Photons, by nature, typically do not exhibit interactions with each other. Creating photon-photon interactions holds immense importance in both fundamental physics and quantum technologies. Currently, such interactions have only been achieved indirectly as mediated by atomic-like quantum emitters with resonant photon-atom interactions. However, the use of these indirect interactions presents substantial fundamental challenges that impede scaling and practical applications. Here we demonstrate creation of non-classical photon correlations, including photon anti-bunching, via a passive InGaP photonic integrated circuit. Our approach employs the quantum interference between uncorrelated light and the two-photon bound state, the latter of which arises from the $χ^{(2)}$-mediated photon interaction. Our work opens a new route in controlling quantum light by harnessing highly-engineerable bulk optical nonlinearities, which has significant implications for nonlinear optical quantum information processing and quantum networking.
Photons, by nature, typically do not exhibit interactions with each other. Creating photon-photon interactions holds immense importance in both fundamental physics and quantum technologies. Currently, such interactions have only been achieved indirectly as mediated by atomic-like quantum emitters with resonant photon-atom interactions. However, the use of these indirect interactions presents substantial fundamental challenges that impede scaling and practical applications. Here we demonstrate creation of non-classical photon correlations, including photon anti-bunching, via a passive InGaP photonic integrated circuit. Our approach employs the quantum interference between uncorrelated light and the two-photon bound state, the latter of which arises from the χ(2)-mediated photon interaction. Our work opens a new route in controlling quantum light by harnessing highly-engineerable bulk optical nonlinearities, which has significant implications for nonlinear optical quantum information processing and quantum networking.
Typical schemes for generating correlated states of light require a highly nonlinear medium that is strongly coupled to an optical mode. However, unavoidable dissipative processes, which cause photon loss and blur nonlinear quantum effects, often impede such methods. In this talk, I will report on our experimental implementation of the opposite approach. Using a strongly dissipative, weakly coupled medium, we generate and study strongly correlated states of light. Specifically, we study the transmission of resonant light through an ensemble of non-interacting atoms that weakly couple to a guided optical mode. Dissipation removes uncorrelated photons while preferentially transmitting highly correlated photons, created through collectively enhanced nonlinear interactions. As a result, the transmitted light constitutes a strongly correlated many-body state of light, revealed in the second-order correlation function. The latter exhibits strong antibunching or bunching, depending on the optical depth of the atomic ensemble. The demonstrated mechanism opens a new avenue for generating nonclassical states of light and for exploring correlations of photons in non-equilibrium systems using a mix of nonlinear and dissipative processes.
Abstract Many technologies emerging from quantum information science heavily rely upon the generation and manipulation of entangled quantum states. Here, we propose and demonstrate a new class of quantum interference phenomena that arise when states are created in and coherently converted between the propagating modes of an optical microcavity. The modal coupling introduces several new creation pathways to a nonlinear optical process within the device, which quantum mechanically interfere to drive the system between states in the time domain. The coherent conversion entangles the generated biphotons between propagation pathways, leading to cyclically evolving path-entanglement and the manifestation of coherent oscillations in second-order temporal correlations. Furthermore, the rich device physics is harnessed to tune properties of the quantum states. In particular, we show that the strength of interference between pathways can be coherently controlled, allowing for manipulation of the degree of entanglement, which can even be entirely quenched. The states can likewise be made to flip-flop between exhibiting initially correlated or uncorrelated behavior. The phenomena presented here open a route to creating higher dimensional entanglement and exotic multi-photon states.
Controlling light photon-by-photon is central to quantum optics. At a fundamental level, photon interactions are mediated by their coupling to atoms, and ultimate control requires deterministic light-matter interfacing of single photons to single atoms. Extending this paradigm to radiatively couple multiple individual atoms in a deterministic and scalable manner opens the arena of many-body quantum optics. Here, we realize such a setting by coherently coupling solid-state artificial atoms to a nanophotonic waveguide and demonstrate higher-order photon correlations that are controlled by the number of quantum emitters. We study the scaling of nonlinear photonic transport induced by emitter-photon scattering and demonstrate that adding a quantum emitter generates higher-order photon correlations. Specifically, we experimentally observe genuine three-photon correlations from a pair of collectively coupled emitters, while contributions from lower photon numbers are suppressed. In addition, we scale to three resonant quantum emitters coupled to the waveguide. These advancements demonstrate the onset of many-body quantum optics in waveguide quantum electrodynamics, enabling new photonic quantum simulators, the creation of many-body entangled states, and the exploration of novel quantum phase transitions.
Abstract Single photons constitute a main platform in quantum science and technology: they carry quantum information over extended distances in the future quantum internet1 and can be manipulated in advanced photonic circuits enabling scalable photonic quantum computing. The main challenge in quantum photonics is how to generate advanced entangled resource states and efficient light-matter interfaces offer a path way. Here we utilize the efficient and coherent coupling of a single quantum emitter to a nanophotonic waveguide for realizing quantum nonlinear interaction between single-photon wavepackets. This inherently multimode quantum system constitutes a new research frontier in quantum optics. We demonstrate control of a photon with another photon and experimentally unravel the dynamical response of two-photon interactions mediated by a quantum emitter, and show that the induced quantum correlations are controlled by the pulse duration. The work will open new avenues for tailoring complex photonic quantum resource states.
Strong coupling between light and matter has been demonstrated both in classical cavity quantum electrodynamics (QED) systems and in more recent circuit-QED experiments. This enables the generation of strong nonlinear photon-photon interactions at the single-photon level, which is of great interest for the observation of quantum nonlinear optical phenomena, the control of light quanta in quantum information protocols such as quantum networking, as well as the study of strongly correlated quantum many-body systems using light. Recently, strong coupling has also been realized in a variety of one-dimensional (1D) waveguide- QED experimental systems, which in turn makes them promising candidates for quantum information processing. Compared to cavity-QED systems, there are two new features in waveguide-QED: the existence of a continuum of states and the restricted 1D phase space, which together bring in new physical effects, such as the bound-state effects. This thesis consists of two parts: 1) understanding the fundamental interaction between local quantum objects, such as two-level systems and four-level systems, and photons confined in the waveguide; 2) exploring its implications in quantum information processing, in particular photonic quantum computation and quantum key distribution. First, we demonstrate that by coupling a two-level system (TLS) or three/fourlevel system to a 1D continuum, strongly-correlated photons can be generated inside the waveguide. Photon-photon bound states, which decay exponentially as a function of the relative coordinates of photons, appear in multiphoton scattering processes. As a result, photon bunching and antibunching can be observed in the photon-photon correlation function, and nonclassical light source can be generated on demand. In the case of an N-type four-level system, we show that the effective photon-photon interaction mediated by the four-level system, gives rise to a variety of nonlinear optical phenomena, including photon blockade, photon-induced tunneling, and creation of single-photon states and photon pairs with a high degree of spectral entanglement, all in the absence of a cavity. However, to enable greater quantum networking potential using waveguide- QED, it is important to study systems having more than just one TLS/qubit. We develop a numerical Green function method to study cooperative effects in a system of two qubits coupled to a 1D waveguide. Quantum beats emerge in photon-photon correlations, and persist to much longer time scales because of non-Markovian processes. In addition, this system can be used to generate a high-degree of long-distance entanglement when one of the two qubits is driven by an on-resonance laser, further paving the way toward waveguide-QED-based quantum networks. Furthermore, based on our study of light-matter interactions in waveguide- QED, we investigate its implications in quantum information processing. First, we study quantum key distribution using the sub-Possonian single photon source obtained by scattering a coherent state off a two-level system. The rate for key generation is found to be twice as large as for other sources. Second, we propose a new scheme for scalable quantum computation using flying qubits--propagating photons in a one-dimensional waveguide--interacting with matter qubits. Photonphoton interactions are mediated by the coupling to a three- or four-level system, based on which photon-photon -phase gates (Controlled-NOT) can be implemented for universal quantum computation. We show that high gate fidelity is possible given recent dramatic experimental progress in superconducting circuits and photonic-crystal waveguides. The proposed system can be an important building block for future on-chip quantum networks.
Quantum information science aims to harness uniquely quantum mechanical properties to enhance measurement and information technologies, and to explore fundamental aspects of quantum physics. Of the various approaches to quantum computing [1], photons are particularly appealing for their low-noise properties and ease of manipulation at the single qubit level [2,3]. Encoding quantum information in photons is also an appealing approach to quantum communication, metrology (eg. [4]), measurement (eg. [5]) and other quantum technologies [6]. However, the implementation of optical quantum circuits with bulk optics has reached practical limits. We have developed an integrated waveguide approach to photonic quantum circuits for high performance, miniaturization and scalability [7]. Here we report high-fidelity silica-on-silicon integrated optical realizations of key quantum photonic circuits, including two-photon quantum interference and a controlled-NOT logic gate [8]. We have demonstrated controlled manipulation of up to four photons on-chip, including highfidelity single qubit operations, using a lithographically patterned resistive phase shifter [9]. We have used this architecture to implement a small-scale compiled version of Shor's quantum factoring algorithm [10], demonstrated heralded generation of tunable four photon entangled states from a six photon input [11], a reconfigurable two-qubit circuit [12], and combined waveguide photonic circuits with superconducting single photon detectors [13]. We describe complex quantum interference behavior in multi-mode interference devices with up to eight inputs and outputs [14], and quantum walks of correlated particles in arrays of coupled waveguides [15]. Finally, we give an overview of our recent work on fundamental aspects of quantum measurement [16,17] and diamond [18,19] and nonlinear [20,21] photon sources.