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arXiv:2303.15185 · Quantum

A probabilistic view of wave-particle duality for single photons

Andrea Aiello

Published Oct 11, 2023• 3 citations
arXivHTMLPDF

Abstract

One of the most puzzling consequences of interpreting quantum mechanics in terms of concepts borrowed from classical physics, is the so-called wave-particle duality. Usually, wave-particle duality is illustrated in terms of complementarity between path distinguishability and fringe visibility in interference experiments. In this work, we instead propose a new type of complementarity, that between the continuous nature of waves and the discrete character of particles. Using the probabilistic methods of quantum field theory, we show that the simultaneous measurement of the wave amplitude and the number of photons in the same beam of light is, under certain circumstances, prohibited by the laws of quantum mechanics. Our results suggest that the concept of “interferometric duality'' could be eventually replaced by the more general one of “continuous-discrete duality''.

DOI
10.22331/q-2023-10-11-1135

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One of the most puzzling consequences of interpreting quantum mechanics in terms of concepts borrowed from classical physics, is the so-called wave-particle duality. Usually, wave-particle duality is illustrated in terms of complementarity between path distinguishability and fringe visibility in interference experiments. In this work, we instead propose a new type of complementarity, that between the continuous nature of waves and the discrete character of particles. Using the probabilistic methods of quantum field theory, we show that the simultaneous measurement of the wave amplitude and the number of photons in the same beam of light is, under certain circumstances, prohibited by the laws of quantum mechanics. Our results suggest that the concept of “interferometric duality'' could be eventually replaced by the more general one of “continuous-discrete duality''.
A single photon exhibits wave-particle duality in the Young's double-slit interferometer. The duality characterized by an interference visibility and a which-path information has trade-off relation known as complementarity. These quantities are related to the first-order coherence, and the interference is based on the phase correlation between lights coming from two arms. However according to quantum optics theory, such a simple wave-particle picture is not enough to understand the nature because the theory showed an importance of higher-order coherence in the sense of both interference and statistical distribution of photons. Second-order intensity correlation is especially crucial to reveal distinctive quantum features of photons with no classical analogue. Here, in an intensity interferometric scenario as represented by the Hong-Ou-Mandel interferometer, we discuss a wave-particle duality of light based on a which-path information and a quantity characterizing a magnitude of the intensity interferometric effect. We show, for classical light, the two quantities obey the complementary principle similar to the case of the double-slit experiment, but do not for nonclassical light. The nonclassical light such as photons at two arms is allowed to show larger which-path information and intensity interference simultaneously beyond the complementary relation. Moreover, the violation reveals a new nonclassical nature of light although both of the above two quantities seem to be understandable classically, which is never found from a consideration of only one side of wave-particle duality.
Classical wisdom of wave–particle duality regulates that a quantum object shows either the particle or wave nature but never both. Consequently, it would be impossible to observe simultaneously the complete wave and particle nature of the quantum object. Mathematically the principle requests that the interference visibility V and which-path distinguishability D satisfy an orthodox limit of V 2 + D 2 ≤ 1 . The present work reports a new wave–particle duality test experiment using single photons in a modified Mach–Zehnder interferometer to demonstrate the possibility of breaking the limit. The key element of the interferometer is a weakly scattering total internal reflection prism surface, which exhibits a pronounced single-photon interference with a visibility of up to 0.97 and simultaneously provides a path distinguishability of 0.83. Apparently, the result of V 2 + D 2 ≈ 1.63 exceeds the orthodox limit set by the classical principle of wave–particle duality for single photons. We expect that more delicate experiments in the future should be able to demonstrate the ultimate limit of V 2 + D 2 ≈ 2 and shed new light on the foundations of contemporary quantum mechanics.
Updating the wave-particle duality Maria C. Bosca e-mail: bosca@ugr.es Departamento de Fisica Atomica, Molecular y Nuclear Universidad de Granada E-18071. Granada Spain The wave-particle-duality, the fundamental component of the new quantum formalism in Bohr’s opinion, must be reformulated by incorporating the results of some experiments accomplished in the last decades of twentieth century. The Bohr´s complementarity principle stated the mutual exclusiveness and joint full completeness of the two (classical) descriptions of quantum systems; after Einstein-Podolsky-Rosen’paper, the wave-particle duality, or wave-particle complementarity, could be expressed by stating that it is impossible to build up an experimental arrangement in which we observe at the same time both corpuscular and wave aspects. In a two-slit experiment, they would correspond, respectively, to the which-way knowledge and the observation of interference pattern. Bohr showed this mutual exclusivity in numerous examples , and linked it to the unavoidable disturbance inherent in any measurement event. In quantum mechanical formalism, the complementarity principle has a clear mathematical expression: two observables are complementary if precise knowledge of one of them implies that all possible outcomes of the other are equally probable; their extension to classical concepts (as wave and particle) is not concerned. In 1991 Scully et al published a variant of the two-slit experiment that incorporates two micromasers cavities and a laser beam to provide which-path information without net momentum transferred during the interaction ; the impossibility of know which slit an atom went through and still observe the interference fringes is preserved by the establishing of quantum correlations between the measuring apparatus and the system being observed. They claimed that complementarity, of which wave-particle duality would be to them a manifestation, is more fundamental than the uncertainty principle . In 1996 B-G. Englert, following an approach originally due to Wooters and Zurek , derived , without making use of Heisenberg’s uncertainty relation, an inequality that quantifies the mutual compatibility relation between fringe visibility and which-way information. The inequality, that they denominated as “interferometric duality”, has the expression D^2 + V^2 ≤ 1, where D stands for the distinguishability of the ways and V for the fringe visibility; both of them are mathematical expressions that can be measured to check experimentally the inequality . Today, it is clear that intermediate particle-wave behaviours exist and, in addition to that, there are single experiments in which both classical wave-like and particle-like behaviours are showed total and simultaneously on an individual system. For instance, in the Bose’s double-prism experiment , tunnelling and perfect anticoincidence were observed in single photon states. Consequently, the meaning of the wave-particle duality must incorporate the simultaneous use of the two classical descriptions in the interpretation of experiments, loosing their original mutual exclusivity , which is incorporated as an extreme case in the new interferometric duality, a continuous quantum concept . The wave-particle duality, therefore, must be formulated as an interpretative addition to quantum mechanics, to which is possible to renounce if any pretension of visualize quantum phenomena in terms of classical concepts and intuitions is abandoned.
Abstract The wave-particle duality, as a manifestation of Bohr’s complementarity, is usually quantified in terms of path predictability and interference visibility. Various characterizations of the wave-particle duality have been proposed from an operational perspective, most of them are in forms of inequalities, and some of them are expressed in forms of equalities by incorporating entanglement or coherence. In this work, we shed different insights into the nature of the wave-particle duality by casting it into a form of information conservation in a multi-path interferometer, with uncertainty as a unified theme. More specifically, by employing the simple yet fundamental concept of variance, we establish a resolution of unity, which can be interpreted as a complementarity relation among wave feature, particle feature, and mixedness of a quantum state. This refines or reinterprets some conventional approaches to wave-particle duality, and highlights informational aspects of the issue. The key idea of our approach lies in that a quantum state, as a Hermitian operator, can also be naturally regarded as an observable, with measurement uncertainty (in a state) and state uncertainty (in a measurement) being exploited to quantify particle feature and wave feature of a quantum state, respectively. These two kinds of uncertainties, although both are defined via variance, have fundamentally different properties and capture different features of a state. Together with the mixedness, which is a kind of uncertainty intrinsic to a quantum state, they add up to unity, and thus lead to a characterization of the wave-particle-mixedness complementarity. This triality relation is further illustrated by examples and compared with some popular wave-particle duality or triality relations.
Complementarity, e.g., the wave–particle duality of nature, lies at the heart of quantum mechanics. It distinguishes the world of quantum phenomena from the reality of classical physics. In the 1920s, quantum theory as we know it today was still new, and examples used to illustrate complementarity emphasized the position (particle-like) and momentum (wave-like) attributes of a quantum mechanical object, be it a photon or a massive particle. This is the historical reason why complementarity is often superficially identified with the so-called wave-particle duality of matter . Complementarity, however, is a more general concept. We say that two observables are complementary if precise knowledge of one of them implies that all possible outcomes of measuring the other one are equally probable. We may illustrate this by two extreme examples. The first example consists of the position and momentum (along one direction) of a particle: if, say, the position is predetermined then the result of a momentum measurement cannot be predicted, all momentum values are equally probable (in a large range). The second extreme involves two orthogonal spin components of a spin- 1/2 particle: if, say, the vertical spin component has a definite value ( up or down ) then upon measuring a horizontal component both values ( left or right , for instance) are found, each with a probability of 50%. Thus, in the microcosmos complete knowledge in the sense of classical physics is not available. The classic example of the merger of wave and particle behavior is provided by Young's double-slit experiment.
We derive a generalized wave-particle duality relation for arbitrary multipath quantum interference phenomena. Beyond the conventional notion of the wave nature of a quantum system, i.e., the interference fringe visibility, we introduce a quantifier as the normalized quantum coherence, recently defined in the framework of quantum information theory. To witness the particle nature, we quantify the path distinguishability or the which-path information based on unambiguous quantum state discrimination. Then, the Bohr complementarity principle for multipath quantum interference can be stated as a duality relation between the quantum coherence and the path distinguishability. For two-path interference, the quantum coherence is identical to the interference fringe visibility, and the relation reduces to the well-known complementarity relation. The duality relation continues to hold in the case where mixedness is introduced due to possible decoherence effects.