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arXiv:2212.14378 · Physical review. B./Physical review. B

Quantum phase transitions in a model Hamiltonian exhibiting entangled simultaneous fermion-pair and exciton condensations

Samuel Warren, LeeAnn M. Sager-Smith, David A. Mazziotti

Published Oct 6, 2022• 3 citations
arXivHTMLPDF

Abstract

Quantum states of a novel Bose-Einstein condensate, in which both fermion-pair and exciton condensations are simultaneously present, have recently been realized theoretically in a model Hamiltonian system. Here we identify quantum phase transitions in that model between fermion-pair and exciton condensations based on a geometric analysis of the convex set of ground-state two-particle reduced density matrices (2-RDMs). The 2-RDM set provides a finite representation of the infinite parameter space of Hamiltonians that readily reveals a fermion-pair condensate phase and two distinct exciton condensate phases, as well as the emergence of first- and second-order phase transitions as the particle number of the system is increased. The set, furthermore, shows that the fermion-exciton condensate (FEC) lies along the second-order phase transition between the exciton and fermion-pair condensate phases. The detailed information about the exciton and fermion-pair phases, the forces behind these phases, as well as their associated transitions provides additional insight into the formation of the FEC condensate, which we anticipate will prove useful in its experimental realization.

DOI
10.1103/physrevb.106.165107

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Quantum states of a novel Bose-Einstein condensate, in which both fermion-pair and exciton condensations are simultaneously present, have recently been realized theoretically in a model Hamiltonian system. Here we identify quantum phase transitions in that model between fermion-pair and exciton condensations based on a geometric analysis of the convex set of ground-state two-particle reduced density matrices (2-RDMs). The 2-RDM set provides a finite representation of the infinite parameter space of Hamiltonians that readily reveals a fermion-pair condensate phase and two distinct exciton condensate phases, as well as the emergence of first- and second-order phase transitions as the particle number of the system is increased. The set, furthermore, shows that the fermion-exciton condensate (FEC) lies along the second-order phase transition between the exciton and fermion-pair condensate phases. The detailed information about the exciton and fermion-pair phases, the forces behind these phases, as well as their associated transitions provides additional insight into the formation of the FEC condensate, which we anticipate will prove useful in its experimental realization.
Fermion-exciton condensation in which both fermion-pair (i.e., superconductivity) and exciton condensations occur simultaneously in a single coherent quantum state has recently been conjectured to exist. Here, we capture the fermion-exciton condensation through a model Hamiltonian that can recreate the physics of this new class of highly correlated condensation phenomena. We demonstrate that the Hamiltonian generates the large-eigenvalue signatures of fermion-pair and exciton condensations for a series of states with increasing particle numbers. The results confirm that the dual-condensate wave function arises from the entanglement of fermion-pair and exciton wave functions, which we previously predicted in the thermodynamic limit. This model Hamiltonian---generalizing well-known model Hamiltonians for either superconductivity or exciton condensation---can explore a wide variety of condensation behavior. It provides significant insights into the required forces for generating a fermion-exciton condensate, which will likely be invaluable for realizing such condensations in realistic materials with applications from superconductors to excitonic materials.
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An extensive theoretical and experimental investigation has been conducted on fermion-pair condensation and exciton condensation as distinct classes of Bose-Einstein-like condensation. In this Rapid Communication, the existence of a fermion-exciton condensate---a single quantum state in which the characters of both fermion-pair and exciton condensates coexist---is established computationally in the low-particle-number (NNN) limit and theoretically in the large-NNN thermodynamic limit. The trade-off between the fermion-pair and excitonic character of the fermion-exciton condensate is shown to be elliptic in nature. The possibility that the properties of fermion-exciton condensates could be a hybrid of the properties of fermion-pair condensates and exciton condensates is discussed, and future experimental and computational exploration of this class of condensate, which may potentially be realizable in a bilayer of superconductors, is anticipated.
Recently, the two-dimensional nanocavity exciton-polariton system confined in semiconductor nanocavities has emerged as a promising alternative of BoseEinstein Condensate (BEC). The strong quantum correlations presents in this system, make it an unique candidate for studying entanglement and quantum phase transitions —qualitative changes in the ground state properties—. In this work, we review previous evidence, obtained by us, in the phase transitions of a finite exciton-polariton system. First, by using a BCS wave function to compute the ground state energy of N excitons without the photonic field, a crossover from the high-density electron-hole phase to the BCS excitonic phase is found, at a density which is roughly four times the close-packing density of excitons. Second, by means of a self-consistent procedure with a trial function composed of a coherent photon field and a BCS function for the electron-hole pairs, we obtain the scaling of the critical temperature with the number of polaritons. Using the method proposed originally by Olliver and Zurek, and subsequently developed by Bo Li and Zhi-Xi Wang , we calculate the discord for a generalized density operator, proposed by Blaizot
We consider composite bosons (cobosons) comprised two elementary particles, fermions or bosons, in an entangled state. First, we show that the effective number of cobosons implies the level of correlation between the two constituent particles. For the maximum level of correlation, the effective number of cobosons is the same as the total number of cobosons, which can exhibit the original Bose–Einstein condensation (BEC). In this context, we study a model of BEC for indistinguishable cobosons with a controllable parameter, i.e., entanglement between the two constituent particles. We find that bi-fermions behave in a predictable way, i.e., the effective number of the ground state coboson is an increasing function of entanglement between a pair of constituent fermions. Interestingly, bi-bosons exhibit the opposite behavior—the effective number of the ground state coboson is a decreasing function of entanglement between a pair of constituent bosons.
(2)-symmetry interaction in the particle-particle and particle-hole channels is carried out. Using the symmetry of the system, its free energy and phase diagram are calculated. It is demonstrated that the superconducting (particle-particle) and excitonic (particle-hole) condensates are both formed in the considered system which undergoes two phase transitions. The calculated phase diagram represents qualitatively the phase diagram typical for materials with the high-temperature superconducting properties, including the existence of two phase transitions, the first and second order phase transitions, triple and tricritical points.