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arXiv:2212.05437 · Physical Review Letters

Experimental Demonstration of Stationary Dark-State Polaritons Dressed by Dipole-Dipole Interaction

Bongjune Kim, Ko-Tang Chen, Kuei-You Chen, Yu-Shan Chiu, Chia-Yu Hsu, Yi‐Hsin Chen, Ite A. Yu

Published Sep 26, 2023• 7 citations
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Abstract

Dark-state polaritons (DSPs) based on the effect of electromagnetically induced transparency are bosonic quasiparticles, representing the superpositions of photons and atomic ground-state coherences. It has been proposed that stationary DSPs are governed by the equation of motion closely similar to the Schrödinger equation and can be employed to achieve Bose-Einstein condensation (BEC) with transition temperature orders of magnitude higher than that of the atomic BEC. The stationary-DSP BEC is a three-dimensional system and has a far longer lifetime than the exciton-polariton BEC. In this Letter, we experimentally demonstrated the stationary DSP dressed by the Rydberg-state dipole-dipole interaction (DDI). The DDI-induced phase shift of the stationary DSP was systematically studied. Notably, the experimental data are consistent with the theoretical predictions. The phase shift can be viewed as a consequence of elastic collisions. In terms of thermalization to achieve BEC, the μm^{2}-size interaction cross section of the DDI can produce a sufficient elastic collision rate for the stationary DSPs. This Letter makes a substantial advancement toward the realization of the stationary-DSP BEC.

DOI
10.1103/physrevlett.131.133001

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Dark-state polaritons (DSPs) based on the effect of electromagnetically induced transparency are bosonic quasiparticles, representing the superpositions of photons and atomic ground-state coherences. It has been proposed that stationary DSPs are governed by the equation of motion closely similar to the Schrödinger equation and can be employed to achieve Bose-Einstein condensation (BEC) with transition temperature orders of magnitude higher than that of the atomic BEC. The stationary-DSP BEC is a three-dimensional system and has a far longer lifetime than the exciton-polariton BEC. In this Letter, we experimentally demonstrated the stationary DSP dressed by the Rydberg-state dipole-dipole interaction (DDI). The DDI-induced phase shift of the stationary DSP was systematically studied. Notably, the experimental data are consistent with the theoretical predictions. The phase shift can be viewed as a consequence of elastic collisions. In terms of thermalization to achieve BEC, the μm^{2}-size interaction cross section of the DDI can produce a sufficient elastic collision rate for the stationary DSPs. This Letter makes a substantial advancement toward the realization of the stationary-DSP BEC.
We propose and analyze a mechanism for Bose-Einstein condensation of stationary dark-state polaritons. Dark-state polaritons (DSPs) are formed in the interaction of light with laser-driven 3-level Lambda-type atoms and are the basis of phenomena such as electromagnetically induced transparency, ultraslow, and stored light. They have long intrinsic lifetimes and in a stationary setup, a 3D quadratic dispersion profile with variable effective mass. Since DSPs are bosons, they can undergo a Bose-Einstein condensation at a critical temperature which can be many orders of magnitude larger than that of atoms. We show that thermalization of polaritons can occur via elastic collisions mediated by a resonantly enhanced optical Kerr nonlinearity on a time scale short compared to the decay time. Finally, condensation can be observed by turning stationary into propagating polaritons and monitoring the emitted light.
The generation of stationary distributions of light with three-dimensional confinement is discussed and a novel scheme for Bose-Einstein condensation of the associated quasi-particles, dark-state polaritons (DSP), is proposed. DSPs are created in the Raman interaction of laser fields with atoms and are the basis of ultra-slow, stopped, and stationary light. Stationary DSPs have a quadratic dispersion profile with very small and variable effective mass and have a long intrinsic lifetime. Due to the small mass the corresponding condensation temperature can be many orders of magnitude higher than that of atoms. After introducing stationary dark-state polaritons their incoherent generation and thermalization is discussed and conditions for condensation analyzed. Finally potential methods for an experimental observation of the condensation will be put forward.
Abstract The combination of Rydberg atoms and electromagnetically induced transparency (EIT) has been extensively studied in the strong-interaction regime. Here we proposed utilizing an EIT medium with a high optical depth (OD) and a Rydberg state of low principal quantum number to create a many-body system of Rydberg polaritons in the weak-interaction regime. The phase shift and attenuation induced by the dipole–dipole interaction (DDI) were still significant, and can be viewed as the consequences of elastic and inelastic collisions among Rydberg polaritons. We further observed that the width of the transverse momentum distribution of Rydberg polaritons at the exit of the system became notably smaller as compared with that at the entrance. The observation demonstrates the cooling effect in this system. The μs-long interaction time due to the high-OD EIT medium plus the μm2-size collision cross section due to the DDI suggests a feasible platform of polariton Bose–Einstein condensation.
Coupling light to Rydberg states of atoms under conditions of electromagnetically induced transparency (EIT) leads to the formation of interacting quasiparticles, termed Rydberg polaritons. We derive a one-dimensional model describing the time evolution of these polaritons under paraxial propagation conditions. Specifically, we obtain a master equation governing the dynamics of Rydberg polaritons and identify conditions when it can essentially be described by an effective Hamiltonian of a single-species polariton. We verify this Hamiltonian by numerical two-excitation simulations. Under typical stationary EIT conditions it is impossible to reach the strongly interacting regime where long-range density-density correlations emerge. In contrast, by employing the time dependence of the control field the regime of strong interactions can be reached where the polaritons attain quasicrystalline order. We provide a physical explanation for the differences between stationary and time-dependent schemes.
The combination of high optical nonlinearity in the electromagnetically induced transparency (EIT) effect and strong electric dipole-dipole interaction (DDI) among the Rydberg-state atoms can lead to important applications in quantum information processing and many-body physics. One can utilize the Rydberg-EIT system in the strongly-interacting regime to mediate photon-photon interaction or qubit-qubit operation. One can also employ the Rydberg-EIT system in the weakly-interacting regime to study the Bose-Einstein condensation of Rydberg polaritons. Most of the present theoretical models dealt with the strongly-interacting cases. Here, we consider the weakly-interacting regime and develop a mean field model based on the nearest-neighbor distribution. Using the mean field model, we further derive the analytical formulas for the attenuation coefficient and phase shift of the output probe field. The predictions from the formulas are consistent with the experimental data in the weakly-interacting regime, verifying the validity of our model. As the DDI-induced phase shift and attenuation can be seen as the consequences of elastic and inelastic collisions among particles, this work provides a very useful tool for conceiving ideas relevant to the EIT system of weakly-interacting Rydberg polaritons and for evaluating experimental feasibility.
We experimentally observed an accumulative type of nonlinear attenuation and distortion of slow light, i.e., Rydberg polaritons, with the Rydberg state $|32{D}_{5/2}\ensuremath{\rangle}$ in the weak-interaction regime. The present effect of attenuation and distortion cannot be explained by considering only the dipole-dipole interaction (DDI) between Rydberg atoms in $|32{D}_{5/2}\ensuremath{\rangle}$. Our observation can be attributed to the atoms in the dark Rydberg states rather than those in the bright Rydberg state, i.e., $|32{D}_{5/2}\ensuremath{\rangle}$, driven by the coupling field. The dark Rydberg states are all the possible states in which the population decaying from $|32{D}_{5/2}\ensuremath{\rangle}$ accumulated over time, and they were not driven by the coupling field. Consequently, the DDI between the dark and bright Rydberg atoms increased the decoherence rate of the Rydberg polaritons. We performed three different experiments to verify the above hypothesis, to confirm the existence of the dark Rydberg states, and to measure the decay rate from the bright to the dark Rydberg states. In the theoretical model, we included the decay process from the bright to the dark Rydberg states and the DDI effect induced by both the bright and dark Rydberg atoms. All the experimental data of slow light taken at various probe Rabi frequencies were in good agreement with the theoretical predictions based on the model. This study points out an additional decoherence rate in the Rydberg-state electromagnetically induced transparency effect and provides a better understanding of the Rydberg-polariton system.