediated interactions between Fermi polarons and the role of impurity quantum statistics
Cosetta Baroni, Bo Huang, Isabella Fritsche, Erich Dobler, Gregor Anich, Emil Kirilov, Rudolf Grimm, M. A. Bastarrachea-Magnani, Pietro Massignan, Georg M. Bruun
Abstract The notion of quasi-particles is essential for understanding the behaviour of complex many-body systems. A prototypical example of a quasi-particle is a polaron, formed by an impurity strongly interacting with a surrounding medium. Fermi polarons, created in a Fermi sea, provide a paradigmatic realization of this concept. Importantly, such quasi-particles interact with each other via the modulation of the medium. However, although quantum simulation experiments with ultracold atoms have substantially improved our understanding of individual polarons, the detection of their interactions has so far remained elusive. Here we report the observation of mediated interactions between Fermi polarons consisting of K impurities embedded in a Fermi sea of Li atoms. Our results confirm two predictions of Landau’s Fermi-liquid theory: the shift in polaron energy due to mediated interactions, which is linear in the concentration of impurities; and its sign inversion with impurity quantum statistics. For weak-to-moderate interactions between the impurities and the medium, our results agree with the static predictions of Fermi-liquid theory. For stronger impurity–medium interactions, we show that the observed behaviour at negative energies can be explained by a more refined many-body treatment including retardation and dressed molecule formation.
Abstract The notion of quasi-particles is essential for understanding the behaviour of complex many-body systems. A prototypical example of a quasi-particle is a polaron, formed by an impurity strongly interacting with a surrounding medium. Fermi polarons, created in a Fermi sea, provide a paradigmatic realization of this concept. Importantly, such quasi-particles interact with each other via the modulation of the medium. However, although quantum simulation experiments with ultracold atoms have substantially improved our understanding of individual polarons, the detection of their interactions has so far remained elusive. Here we report the observation of mediated interactions between Fermi polarons consisting of K impurities embedded in a Fermi sea of Li atoms. Our results confirm two predictions of Landau’s Fermi-liquid theory: the shift in polaron energy due to mediated interactions, which is linear in the concentration of impurities; and its sign inversion with impurity quantum statistics. For weak-to-moderate interactions between the impurities and the medium, our results agree with the static predictions of Fermi-liquid theory. For stronger impurity–medium interactions, we show that the observed behaviour at negative energies can be explained by a more refined many-body treatment including retardation and dressed molecule formation.
The notion of a polaron, originally introduced in the context of electrons in ionic lattices, helps us to understand how a quantum impurity behaves when being immersed in and interacting with a many-body background. We discuss the impact of the impurities on the medium particles by considering feedback effects from polarons that can be realized in ultracold quantum gas experiments. In particular, we exemplify the modifications of the medium in the presence of either Fermi or Bose polarons. Regarding Fermi polarons we present a corresponding many-body diagrammatic approach operating at finite temperatures and discuss how mediated two- and three-body interactions are implemented within this framework. Utilizing this approach, we analyze the behavior of the spectral function of Fermi polarons at finite temperature by varying impurity-medium interactions as well as spatial dimensions from three to one. Interestingly, we reveal that the spectral function of the medium atoms could be a useful quantity for analyzing the transition/crossover from attractive polarons to molecules in three-dimensions. As for the Bose polaron, we showcase the depletion of the background Bose-Einstein condensate in the vicinity of the impurity atom. Such spatial modulations would be important for future investigations regarding the quantification of interpolaron correlations in Bose polaron problems.
The notion of a polaron, originally introduced in the context of electrons in ionic lattices, helps us to understand how a quantum impurity behaves when being immersed in and interacting with a many-body background. We discuss the impact of the impurities on the medium particles by considering feedback effects from polarons that can be realized in ultracold quantum gas experiments and in particular we exemplify the modifications of the medium either in the presence of Fermi or Bose polarons. Regarding Fermi polarons we present a corresponding many-body diagrammatic approach operating at finite temperatures and discuss how mediated two- and three-body interactions are implemented within this framework. Utilizing this approach, we analyze the behavior of the spectral function of Fermi polarons at finite temperature by varying impurity-medium interactions as well as spatial dimensions from three to one. Interestingly, we reveal that the spectral function of the medium atoms could be a useful quantity for analyzing the transition/crossover from attractive polarons to molecules in three-dimensions. As for the Bose polaron, we showcase the depletion of the background Bose-Einstein condensate in the vicinity of the impurity atom. Such spatial modulations would be important for future investigations regarding the quantification of interpolaron correlations in Bose polaron problems.
Mediated interactions between quasiparticles lie at the heart of Landau Fermi-liquid theory, yet their behavior in the strongly correlated regime is not fully understood. Motivated by recent experiments [Nat. Phys. 20, 68--73 (2024)], we investigate mediated interactions between quasiparticles emerging from a Fermi sea---Fermi polarons---using zero-temperature quantum Monte Carlo methods. Our main result is that the Landau interaction between polarons remains repulsive in the strongly interacting regime for any coupling strength in the polaronic branch, in contrast to the downward trend observed experimentally near resonance. Deep in the short-range universal regime, our results are insensitive to the microscopic details of the interaction potential, providing robust evidence for the sign of the ground-state induced interaction. In addition, we determine the real-space interaction between static impurities, recovering a Ruderman-Kittel-Kasuya-Yosida (RKKY)-like behavior at weak coupling and the nonperturbative Born-Oppenheimer result at strong coupling. More broadly, our results establish a microscopic benchmark for how Landau quasiparticle interactions survive beyond the perturbative regime of strongly correlated quantum matter.
Polaron quasiparticles are formed when a mobile impurity is coupled to the elementary excitations of a many-particle background. In the field of ultracold atoms, the study of the associated impurity problem has attracted a growing interest over the last fifteen years. Polaron quasiparticle properties are essential to our understanding of a variety of paradigmatic quantum many-body systems realized in ultracold atomic gases and in the solid state, from imbalanced Bose–Fermi and Fermi–Fermi mixtures to fermionic Hubbard models. In this topical review, we focus on the so-called repulsive polaron branch, which emerges as an excited many-body state in systems with underlying attractive interactions such as ultracold atomic mixtures, and is characterized by an effective repulsion between the impurity and the surrounding medium. We give a brief account of the current theoretical and experimental understanding of repulsive polaron properties, for impurities embedded in both fermionic and bosonic media, and we highlight open issues deserving future investigations.
We consider the behavior of a small density of mobile impurities (polarons) immersed in a quantum gas, a generic scenario that can be realized in cold atomic gases, liquid helium mixtures, and doped semiconductors. We present a unified theoretical framework for understanding polaron quasiparticles beyond the single-impurity limit, and we identify two key factors that control the polaron-polaron interactions: (i) the statistics of the impurities, including whether or not they are degenerate, and (ii) the constraints on the medium response, i.e., whether the medium density or chemical potential is held fixed. By constructing wave functions for two bosonic, fermionic, or distinguishable impurities immersed in a Bose or Fermi gas, we derive rigorous results for the polaron interactions in the limit of weak impurity-medium coupling. We furthermore obtain an exact relationship between the polaron interactions at fixed medium density and at fixed chemical potential, a result which is valid for arbitrary interaction strength. Our work provides an important guide for understanding experiments, and it acts as a starting point for future strong-coupling theories of polaron interactions that capture all of the effects identified in this work.
The Fermi polaron, formed by an impurity interacting with a surrounding Fermi sea, exemplifies the canonical quasiparticle concept as a cornerstone in our description of quantum many-body systems across a wide range of energy scales. Experiments on atomic quantum gases have provided profound insights into the universal nature of the Fermi polaron. While most previous studies have focused on the case of zero impurity momentum, finite-momentum properties have remained largely uncharted. Here, we investigate the moving Fermi polaron by combining a novel Raman acceleration scheme with high-precision radio-frequency spectroscopy, exploring the quasiparticle dispersion relation over a wide range of momenta. We compare our measurements of energy shifts and spectral linewidths with a microscopic theory and reach quantitative agreement for all momenta. For low momenta, we find the energy of the moving polaron to be fully consistent with the Fermi liquid picture of a dressed particle with a constant effective mass. At high momenta, the polaron approaches the behavior of a weakly interacting bare particle, featuring small energy shifts and weak broadening. For intermediate momenta, broadening is generally larger and, most strikingly, the behavior differs for attractive and repulsive polarons. While the repulsive polaron exhibits a smooth connection between both regimes along with a monotonic change of the energy shift, the attractive case shows a peculiar non-monotonic behavior. With increasing momentum, the attractive polaron enters a regime where its energy deviates from the constant effective mass expression and broadening suddenly increases. By comparing this observation with theory, we show that this abrupt behavior coincides with the attractive polaron entering a molecule-hole continuum, where it is no longer the ground state. We interpret this as a motion-induced polaron-molecule transition.