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arXiv:2302.14328 · Physical review. B./Physical review. B

Emergent glassiness in the disorder-free Kitaev model: Density matrix renormalization group study on a one-dimensional ladder setting

K. B. Yogendra, Tanmoy Das, G. Baskaran

Published Oct 12, 2023• 13 citations
arXivHTMLPDF

Abstract

The complete phase diagram of the Kitaev model with a magnetic field remains elusive, as do the experimental results in the candidate material $\ensuremath{\alpha}\ensuremath{-}{\mathrm{RuCl}}_{3}$. Here, we study the Kitaev model on a one-dimensional ladder setting within the density-matrix renormalization group method in the presence of a magnetic field at zero temperature. We find five distinct phases with increasing magnetic field, which are characterized by a homogeneous flux phase, the ${Z}_{2}$ vortex gas, solid and emergent glass phase, and finally, a spin-polarized phase. The emergent glassiness is confirmed by calculating correlation functions showing quasi-long-range behavior and ground state fidelity, showing a plethora of energetically accessible orthogonal saddle points corresponding to different flux configurations. This glassy behavior seems to arise from the slow dynamics of the ${Z}_{2}$ fluxes, which is a consequence of the local constraints present in the underlying Hilbert space. This phenomenon can also be explored in other spin-liquid systems where the corresponding low-energy excitations are similarly retarded due to constraints.

DOI
10.1103/physrevb.108.165118

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The complete phase diagram of the Kitaev model with a magnetic field remains elusive, as do the experimental results in the candidate material \ensuremathα\ensuremath−RuCl3\ensuremath{\alpha}\ensuremath{-}{\mathrm{RuCl}}_{3}\ensuremathα\ensuremath−RuCl3​. Here, we study the Kitaev model on a one-dimensional ladder setting within the density-matrix renormalization group method in the presence of a magnetic field at zero temperature. We find five distinct phases with increasing magnetic field, which are characterized by a homogeneous flux phase, the Z2{Z}_{2}Z2​ vortex gas, solid and emergent glass phase, and finally, a spin-polarized phase. The emergent glassiness is confirmed by calculating correlation functions showing quasi-long-range behavior and ground state fidelity, showing a plethora of energetically accessible orthogonal saddle points corresponding to different flux configurations. This glassy behavior seems to arise from the slow dynamics of the Z2{Z}_{2}Z2​ fluxes, which is a consequence of the local constraints present in the underlying Hilbert space. This phenomenon can also be explored in other spin-liquid systems where the corresponding low-energy excitations are similarly retarded due to constraints.
We study the Kitaev spin ladder with random couplings by using the real-space strong-disorder renormalization group (SDRG) technique. This model is the minimum model in Kitaev systems that has conserved plaquette fluxes, and its quasi-one-dimensional geometry makes it possible to study the strong-disorder fixed points for both spin- and flux-excitation gaps. In the Ising limit where the xxx-type Ising couplings compete with the zzz-type couplings and the yyy-type couplings are small but nonzero, the behavior of the spin gap is consistent with a random transverse-field Ising chain, but the flux gap is dominated by the yyy-type couplings. In the XX limit, while the xxx- and yyy-type couplings are locally equal and renormalized simultaneously, the zzz-type couplings are not renormalized drastically and lead to nonuniversal disorder criticality at low-energy scales. We show that different types of fractionalized degrees of freedom in the disordered Kitaev model can result in different critical behaviors, as long as its fluxes can survive the perturbative treatment.
Motivated by intense research on two-dimensional spin-12\frac{1}{2}21​ Kitaev materials, Kitaev spin chains and ladders, though geometrically limited, have been studied for their numerical simplicity and insights into extended Kitaev models. The phase diagrams under the magnetic field were also explored for these quasi-one-dimensional models. For an isotropic Kitaev chain, it was found that a magnetic field polarizes the ground state except along the symmetric field angle, where the chain is found to remain gapless up to a critical field strength where it enters an intriguing soliton phase before reaching the polarized state at higher field strengths. Here we study an anisotropic Kitaev chain under a magnetic field using the density matrix renormalization group technique, where the ground state has a macroscopic degeneracy with a finite gap in the absence of the magnetic field. When the field is mainly aligned parallel to the strong bond, four-site and large unit-cell ordered phases arise. In a certain angle of the field, another ordered phase characterized by a uniform chirality with six-site periodicity emerges. We employ a perturbation theory to understand such field-induced ordered phases. The effective model uncovers the presence of transverse Ising and Dzyaloshinskii-Moriya interactions between unit cells, as well as further-neighbor Ising interaction induced by the magnetic field, which collectively explain the mechanisms behind these ordered states. Open questions and challenges are also discussed.
Interactions between the microscopic constituents of a solid---a many-body system--- can lead to novel phases and exotic physical phenomena like fractionalization, topological order, quantum spin liquids, emergent gauge field, etc.. The concept of frustration provides a ground for such exotic phenomena. Frustration can prevent a many-body system from establishing long-range order down to the lowest temperatures due to competing interactions. Instead, competing interactions may result in disordered and liquid-like phases of matter that provide the vacuum for fractional excitations. The absence of any order parameter in strongly frustrated systems---due to not breaking any symmetry spontaneously--- immediately raises the question about possible experimental probes of spin-liquids and their fractional excitations. Dynamic probes, like inelastic neutron scattering or Raman scattering, provide an experimental method to detect signatures of fractionalised quasiparticles. The energy and momentum transferred in a scattering event is split between the fractional quasiparticles. On the theory side, computing such dynamical signatures beyond one spatial dimension is generally a difficult task. In this thesis, numerical methods like density matrix renormalisation group and matrix product states are used to study strongly frustrated magnets and their dynamics in a non-perturbative way. This thesis covers two physical models in the context of frustration and emergent gauge fields. Firstly, the Kitaev model of spin-1/2 degrees of freedom subject to strongly anisotropic spin exchange. The Kitaev model features quantum spin liquid ground states with fractionalization of spins into Majorana fermions and Z_2-fluxes---the visons of an emergent Z_2 gauge theory. The main questions addressed here concern the stability of the quantum spin liquid phase upon adding perturbations relevant in magnetic compounds such as Heisenberg or the symmetric-offdiagonal Gamma exchange. Applying a magnetic field drives the Kitaev model into a topologically ordered phase. The excitations and dynamical signatures within the spin liquid, the topologically ordered phase, and within ordered phases are studied. Secondly, a classical minimal model of the proton configuration in water ice is studied. The ice rules, a local constraint describing the low energy manifold, result in emergent Maxwell's equation. Upon applying an external electric field along certain axis, a polarization plateau occurs in which the remaining degrees of freedom can be described by dimers on two-dimensional lattices.
Recently there has been considerable excitement surrounding the promising realization of high-spin Kitaev material, such as the quasi-2D compound CrI3_33​ and CrGeTe3_33​. However, the stability of quantum spin liquids (QSL) against single ion anisotropy (SIA) in these materials and the global quantum phase diagram of the extended spin-3/2 Kitaev model with finite SIA remain unclear. In this study, we perform large-scale density matrix renormalization group (DMRG) to explore the quantum phase diagram of the generalized spin-3/2 Kitaev-Heisenberg (K-H) model accompanied with SIA AcA_cAc​. In the Ac=0A_c=0Ac​=0 limit, the spin-3/2 K-H model exhibits a quantum phase diagram similar to that of a spin-1/2 system, including two QSLs around antiferromagnetic and ferromagnetic Kitaev models. For models with finite AcA_cAc​, we map out the quantum phase diagram around two Kitaev points and observe distinct types of in-plane vortex orders developed from these two QSL phases. Interestingly, series of nearly degenerate vortex configurations are discovered in each vortex phases. Using linear spin-wave theory, we demonstrate that these vortex configurations can be understood as a consequence of the quantum correction on a continuous family of degenerate classical states.
We study the dynamics of fractionalized excitations in a Kitaev spin liquid (KSL) induced by a local magnetic field perpendicular to the Kitaev honeycomb lattice. The local magnetic field induces a dynamic excitation of a pair of fluxes described by a generally particle-hole asymmetric interacting resonant level model and the dynamics resembles that of a Kondo problem. The p-h asymmetry competes with the magnetic field and results in a rich phase diagram. Moreover, the magnetic field breaks the gauge equivalence of the ferromagnetic (FM) and anti-ferromagnetic (AFM) Kitaev couplings of the ground state and leads to dramatically different behaviors for the two cases. The latter experiences a first order phase transition during magnetization whereas the former does not. By studying the response of the KSL to the magnetic field in different regimes, we obtain the RG flow and phase diagram of the system in the whole space. This study can be generalized to the KSL in a uniform magnetic field and help resolve issues in recent experiments on KSL candidates.
We study an extended Kitaev-Heisenberg model including additional anisotropic couplings by using the two-dimensional density-matrix renormalization group method. Calculating the ground-state energy, entanglement entropy, and spin-spin correlation functions, we make a phase diagram of the extended Kitaev-Heisenberg model around the spin-liquid phase. We find a zigzag antiferromagnetic phase, a ferromagnetic phase, a ${120}^{\ensuremath{\circ}}$ antiferromagnetic phase, and two kinds of incommensurate phases around the Kitaev spin-liquid phase. Furthermore, we study the entanglement spectrum of the model, and we find that entanglement levels in the Kitaev spin-liquid phase are degenerate forming pairs, but those in the magnetically ordered phases are nondegenerate. The Schmidt gap defined as the energy difference between the lowest two levels changes at the phase boundary adjacent to the Kitaev spin-liquid phase. However, we find that phase boundaries between magnetically ordered phases do not necessarily agree with the change of the Schmidt gap.