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arXiv:2304.02436 · Physical Review A

Metrics and properties of optimal gauges in multimode cavity QED

Geva Arwas, Vladimir Manucharyan, Cristiano Ciuti

Published Aug 16, 2023• 9 citations
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Abstract

Multimode cavity quantum electrodynamics describes, for example, the coupling between an atom and a multimode electromagnetic resonator. The gauge choice is important for practical calculations in truncated Hilbert spaces, because the exact gauge invariance is recovered only in the whole space. An optimal gauge can be defined as the one predicting the most accurate observables for the same number of atomic levels and modes. Different metrics quantifying the gauge performance can be introduced depending on the observable of interest. In this paper we demonstrate that the optimal choice is generally mode dependent, i.e., a different gauge is needed for each cavity mode. While the choice of gauge becomes more important for increasing light-matter interaction, we also show that the optimal gauge does not correspond to the situation where the entanglement between light and matter is the smallest.

DOI
10.1103/physreva.108.023714

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Multimode cavity quantum electrodynamics describes, for example, the coupling between an atom and a multimode electromagnetic resonator. The gauge choice is important for practical calculations in truncated Hilbert spaces, because the exact gauge invariance is recovered only in the whole space. An optimal gauge can be defined as the one predicting the most accurate observables for the same number of atomic levels and modes. Different metrics quantifying the gauge performance can be introduced depending on the observable of interest. In this paper we demonstrate that the optimal choice is generally mode dependent, i.e., a different gauge is needed for each cavity mode. While the choice of gauge becomes more important for increasing light-matter interaction, we also show that the optimal gauge does not correspond to the situation where the entanglement between light and matter is the smallest.
Abstract We have investigated the gauge dependence of physical observables in a quantum Rabi model under different potential fields arising from the Hilbert space truncation of the atomic degrees of freedom. In both the square-well and harmonic potentials, the optimal gauge for the ground-state energy depends on the cavity frequency, which is optimal in the low-frequency limit, whereas the Coulomb gauge is optimal in the high-frequency limit. For a dynamic quantity, such as an out-of-time-order correlator, we have demonstrated the necessity of introducing an optimal dynamic gauge. This study provides deeper insight into the intricate relationship between gauge choice and the dynamics of quantum electrodynamics systems, resulting in more accurate theoretical frameworks.
Systems of interacting charges and fields are ubiquitous in physics. Recently, it has been shown that Hamiltonians derived using different gauges can yield different physical results when matter degrees of freedom are truncated to a few low-lying energy eigenstates. This effect is particularly prominent in the ultra-strong coupling regime. Such ambiguities arise because transformations reshuffle the partition between light and matter degrees of freedom and so level truncation is a gauge dependent approximation. To avoid this gauge ambiguity, we redefine the electromagnetic fields in terms of potentials for which the resulting canonical momenta and Hamiltonian are explicitly unchanged by the gauge choice of this theory. Instead the light/matter partition is assigned by the intuitive choice of separating an electric field between displacement and polarisation contributions. This approach is an attractive choice in typical cavity quantum electrodynamics situations.
The loss of gauge invariance in models of light-matter interaction which arises from material and photonic space truncation can pose significant challenges to conventional quantum optical models when matter and light strongly hybridize. In structured photonic environments, necessary in practice to achieve strong light-matter coupling, a rigorous model of field quantization within the medium is also needed. Here we use the framework of macroscopic QED by quantizing the fields in an arbitrary material system, with a spatially dependent dispersive and absorptive dielectric, starting from a fundamental light-matter action. We truncate the material and mode degrees of freedom while respecting the gauge principle by imposing a partial gauge-fixing constraint during canonical quantization, which admits a large number of gauges including the Coulomb and multipolar gauges commonly used in quantum optics. We also consider gauge conditions with explicit time dependence, enabling us to unambiguously introduce additional phenomenologically time-dependent light-matter interactions in any gauge. Our results allow one to derive rigorous nonrelativistic models of ultrastrong light-matter interactions in structured photonic environments with no gauge ambiguity. Results for two-level systems and the dipole approximation are discussed, as well as how to go beyond the dipole approximation for effective single-particle models. By comparing with the limiting case of an inhomogeneous dielectric, where dispersion and absorption can be neglected and the fields can be expanded in terms of the generalized transverse eigenfunctions of the dielectric, we show how lossy systems can introduce an additional gauge ambiguity, which we resolve and predict to have fundamental implications for open quantum system models. Finally, we show how observables in mode-truncated systems can be calculated without ambiguity by using a simple gauge-invariant model of photodetection.
This article reviews the meaning of gauge freedom in quantum electrodynamics and emphasizes its consistency with examples and analyses. It thus demonstrates that ambiguities and recent controversies are resolved by proper identification of physically relevant observables of field and matter subsystems. Since these observables differ for different gauges, light and matter subsystems can only be defined relative to the choice of gauge, with implications for the identification of effective few-dimensional models, entanglement, phase transitions, and cavity quantum electrodynamics effects beyond weak-coupling regimes.
In the multimode regime of cavity quantum electrodynamics (cQED), light-matter coupling can be strong enough such as to allows a quantum emitter to couple with multiple resonant field modes. This regime leaves distinctive signatures in the behavior of both the field and the emitter, which are already accessible by modern experimental techniques. To model such effects in lossy cavities, effective discrete-mode approaches have been widely employed, despite their accuracy beyond two modes remaining rarely benchmarked. In this work, we demonstrate the necessity of employing multiple modes to describe the multimode signatures by analyzing the dynamics of an atom in a one-dimensional lossy resonator. The atom's dynamics is simulated using the formalism developed in Weitzel et al. (2026) (arXiv:2512.18478), where a resonance quantization prescription is provided. We investigate its dependency with respect to two different parameters: the light-matter coupling strength and the atom's position. In the former case, we find that the minimal number of modes necessary to capture the essential features of the atom's dynamics increases with the coupling strength. In the latter, we further observe that the multimode regime leads to a strong position-dependency of the atom's dynamics. In all cases, we discuss the physical interpretation of our results and further discuss about how the employed formalism can be used to recover physically relevant quantities.
The interaction between quantized electromagnetic fields in cavities and natural or artificial atoms has played a crucial role in developing our understanding of light-matter interactions and quantum technologies.Recently, new regimes beyond the weak and strong light-matter coupling of cavity-QED have been explored in several settings, wherein the light-matter coupling rate becomes comparable to (ultrastrong coupling) or even exceeds (deep-strong coupling) the photon frequency.These ultrastrong coupling regimes can give rise to new physical effects and applications, and they challenge our understanding of cavity QED; fundamental issues like the proper definition of subsystems, their quantum measurements, the structure of light-matter ground states, and the analysis of time-dependent interactions are subject to gauge ambiguities that lead to even qualitatively distinct predictions.The resolution of these ambiguities is important for understanding and designing next-generation quantum devices that can operate in extreme coupling regimes.Here we discuss and provide solutions to these ambiguities by adopting an approach based on operational procedures involving measurements on the individual light and matter components of the interacting system.