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arXiv:2302.14047 · Physical Review Research

Third quantization of open quantum systems: Dissipative symmetries and connections to phase-space and Keldysh field-theory formulations

Alexander McDonald, Aashish A. Clerk

Published Aug 16, 2023• 33 citations
arXivHTMLPDF

Abstract

The connections between standard theoretical tools used to study open quantum systems can sometimes seem opaque. Whether it is a Lindblad master equation, the equation of motion for the Wigner function, or a dissipative Keldysh action, features evident in one formalism are often masked in another. Here, we reformulate the technique of third quantization in a way that explicitly connects all three methods. We first show that our formulation reveals a fundamental dissipative symmetry present in all quadratic bosonic or fermionic Lindbladians. This symmetry can then be used to easily diagonalize these models, and it provides an intuitive way to demonstrate the separation of dissipation and fluctuations in linear systems. For bosons, we then show that the Wigner function and the characteristic function can be thought of as ``wave functions'' of the density matrix in the eigenbasis of the third-quantized superoperators we introduce. The field-theory representation of the time-evolution operator in this basis is then the Keldysh path integral. To highlight the utility of our approach, we apply our version of third quantization to a dissipative nonlinear oscillator, and we use it to obtain new exact results.

DOI
10.1103/physrevresearch.5.033107

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The connections between standard theoretical tools used to study open quantum systems can sometimes seem opaque. Whether it is a Lindblad master equation, the equation of motion for the Wigner function, or a dissipative Keldysh action, features evident in one formalism are often masked in another. Here, we reformulate the technique of third quantization in a way that explicitly connects all three methods. We first show that our formulation reveals a fundamental dissipative symmetry present in all quadratic bosonic or fermionic Lindbladians. This symmetry can then be used to easily diagonalize these models, and it provides an intuitive way to demonstrate the separation of dissipation and fluctuations in linear systems. For bosons, we then show that the Wigner function and the characteristic function can be thought of as ``wave functions'' of the density matrix in the eigenbasis of the third-quantized superoperators we introduce. The field-theory representation of the time-evolution operator in this basis is then the Keldysh path integral. To highlight the utility of our approach, we apply our version of third quantization to a dissipative nonlinear oscillator, and we use it to obtain new exact results.
Abstract Open quantum systems that interact with a Markovian environment can be described by a Lindblad master equation. The generator of time-translation is given by a Liouvillian superoperator acting on the density matrix of the system. As the Fock space for a single bosonic mode is already infinite-dimensional, the diagonalization of the Liouvillian has to be done on the creation- and annihilation-superoperators, a process called ‘third quantization’. We propose a method to solve the Liouvillian for quadratic systems using a single symplectic transformation. We show that the non-Hermitian effective Hamiltonian of the system, next to incorporating the dynamics of the system, is a tool to analyze its symmetries. As an example, we use the effective Hamiltonian to formulate a -‘symmetry’ of an open system. We describe how the inclusion of source terms allows us to obtain the cumulant generating function for observables such as the photon current.
Abstract The dynamics of Markovian open quantum systems are described by Lindblad master equations. For fermionic and bosonic systems that are quasi-free, i.e. with Hamiltonians that are quadratic in the ladder operators and Lindblad operators that are linear in the ladder operators, we derive the equation of motion for the covariance matrix. This determines the evolution of Gaussian initial states and the steady states, which are also Gaussian. Using ladder super-operators (a.k.a. third quantization), we show how the Liouvillian can be transformed to a many-body Jordan normal form which also reveals the full many-body spectrum. Extending previous work by Prosen and Seligman, we treat fermionic and bosonic systems on equal footing with Majorana operators, shorten and complete some derivations, also address the odd-parity sector for fermions, give a criterion for the existence of bosonic steady states, cover non-diagonalizable Liouvillians also for bosons, and include quadratic systems. In extension of the quasi-free open systems, quadratic open systems comprise additional Hermitian Lindblad operators that are quadratic in the ladder operators. While Gaussian states may then evolve into non-Gaussian states, the Liouvillian can still be transformed to a useful block-triangular form, and the equations of motion for k -point Green’s functions form a closed hierarchy. Based on this formalism, results on criticality and dissipative phase transitions in such models are discussed in a companion paper.
We develop a theory of symmetry in open quantum systems.Using the operator-state mapping, we characterize symmetry of Liouvillian superoperators for the open quantum dynamics by symmetry of operators in the double Hilbert space and apply the 38-fold internal-symmetry classification of non-Hermitian operators.We find rich symmetry classification due to the interplay between symmetry in the corresponding closed quantum systems and symmetry inherent in the construction of the Liouvillian superoperators.As an illustrative example of open quantum bosonic systems, we study symmetry classes of dissipative quantum spin models.For open quantum fermionic systems, we develop the Z 4 classification of fermion parity symmetry and antiunitary symmetry in the double Hilbert space, which contrasts with the Z 8 classification in closed quantum systems.We also develop the symmetry classification of open quantum fermionic many-body systems-a dissipative generalization of the Sachdev-Ye-Kitaev (SYK) model described by the Lindblad master equation.We establish the periodic tables of the SYK Lindbladians and elucidate the difference from the SYK Hamiltonians.Furthermore, from extensive numerical calculations, we study its complex-spectral statistics and demonstrate dissipative quantum chaos enriched by symmetry.
Phenomenological Equations of Motion for Dissipative Systems Lagrangian Hamiltonian and Hamilton-Jacobi Formulation of the Classical Dissipative Systems Noether's Theorem and Non-Noether Conservation Laws Dissipative Forces Derived from Many-Body Problems A Particle Coupled to a Field and the Damped Motion of a Central Particle Coupled to a Heat Bath Quantization of Dissipative Systems in General and of Explicitly Time-Dependent Hamiltonians in Particular Density Matrix and the Wigner Distribution Function for Damped Systems Path Integral Formulation of a Damped Harmonic Oscillator Quantization of the Motion of an Infinite Chain Heisenberg's Equations of Motion for a Particle Coupled to a Heat Bath Quantum Mechanical Models of Dissipative Systems and the Concept of Optical Potential.
The extraordinary quantum properties of nonequilibrium systems governed by dissipative dynamics have become a focal point in contemporary scientific inquiry. The nonequilibrium Green's functions (NEGF) theory provides a versatile method for addressing driven nondissipative systems, utilizing the powerful diagrammatic technique to incorporate correlation effects. We here present a second-quantization approach to the dissipative NEGF theory, reformulating Keldysh ideas to accommodate Lindbladian dynamics and extending the Kadanoff-Baym equations accordingly. Generalizing diagrammatic perturbation theory for many-body Lindblad operators, the formalism enables correlated and dissipative real-time simulations for the exploration of transient and steady-state changes in the electronic, transport, and optical properties of materials.
The exact solution of the Lindblad equation with a quadratic Hamiltonian and linear coupling operators was derived within the chord representation, that is, for the Fourier transform of the Wigner function, also known as the characteristic function. It is here generalized for several degrees of freedom, so as to provide an explicit expression for the reduced density operator of any subsystem, as well as moments expressed as derivatives of this evolving chord function. The Wigner function is then the convolution of its straightforward classical evolution with a widening multidimensional Gaussian window, eventually ensuring its positivity. Futher on, positivity also holds for the Glauber-Sundarshan P function, which guarantees separability of the components. In the context of several degrees of freedom, a full dissipation matrix is defined, whose trace is equal to twice the previously derived dissipation coefficient. This governs the rate at which the phase space volume of the argument of the Wigner function contracts, while that of the chord function expands. Examples of Markovian evolution of a triatomic molecule and of an array of harmonic oscillators are discussed.