We explore a large
N generalization of the Kitaev model on the honeycomb lattice with a simple nearest-neighbor interacting Hamiltonian. In particular, we focus on the
Z4 case with isotropic couplings, which is characterized by an exact
Z4 1-form symmetry. Guided by symmetry considerations and an analytical study in the single-chain limit, on infinitely long cylinders, we find the model is gapped with an extremely short correlation length. Combined with the
Z4 1-form symmetry, this suggests the model is topologically ordered. To pin down the nature of this phase, we further study the model on both finite and infinitely long strips, where we consistently find a
c=1 conformal field theory (CFT) description, suggesting the existence of chiral edge modes described by a free boson CFT. Further evidence is found by studying the dimer correlators on infinitely long strips. We find the dimer correlation functions show a power-law decay with the exponent close to 2 on the boundary of the strip, while decaying much faster in the bulk. Combined with the topological entanglement entropy extracted from cylinder geometry, we identify the phase as a chiral spin liquid with a $\mathrm{U}{(1)}_{\ensuremath{-}8}$ chiral topological order. A unified perspective for all
ZN type Kitaev models is also discussed.
The frustrated XY model on the honeycomb lattice has drawn lots of attention because of the potential emergence of chiral spin liquid (CSL) with the increasing of frustrations or competing interactions. In this paper, we study the extended spin-
21 XY model with nearest-neighbor
(J1), and next-nearest-neighbor
(J2) interactions in the presence of a three-spins chiral $({J}_{\ensuremath{\chi}})$ term using density matrix renormalization group methods. We obtain a quantum phase diagram with both conventionally ordered and topologically ordered phases. In particular, the long-sought Kalmeyer-Laughlin CSL is shown to emerge under a small ${J}_{\ensuremath{\chi}}$ perturbation due to the interplay of the magnetic frustration and chiral interactions. The CSL, which is a nonmagnetic phase, is identified by the scalar chiral order, the finite spin gap on a torus, and the chiral entanglement spectrum described by chiral
SU(2)1 conformal field theory.
We perform large-scale density matrix renormalization group simulations of the SU(4) Heisenberg model on the honeycomb lattice to address the long-standing question of its ground state in an unbiased and quantitatively controlled manner. We find reliable numerical evidence that the ground state is a gapped spin-orbital liquid, presumably with a Z_{4} topological order, characterized by a finite topological entanglement entropy close to ln(4), the absence of both SU(4) and lattice symmetry breaking, and a variationally optimized ground-state energy well below the previously proposed π-flux variational state. By exploiting full SU(4) symmetry and keeping up to 12 800 SU(4) multiplets, corresponding to more than 1×10^{6} U(1) states, we achieve unprecedented accuracy for two-dimensional SU(4) quantum magnets. Finite-size scaling of energies and entanglement entropies supports a robust gapped phase in the two-dimensional limit, while a gapless critical state on narrow cylinders is identified as a proximate remnant of a Dirac spin-orbital liquid. Our results find the SU(4) honeycomb Heisenberg model a realization of a gapped topological spin-orbital liquid and provide convincing numerical evidence for topological order in a highly symmetric two-dimensional quantum magnet.
The possible existence of a quantum spin liquid (QSL) phase, an exotic state of matter with long-range quantum entanglement and fractionalized excitations, in
α-RuCl
3 has sparked widespread interests in exploring QSLs in various Kitaev models under magnetic fields. Recently, a
K-
J-
Γ-
Γ′ model has been proposed to accurately describe the compound by fitting the measured thermodynamic data, where
J is Heisenberg interaction, and
Γ,
Γ′ are off-diagonal exchanges on top of the dominant Kitaev coupling
K. Based on this effective model, an intermediate QSL phase in presence of an out-of-plane fields along the
[111] direction, between the low-field zigzag order and high-field polarized phase, has been predicted. By combining density matrix renormalization group (DMRG), exponential tensor renormalization group (XTRG), and variational Monte Carlo (VMC) calculations, we address the nature of this QSL phase in the honeycomb
K-
J-
Γ-
Γ′ model under the
[111]-direction field. Our DMRG calculations find the algebraic-like decay of spin correlation function, the finite spin scalar chiral order, and lattice nematic order. Together with the XTRG results of power-law specific heat at low temperature, our findings naturally suggest a gapless nematic chiral spin liquid. On the other hand, our VMC study finds a gapped nematic chiral spin liquid with the variational energy very close to that obtained in DMRG. As VMC finds a very small gap that is beyond the current resolution of both ground-state DMRG and finite-temperature XTRG calculations on finite-width cylinders, we resort the full clarification for the nature of the intermediate QSL to future studies. Lastly, we discuss the implications of our results to the recent experiment on
α-RuCl
3 and the QSL-like phase in a similar
K-
Γ-
Γ′ model.
We study the interplay of competing interactions in spin-
21 triangular Heisenberg model through tuning the first- (
J1), second- (
J2), and third-neighbor (
J3) couplings. Based on a large-scale density-matrix renormalization group calculation, we identify a quantum phase diagram of the system and discover a gapless chiral spin-liquid (CSL) phase in the intermediate
J2 and
J3 regime. This CSL state spontaneously breaks time-reversal symmetry with finite scalar chiral order, and it has gapless excitations implied by a vanishing spin triplet gap and a finite central charge on the cylinder. Moreover, the central charge grows rapidly with the cylinder circumference, indicating emergent spinon Fermi surfaces. To understand the numerical results we propose a parton mean-field spin-liquid state, the
U(1) staggered flux state, which breaks time-reversal symmetry with chiral edge modes by adding a Chern insulator mass to Dirac spinons in the
U(1) Dirac spin liquid. This state also breaks lattice rotational symmetries and possesses two spinon Fermi surfaces driven by nonzero
J2 and
J3, which naturally explains the numerical results. This realizes an example of a gapless CSL state with coexisting spinon Fermi surfaces and chiral edge states, demonstrating the rich family of interesting quantum phases emergent from competing interactions in triangular-lattice magnets.
The chiral central charge
c− is a key topological invariant of the edge characterizing the bulk two-dimensional chiral topological order, but its direct evaluation in microscopic spin models has long been a challenge, especially for non-abelian topological order. Building on the recently developed modular commutator formalism, we numerically obtain
c− directly from single ground-state wave functions of two-dimensional interacting spin models that have chiral topological order. This provides a geometry-independent and bulk diagnostic of chirality. We study two nonintegrable systems -- the Zeeman-Kitaev honeycomb model and the kagome antiferromagnet -- both subjected to scalar spin chirality perturbations. We find that the modular commutator yields results consistent with the expected topological quantum field theories. We also compute the topological entanglement entropy which provides an independent diagnostic of the topological orders. Our work establishes modular commutators as a powerful numerical probe of chiral topological order in strongly correlated quantum magnets.