Chirality, or handedness, is a geometrical property denoting a lack of mirror symmetry. Chirality is ubiquitous in nature and is associated with the nonreciprocal interactions observed in complex systems ranging from biomolecules to topological materials. Here, we demonstrate that chiral arrangements of dipole-coupled atoms or molecules can facilitate the helicity-dependent superradiant emission of light. We show that the collective modes of these systems experience an emergent spin-orbit coupling that leads to chirality-dependent photon transport and nontrivial topological properties. These phenomena are fully described within the electric dipole approximation, resulting in very strong optical responses. Our results demonstrate an intimate connection between chirality, superradiance, and photon helicity and provide a comprehensive framework for studying electron transport dynamics in chiral molecules using cold atom quantum simulators. Published by the American Physical Society 2024
Chirality, or handedness, is a geometrical property denoting a lack of mirror symmetry. Chirality is ubiquitous in nature and is associated with the nonreciprocal interactions observed in complex systems ranging from biomolecules to topological materials. Here, we demonstrate that chiral arrangements of dipole-coupled atoms or molecules can facilitate the helicity-dependent superradiant emission of light. We show that the collective modes of these systems experience an emergent spin-orbit coupling that leads to chirality-dependent photon transport and nontrivial topological properties. These phenomena are fully described within the electric dipole approximation, resulting in very strong optical responses. Our results demonstrate an intimate connection between chirality, superradiance, and photon helicity and provide a comprehensive framework for studying electron transport dynamics in chiral molecules using cold atom quantum simulators. Published by the American Physical Society 2024
Chiroptical responses in atomic systems are usually weak, as they arise from the interference between electric- and much weaker magnetic-dipole transitions. We show that atoms arranged in chiral geometries can instead exhibit a strong collective chiroptical response mediated entirely by electric-dipole interactions. Using a coupled-dipole framework, we identify a regime of pronounced chiroptical response emerging at subwavelength interatomic separations, which can be tuned by the probe frequency. This enhancement is directly linked to the formation of subradiant collective modes. Our results establish a fundamental connection between geometric chirality and collective light-matter interactions, opening new pathways for engineering and exploiting chiral optical responses in atomic systems.
Spin-orbit coupling is of fundamental interest in both quantum optical and condensed matter systems alike. In this work, we show that optically induced electronic excitations in lattices of V-type atoms exhibit an emergent spin-orbit coupling when the geometry is chiral. This spin-orbit coupling arises naturally from the electric dipole interaction between the atomic sites and leads to a nontrivial topology for the lattice band structure. Using a general quantum optical model, we determine analytically the conditions that give rise to spin-orbit coupling and characterize the behavior under various symmetry transformations. We demonstrate that chirality-induced spin-orbit coupling can result from either the chirality of the underlying lattice geometry or the combination of an achiral lattice with a suitably chosen external quantization axis. We then discuss how these results are influenced by dissipation, which breaks time-reversal symmetry and illuminates the distinction between true and false chirality. Our results demonstrate that chiral atom arrays are a robust platform for realizing spin-orbit-coupled topological states of matter.
Nanophotonic components allow the control of the flow of light in integrated optical environments. Thereby, the light’s strong confinement leads to an inherent link between its local polarization and propagation direction which fundamentally alters the physics of light-matter interaction and gives rise to phenomena such as directional emission and direction-dependent coupling strengths [1]. I will present the underlying principles of this chiral light-matter interaction and its consequences for integrated applications [1]. In particular, I will show how we employ this effect to control the direction of spontaneous emission [2] and to realize low-loss nonreciprocal transmission at the single-photon level through a silica nanofiber [3]. We use two different approaches where either an ensemble of spin-polarized atoms is weakly coupled to a nanofiber or a single atom is strongly coupled to the nanofiber via a whispering-gallery-mode resonator. The resulting optical isolators show a strong imbalance between the transmissions in forward and reverse direction and, at the same time, a forward transmissions exceeding 70%. We extended this system to a 4-port device, where a single atom routes photons nonreciprocally from one fiber port to the next. This realizes a quantum optical circulator [4] which can even be prepared in a superposition of its operational modes. The demonstrated systems exemplify a new class of (quantum) nanophotonic devices that are ideally suited for photonic quantum information processing and quantum simulation. [1] Nature 541, 473, (2017). [2] Science 346, 67 (2014). [3] Phys. Rev. X 5, 041036 (2015). [4] Science 354, 1577 (2016).
We demonstrate that light propagation in reciprocal chiral photonic media admits a unified description in terms of an emergent Dirac structure in helicity space. Starting from Maxwell's equations, we reformulate the electromagnetic field as a four-component spinor governed by an effective non-Hermitian optical Dirac equation. In this representation, the magnetoelectric response of the chiral medium appears as a helicity-dependent background that modifies the spectrum and eigenmodes, while the breaking of the spin-degenerate condition generates the intrinsic spin-orbit coupling between helicity and orbital degrees of freedom. After projection onto the positive-frequency sector, the theory reduces to an exact two-level helicity-orbital model. This model is found to have an analytical solution and describes coherent Rabi-like oscillations between spin-orbit-coupled vector modes. Chirality controls the helicity splitting and detuning, whereas the electromagnetic mismatch of the medium determines the coupling strength responsible for oscillatory spin-orbit conversion. The resulting dynamics is constrained by exact conservation of the total angular momentum, leading to reversible conversion between spin and orbital angular momentum with well-defined selection rules. Our work establishes an optical Dirac framework for structured light in chiral media, and provides experimentally accessible predictions for chirality-controlled oscillations, polarization dynamics, and orbital angular momentum conversion in structured optical fields.
Recent advances in generating well controlled dense arrangements of individual atoms in free space have generated interest in understanding how the extended nature of these systems influences superradiance phenomena. Here, we provide an in-depth analysis on how space-dependent light shifts and decay rates induced by dipole-dipole interactions modify the steady-state properties of coherently driven arrays of quantum emitters. We characterize the steady-state phase diagram, with particular focus on the radiative properties in the steady state. Interestingly, we find that diverging from the well-established Dicke paradigm of equal all-to-all interactions significantly modifies the emission properties. In particular, the prominent quadratic scaling of the radiated light intensity with particle number in the steady state—a hallmark of steady-state Dicke superradiance—is entirely suppressed, resulting in only linear scaling with particle number. We show that this breakdown of steady-state superradiance occurs due to the emergence of additional dissipation channels that populate not only superradiant states but also subradiant ones. The additional contribution of subradiant dark states in the dynamics leads to a divergence in the time scales needed to achieve steady states. Building on this, we further show that measurements taken at finite times for extended atom ensembles reveal properties closely mirroring the idealized Dicke scenario. Published by the American Physical Society 2024
A structural pattern emerges across several recent preprints in quantum optics and photonics: the deliberate engineering of *optical mode structure*—spatial, polarization, temporal, and chiral degrees of freedom—as the primary handle for controlling quantum state generation, light–matter coupling, and sensing precision. This synthesis draws on six corpus papers spanning physics.optics and quant-ph, connecting (1) electrically switchable chirality in slow-light photonic-crystal waveguides [corpus:arxiv:2605.30047], (2) bright squeezed vacuum (BSV) as a driver for macroscopic quantum state preparation in matter [corpus:arxiv:2605.30224], (3) BSV-driven strong-field photon subtraction via above-threshold ionization [corpus:arxiv:2605.31160], (4) superradiant intensity-correlation LIDAR exploiting collective thermal-source emission [corpus:arxiv:2605.28378], (5) engineered random states achieving Heisenberg-limited metrology across exponential-dimensional Hilbert space [corpus:arxiv:2605.31442], and (6) security metrics for four-wave-mixing sources derived from interferometric field reconstruction [corpus:arxiv:2605.28695]. The thesis—advanced as a heuristic reading, not a derivation—is that these findings collectively reveal *optical mode structure* (chirality handedness, quadrature phase, photon-number distribution, spatial correlation order, and polarization coherence) as a tunable control knob that simultaneously governs state macroscopicity, directionality of coupling, sensing precision, and information-theoretic security. The falsification path is concrete: if the claimed mode-structure dependences are primary, then removing mode selectivity (e.g., replacing chiral coupling with achiral emission, replacing squeezed with coherent driving, replacing correlated multi-source LIDAR with single-source) should degrade each figure of merit in a predictable, mode-geometry-calculable way. The synthesis is bounded by abstract-only reading and does not claim a shared mathematical formalism across all six papers. --- Authorship: Saluca Agentic AI Research Team (Saluca LLC). AI-drafted from arXiv preprint corpus on the date in the filename. Cited arXiv preprints: 2605.28378, 2605.28695, 2605.28815, 2605.30013, 2605.30047, 2605.30224, 2605.30301, 2605.31160, 2605.31409, 2605.31442