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arXiv:2303.10238 · Physical Review X

Observation of a Prethermal U(1) Discrete Time Crystal

Andrew Stasiuk, Paola Cappellaro

Published Oct 26, 2023• 20 citations
arXivHTMLPDF

Abstract

A time crystal is a state of periodically driven matter that breaks discrete time-translation symmetry.Time crystals have been demonstrated experimentally in various programmable quantum simulators, and they exemplify how nonequilibrium, driven quantum systems can exhibit intriguing and robust properties absent in systems at equilibrium.These robust driven states need to be stabilized by some mechanism, with the preeminent candidates being many-body localization and prethermalization.This introduces additional constraints that make it challenging to experimentally observe time crystallinity in naturally occurring systems.Recent theoretical work has developed the notion of prethermalization without temperature, expanding the class of time-crystal systems to explain time-crystalline observations at (or near) infinite temperature.In this work, we conclusively observe the emergence of a prethermal Uð1Þ time-crystalline state at quasi-infinite temperature in a solid-state NMR quantum emulator by verifying the requisites of prethermalization without temperature.In addition to observing the signature period-doubling behavior, we show the existence of a long-lived prethermal regime whose lifetime is significantly enhanced by strengthening an emergent Uð1Þ conservation law.Not only do we measure this enhancement through the global magnetization, but we also exploit on-site disorder to measure local observables, ruling out the possibility of many-body localization and confirming the emergence of long-range correlations.

DOI
10.1103/physrevx.13.041016

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A time crystal is a state of periodically driven matter that breaks discrete time-translation symmetry.Time crystals have been demonstrated experimentally in various programmable quantum simulators, and they exemplify how nonequilibrium, driven quantum systems can exhibit intriguing and robust properties absent in systems at equilibrium.These robust driven states need to be stabilized by some mechanism, with the preeminent candidates being many-body localization and prethermalization.This introduces additional constraints that make it challenging to experimentally observe time crystallinity in naturally occurring systems.Recent theoretical work has developed the notion of prethermalization without temperature, expanding the class of time-crystal systems to explain time-crystalline observations at (or near) infinite temperature.In this work, we conclusively observe the emergence of a prethermal Uð1Þ time-crystalline state at quasi-infinite temperature in a solid-state NMR quantum emulator by verifying the requisites of prethermalization without temperature.In addition to observing the signature period-doubling behavior, we show the existence of a long-lived prethermal regime whose lifetime is significantly enhanced by strengthening an emergent Uð1Þ conservation law.Not only do we measure this enhancement through the global magnetization, but we also exploit on-site disorder to measure local observables, ruling out the possibility of many-body localization and confirming the emergence of long-range correlations.
While a clean, driven system generically absorbs energy until it reaches "infinite temperature," it may do so very slowly exhibiting what is known as a prethermal regime. Here, we show that the emergence of an additional approximately conserved quantity in a periodically driven (Floquet) system can give rise to an analogous long-lived regime. This can allow for nontrivial dynamics, even from initial states that are at a high or infinite temperature with respect to an effective Hamiltonian governing the prethermal dynamics. We present concrete settings with such a prethernial regime, one with a period-doubled (time-crystalline) response. We also present a direct diagnostic to distinguish this prethermal phenomenon from its infinitely long-lived many-body localized cousin. We apply these insights to a model of the recent NMR experiments by Rovny et al. [Phys. Rev. Lett. 120, 180603 (2018)] which, intriguingly, detected signatures of a Floquet time crystal in a clean three-dimensional material. We show that a mild but subtle variation of their driving protocol can increase the lifetime of the time-crystalline signal by orders of magnitude.
We present fresh evidence for the presence of discrete quantum time crystals in two spatial dimensions. Discrete time crystals are intricate quantum systems that break discrete time translation symmetry in driven quantum many-body systems undergoing nonequilibrium dynamics. They are stabilized by many-body localization arising from disorder. We directly target the thermodynamic limit using instances of infinite tensor network states, and we implement disorder in a translationally invariant setting by introducing auxiliary systems at each site. We discuss how such disorder can be realized in programmable quantum simulators: This gives rise to the interesting situation in which a classical tensor network simulation can contribute to devising a blueprint of a quantum simulator featuring prethermal time crystalline dynamics, one that will ultimately have to be built in order to explore the stability of this phase of matter for long times.
The discrete time crystal (DTC) is a nonequilibrium phase of matter that spontaneously breaks time-translation symmetry. Disorder-induced many-body localization can stabilize the DTC phase by breaking ergodicity and preventing thermalization. Here, we observe the hallmark signatures of the many-body–localized DTC using a quantum simulation platform based on individually controllable carbon-13 nuclear spins in diamond. We demonstrate long-lived period-doubled oscillations and confirm that they are robust for generic initial states, thus showing the characteristic time-crystalline order across the many-body spectrum. Our results are consistent with the realization of an out-of-equilibrium Floquet phase of matter and introduce a programmable quantum simulator based on solid-state spins for exploring many-body physics.
Prethermal discrete time crystals (DTCs) are a novel phase of periodically driven matter that exhibits robust subharmonic oscillations without requiring disorder. However, previous realizations of prethermal DTCs have relied on the presence of polarization, either spontaneous or induced. Here we introduce a class of prethermal DTCs termed ``unpolarized prethermal discrete time crystals'' (UPDTCs) that arise without any uniform or staggered polarization and propose an experiment to observe them in current trapped-ion quantum simulators. By studying a model of trapped ions using a quantum circuit simulator, we demonstrate that robust period-doubled dynamics can persist in the autocorrelation function of the staggered magnetization, even though its expectation value does not exhibit such dynamics. The period-doubled dynamics is not explained by the classical picture of flipping spins but by quantum fluctuations. We establish that UPDTCs are exponentially long-lived in the high-frequency driving regime, a hallmark of prethermalization. These results expand the known phenomenology and mechanism of prethermal time crystals and underscore the role of quantum effects in stabilizing novel nonequilibrium phases.
Extending the framework of statistical physics to the nonequilibrium setting has led to the discovery of previously unidentified phases of matter, often catalyzed by periodic driving. However, preventing the runaway heating that is associated with driving a strongly interacting quantum system remains a challenge in the investigation of these newly discovered phases. In this work, we utilize a trapped-ion quantum simulator to observe the signatures of a nonequilibrium driven phase without disorder-the prethermal discrete time crystal. Here, the heating problem is circumvented not by disorder-induced many-body localization, but rather by high-frequency driving, which leads to an expansive time window where nonequilibrium phases can emerge. Floquet prethermalization is thus presented as a general strategy for creating, stabilizing, and studying intrinsically out-of-equilibrium phases of matter.
The idea of breaking time-translation symmetry has fascinated humanity at least since ancient proposals of the perpetuum mobile. Unlike the breaking of other symmetries, such as spatial translation in a crystal or spin rotation in a magnet, time translation symmetry breaking (TTSB) has been tantalisingly elusive. We review this history up to recent developments which have shown that discrete TTSB does takes place in periodically driven (Floquet) systems in the presence of many-body localization. Such Floquet time-crystals represent a new paradigm in quantum statistical mechanics --- that of an intrinsically out-of-equilibrium many-body phase of matter. We include a compendium of necessary background, before specializing to a detailed discussion of the nature, and diagnostics, of TTSB. We formalize the notion of a time-crystal as a stable, macroscopic, conservative clock --- explaining both the need for a many-body system in the infinite volume limit, and for a lack of net energy absorption or dissipation. We also cover a range of related phenomena, including various types of long-lived prethermal time-crystals, and expose the roles played by symmetries -- exact and (emergent) approximate -- and their breaking. We clarify the distinctions between many-body time-crystals and other ostensibly similar phenomena dating as far back as the works of Faraday and Mathieu. En route, we encounter Wilczek's suggestion that macroscopic systems should exhibit TTSB in their ground states, together with a theorem ruling this out. We also analyze pioneering recent experiments detecting signatures of time crystallinity in a variety of different platforms, and provide a detailed theoretical explanation of the physics in each case. In all existing experiments, the system does not realize a `true' time-crystal phase, and we identify necessary ingredients for improvements in future experiments.