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arXiv:2302.12575 · Physical Review Letters

Fast Single-Shot Imaging of Individual Ions via Homodyne Detection of Rydberg-Blockade-Induced Absorption

Jinjin Du, Thibault Vogt, Wenhui Li

Published Apr 6, 2023• 1 citation
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Abstract

We introduce well-separated ^{87}Rb^{+} ions into an atomic ensemble by microwave ionization of Rydberg excitations and realize single-shot imaging of the individual ions with an exposure time of 1 μs. This imaging sensitivity is reached by using homodyne detection of ion-Rydberg-atom interaction induced absorption. We obtain an ion detection fidelity of (80±5)% from analyzing the absorption spots in acquired single-shot images. These in situ images provide a direct visualization of the ion-Rydberg interaction blockade and reveal clear spatial correlations between Rydberg excitations. The capability of imaging individual ions in a single shot is of interest for investigating collisional dynamics in hybrid ion-atom systems and for exploring ions as a probe for measurements of quantum gases.

DOI
10.1103/physrevlett.130.143004

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We introduce well-separated ^{87}Rb^{+} ions into an atomic ensemble by microwave ionization of Rydberg excitations and realize single-shot imaging of the individual ions with an exposure time of 1 μs. This imaging sensitivity is reached by using homodyne detection of ion-Rydberg-atom interaction induced absorption. We obtain an ion detection fidelity of (80±5)% from analyzing the absorption spots in acquired single-shot images. These in situ images provide a direct visualization of the ion-Rydberg interaction blockade and reveal clear spatial correlations between Rydberg excitations. The capability of imaging individual ions in a single shot is of interest for investigating collisional dynamics in hybrid ion-atom systems and for exploring ions as a probe for measurements of quantum gases.
Rydberg atoms are currently a very fast-advancing quantum platform. For many interesting and demanding applications, including quantum computation, fast detection of a Rydberg excitation or a Rydberg qubit for information readout would be one of the most desirable developments. We demonstrate single-shot and in situ absorption imaging of individual Rydberg excitations. This level of resolution is achieved using an electromagnetically induced transparency scheme involving a Rydberg energy level that is highly sensitive to the presence of Rydberg atoms due to Förster-resonance-enhanced dipole couplings. Spectroscopic measurements illustrate the existence of the Förster resonance and underscore the state-selectivity of the technique. With an imaging exposure time as short as 3 µs, we successfully resolve linear chains of Rydberg excitations in a one-dimensional configuration. The extracted second-order correlation shows strong anti-bunching due to excitation blockade, and a Fourier analysis reveals the long-range order in the chains of Rydberg excitations. This imaging technique, with minimal destruction, will be of great interest for leveraging ensemble-encoded qubits in quantum computation and quantum simulation applications.
We propose a new all-optical method to image individual Rydberg atoms embedded within dense gases of ground state atoms. The scheme exploits interaction-induced shifts on highly polarizable excited states of probe atoms, which can be spatially resolved via an electromagnetically induced transparency resonance. Using a realistic model, we show that it is possible to image individual Rydberg atoms with enhanced sensitivity and high resolution despite photon-shot noise and atomic density fluctuations. This new imaging scheme could be extended to other impurities such as ions, and is ideally suited to equilibrium and dynamical studies of complex many-body phenomena involving strongly interacting particles. As an example we study blockade effects and correlations in the distribution of Rydberg atoms optically excited from a dense gas.
We study the long-range interaction of a single ion with a highly excited ultracold Rydberg atom and report on the direct observation of an ion-induced Rydberg excitation blockade mediated over tens of micrometer distances. Our hybrid ion-atom system is directly produced from an ultracold atomic ensemble via near-threshold photoionization of a single Rydberg excitation, employing a two-photon scheme that is specifically suited for generating a very low-energy ion. The ion's motion is precisely controlled by small electric fields, which allows us to analyze the blockade mechanism for a range of principal quantum numbers. Finally, we explore the capability of the ion as a high-sensitivity, single-atom-based electric field sensor. The observed ion-Rydberg-atom interaction is of current interest for entanglement generation or studies of ultracold chemistry in hybrid ion-atom systems.
This thesis investigates how a single highly excited atom, called Rydberg atom, can be optically imaged. Direct detection methods based on the scattering of light are hardly applicable due to the small scattering rate of the ground to Rydberg state transition. Instead, a cloud of ground state atoms, normally absorptive, is rendered transparent using electromagnetically induced transparency (EIT), involving an auxiliary probe Rydberg state. The cloud acts as a contrast medium, whose optical response is locally perturbed by the strong Rydberg-Rydberg interaction between the probe and the Rydberg impurity which we want to detect. This perturbation restores absorption within a small volume around the impurity, readily detected and \nspatially resolved on a camera. We call this technique Interaction Enhanced Imaging (IEI). To implement IEI we characterize the optical response of the EIT contrast \nmedium in absence of interactions. By combining measurements of the spatially resolved optical spectrum and of the total Rydberg atom number, we can reconstruct \nthe full one-body density matrix of the three-level system. Next, we excite |nS> or |nP> states and, using IEI, we demonstrate spatially resolved imaging, enabling us \nto study dipolar energy transport. To reach single impurity sensitivity we investigate our current detection fidelity and characterize the signal and noise contributions in \nIEI. We model our interacting system, finding good agreement with experimental data. Based on this model, we predict combinations of Rydberg states for which single-shot single impurity sensitivity should be possible in future experiments.
We demonstrate imaging of ions in an atomic gas with ion-Rydberg-atom interaction induced absorption. This is made possible by utilizing a multiphoton electromagnetically induced transparency (EIT) scheme and the extremely large electric polarizability of a Rydberg state with high orbital angular momentum. We process the acquired images to obtain the distribution of ion clouds and to spectroscopically investigate the effect of the ions on the EIT resonance. Furthermore, we show that our method can be employed to image the dynamics of ions in a time resolved way. As an example, we map out the avalanche ionization of a gas of Rydberg atoms. The minimal disruption and the flexibility offered by this imaging technique make it ideally suited for the investigation of cold hybrid ion-atom systems.
We demonstrate a new approach for fast preparation, manipulation, and collective readout of an atomic Rydberg-state qubit. By making use of Rydberg blockade inside a small atomic ensemble, we prepare a single qubit within $3\text{ }\text{ }\ensuremath{\mu}\mathrm{s}$ with a success probability of ${F}_{p}=0.93\ifmmode\pm\else\textpm\fi{}0.02$, rotate it, and read out its state in $6\text{ }\text{ }\ensuremath{\mu}\mathrm{s}$ with a single-shot fidelity of ${F}_{d}=0.92\ifmmode\pm\else\textpm\fi{}0.04$. The ensemble-assisted detection is 103{10}^{3}103 times faster than imaging of a single atom with the same optical resolution, and enables fast repeated nondestructive measurement. We observe qubit coherence times of $15\text{ }\text{ }\ensuremath{\mu}\mathrm{s}$, much longer than the $\ensuremath{\pi}$ rotation time of 90 ns. Potential applications ranging from faster quantum information processing in atom arrays to efficient implementation of quantum error correction are discussed.