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arXiv:2301.00425 · The Innovation

Revealing excited states of rotational Bose-Einstein condensates

Jianyuan Yin, Zhen Huang, Yongyong Cai, Qiang Du, Lei Zhang

Published Nov 23, 2023• 10 citations
arXivHTMLPDF

Abstract

Rotational Bose-Einstein condensates can exhibit quantized vortices as topological excitations. In this study, the ground and excited states of the rotational Bose-Einstein condensates are systematically studied by calculating the stationary points of the Gross-Pitaevskii energy functional. Various excited states and their connections at different rotational frequencies are revealed in solution landscapes constructed with the constrained high-index saddle dynamics method. Four excitation mechanisms are identified: vortex addition, rearrangement, merging, and splitting. We demonstrate changes in the ground state with increasing rotational frequencies and decipher the evolution of the stability of ground states.

DOI
10.1016/j.xinn.2023.100546

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Rotational Bose-Einstein condensates can exhibit quantized vortices as topological excitations. In this study, the ground and excited states of the rotational Bose-Einstein condensates are systematically studied by calculating the stationary points of the Gross-Pitaevskii energy functional. Various excited states and their connections at different rotational frequencies are revealed in solution landscapes constructed with the constrained high-index saddle dynamics method. Four excitation mechanisms are identified: vortex addition, rearrangement, merging, and splitting. We demonstrate changes in the ground state with increasing rotational frequencies and decipher the evolution of the stability of ground states.
This thesis contains theoretical studies of weakly interacting, trapped Bose-Einstein condensed gases. The main emphasis is on the rotational properties of these systems. A typical Bose-Einstein condensate reacts to external rotation by forming singly quantized vortices. By the word ”typical” we refer to a condensate with repulsive interparticle interactions and with a frozen spin degree of freedom. However, there are some atomic species for which the low-energy interactions are attractive. Moreover, the tuning of different condensate properties is relatively easy. For example, there are ways to experimentally change the effective interaction from repulsive to attractive. For an attractively interacting condensate the vortex is not the only possible rotational state but the sample may also experience rotation through its center of mass. In the first part of the thesis, we analyze some properties of a rotating attractive Bose gas at the zero temperature limit. First, we note that in order to maintain energetical stability, the gas has to be rotated in an external trap which is steeper than a harmonic trap. We study the system in an anharmonic quadratic + quartic potential. The rotating ground state phase-space is determined with analytical and numerical methods. If the interactions are strong enough, the rotating ground state appears to be a state with the rotating center of mass. On the other hand, at the limit of weak interactions the system experiences rotation by forming a multiply quantized vortex. We also determine the spectrum of elementary excitations for these quantum many-particle states. We find that the broken symmetry of the center of mass rotating state induces an additional zero-energy (Goldstone) mode and that the small oscillations of the ground state exhibit the decoupling between the center of mass and relative motions. If the spin of the atoms is allowed to change freely, a rich variety of topological excitations in condensates can be studied. External rotation is one of the tools for examining the excitations in spinor condensates. In a spinless scalar condensate the appearance of a quantized vortex is manifested by the vortex line in which the condensate density vanishes. In the plane perpendicular to the vortex line, one speaks of the vortex core for the density minimum. We study the properties of slowly rotated F = 1 spinor condensates and show that for ferromagnetic interactions the ground state is a coreless vortex. While the individual spin components may carry ordinary vortices the overall density of the system is coreless. We also study a method to create a point-like monopole structure in a ferromagnetic condensate by suitably imprinting vortices and solitons for different spin components of the condensate.
Dipolar Bose--Einstein condensates (BECs), i.e., BECs with long-range dipole-dipole interactions (DDI), exhibit extraordinarily rich physics and serve as a versatile experimental platform for exploring exotic quantum states of matter. Within the mean-field framework, a dipolar BEC can be described by the Gross--Pitaevskii (GP) model with a DDI term. Its stationary states consist of the ground state, which minimizes the GP energy functional under the normalization constraint, and excited states, which are higher-energy critical points that typically correspond to constrained saddle points. Excited states encode collective excitation modes and play a key role in the dynamical stability and quantum phase transitions of cold-atom systems. However, in contrast to the extensively studied ground state, they remain far less explored numerically, especially in dipolar systems. In this work, we develop a numerical method based on the constrained gentlest ascent dynamics (CGAD) that systematically computes excited states of dipolar BECs by stably targeting constrained saddle points with any prescribed Morse index. Specifically, a semi-implicit sine-pseudospectral discretization with an orthonormalization correction step is adopted, and the nonlocal DDI terms are evaluated efficiently and accurately via the nonuniform fast Fourier transform (NUFFT). The resulting scheme is applied to one-, two-, and three-dimensional dipolar BECs, enabling a detailed numerical investigation of their excited states. Remarkably, our simulations reveal that excited states can persist even in regimes where the ground state of the condensate becomes mean-field unstable. This work provides a computational framework for studying excited states in dipolar quantum gases and offers insights for future theoretical and experimental investigations.
We study ground, symmetric and central vortex states, as well as their energy and chemical potential diagrams, in rotating Bose-Einstein condensates (BEC) analytically and numerically.We start from the three-dimensional (3D) Gross-Pitaevskii equation (GPE) with an angular momentum rotation term, scale it to obtain a four-parameter model, reduce it to a 2D GPE in the limiting regime of strong anisotropic confinement and present its semiclassical scaling and geometrical optics.We discuss the existence/nonexistence problem for ground states (depending on the angular velocity) and find that symmetric and central vortex states are independent of the angular rotational momentum.We perform numerical experiments computing these states using a continuous normalized gradient flow (CNGF) method with a backward Euler finite difference (BEFD) discretization.Ground, symmetric and central vortex states, as well as their energy configurations, are reported in 2D and 3D for a rotating BEC.Through our numerical study, we find various configurations with several vortices in both 2D and 3D structures, energy asymptotics in some limiting regimes and ratios between energies of different states in a strong replusive interaction regime.Finally we report the critical angular velocity at which the ground state loses symmetry, numerical verification of dimension reduction from 3D to 2D, errors for the Thomas-Fermi approximation, and spourous numerical ground states when the rotation speed is larger than the minimal trapping frequency in the xy plane.
We investigate the ground states and rich dynamics of vortices in spin-orbit coupled Bose-Einstein condensates (BEC) subject to position-dependent detuning. Such a detuning plays the role of an effective rotational frequency, causing the generation of a synthetic magnetic field. Through scanning the detuning gradient, we numerically obtain static vortex lattice structures containing 1 to 6 vortices using the coupled Gross-Pitaevskii equations. When quenching detuning gradient below its initial value, the vortex lattices exhibit interesting periodic rotation motion, and their dynamical stability can persist for up to 1000ms. In particular, depending on the detuning gradient, the twin vortices exhibit either a scissors-like rotational oscillation or a clockwise periodic rotation, reflecting the response to the magnetic field gradient experienced by the condensates. We fit the numerical results to quantitatively analyze the relation between rotation dynamics and magnetic field gradients. When quenching the detuning gradient beyond its initial value, additional vortices appear. Our findings may motivate further experimental studies of vortex dynamics in synthetic magnetic fields and offer insights for engineering a BEC-based magnetic field gradiometer.
The condensation of weakly interacting alkali atom gases observed in 1995 is a manifestation of the macroscopic quantum phenomenon called Bose-Einstein condensation. In contrast to superconductivity and Helium superfluids, the dilute alkali atom condensates are directly observable using optical imaging techniques and they constitute highly controllable quantum systems. Hence, they offer an ideal test bench to investigate the applicability of quantum field theories and to predict the properties of the condensates starting from the first principles.\n\nSince the first experimental realizations of dilute Bose-Einstein condensates, a great interest has been focused on this field, resulting in numerous experimental studies concerning, for example, nonlinear dynamics and the elementary excitations of these many-particle quantum systems. The existence of topological phase singularities, quantized vortices, first predicted theoretically and finally observed experimentally in 1999, led to another series of pioneering theoretical and experimental studies.\n\nSeveral methods to create single-quantum vortices were realized already in 2001 but, however, the puzzle of creating multiply quantized vortices still remained. In this thesis, the so-called topological method to create two and four times quantized vortices is studied in detail. Since the instrumentation required for the experimental realization of the topological method had already been installed in many laboratories, the theoretical predictions of this thesis were experimentally verified shortly after their publication. Multiply quantized vortices are energetically unstable and tend to split into singly quantized vortices. However, the dissipation of energy in the condensates is minimal at low temperatures and, consequently, can lead to long lifetimes for the multiquantum vortices. Nevertheless, one prediction of this thesis is that the lifetimes of doubly quantized vortices are relatively short, owing to the known dynamical instability of the state. The splitting of the doubly quantized vortex has recently been observed experimentally.\n\nThe stability of vortices in dilute Bose-Einstein condensates is intimately related to the excitation spectrum of the stationary vortex state. However, developing an accurate, computationally feasible finite-temperature quantum field theory remains an open problem. In this thesis, we study the elementary excitations of an irrotational condensate within a recently developed systematic second order perturbation theory. The collapse and revival of certain elementary excitations is discovered.\n\nThe most recent studies of this thesis are devoted to stationary, but rotationally asymmetric vortex states. In weakly interacting condensates, a novel stationary state, a vortex tripole holding finite angular momentum is presented. Also the lowest elementary excitations of the so-called vortex dipole, tripole, and quadrupole states are studied.
In this review, we give an overview of the experimental and theoretical advances in the physics of quantized vortices in dilute atomic-gas Bose--Einstein condensates in a trapping potential, especially focusing on experimental research activities and their theoretical interpretations. Making good use of the atom optical technique, the experiments have revealed many novel structural and dynamic properties of quantized vortices by directly visualizing vortex cores from an image of the density profiles. These results lead to a deep understanding of superfluid hydrodynamics of such systems. Typically, vortices are stabilized by a rotating potential created by a laser beam, magnetic field, and thermal gas. Finite size effects and inhomogeneity of the system, originating from the confinement by the trapping potential, yield unique vortex dynamics coupled with the collective excitations of the condensate. Measuring the frequencies of the collective modes is an accurate tool for clarifying the character of the vortex state. The topics included in this review are the mechanism of vortex formation, equilibrium properties, and dynamics of a single vortex and those of a vortex lattice in a rapidly rotating condensate.