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arXiv:2212.05372

Multipartite entanglement in the 1-D spin-$\frac{1}{2}$ Heisenberg Antiferromagnet

Varun Menon, Nicholas E. Sherman, Maxime Dupont, Scheie, Allen O., D. M. Tennant, Joel E. Moore

Published Dec 10, 2022• 0 citations
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Abstract

Multipartite entanglement refers to the simultaneous entanglement between multiple subsystems of a many-body quantum system. While multipartite entanglement can be difficult to quantify analytically, it is known that it can be witnessed through the Quantum Fisher information (QFI), a quantity that can also be related to dynamical Kubo response functions. In this work, we first show that the finite temperature QFI can generally be expressed in terms of a static structure factor of the system, plus a correction that vanishes as $T\rightarrow 0$. We argue that this implies that the static structure factor witnesses multipartite entanglement near quantum critical points at temperatures below a characteristic energy scale that is determined by universal properties, up to a non-universal amplitude. Therefore, in systems with a known static structure factor, we can deduce finite temperature scaling of multipartite entanglement and low temperature entanglement depth without knowledge of the full dynamical response function of the system. This is particularly useful to study 1D quantum critical systems in which sub-power-law divergences can dominate entanglement growth, where the conventional scaling theory of the QFI breaks down. The 1D spin-$\frac{1}{2}$ antiferromagnetic Heisenberg model is an important example of such a system, and we show that multipartite entanglement in the Heisenberg chain diverges non-trivially as $\sim \log(1/T)^{3/2}$. We verify these predictions with calculations of the QFI using conformal field theory and matrix product state simulations. Finally we discuss the implications of our results for experiments to probe entanglement in quantum materials, comparing to neutron scattering data in KCuF$_3$, a material well-described by the Heisenberg chain.

DOI
10.48550/arxiv.2212.05372

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Multipartite entanglement in the 1-D spin-12\frac{1}{2}21​ Heisenberg Antiferromagnet
Multipartite entanglement refers to the simultaneous entanglement between multiple subsystems of a many-body quantum system. While multipartite entanglement can be difficult to quantify analytically, it is known that it can be witnessed through the Quantum Fisher information (QFI), a quantity that can also be related to dynamical Kubo response functions. In this work, we first show that the finite temperature QFI can generally be expressed in terms of a static structure factor of the system, plus a correction that vanishes as T→0T\rightarrow 0T→0. We argue that this implies that the static structure factor witnesses multipartite entanglement near quantum critical points at temperatures below a characteristic energy scale that is determined by universal properties, up to a non-universal amplitude. Therefore, in systems with a known static structure factor, we can deduce finite temperature scaling of multipartite entanglement and low temperature entanglement depth without knowledge of the full dynamical response function of the system. This is particularly useful to study 1D quantum critical systems in which sub-power-law divergences can dominate entanglement growth, where the conventional scaling theory of the QFI breaks down. The 1D spin-12\frac{1}{2}21​ antiferromagnetic Heisenberg model is an important example of such a system, and we show that multipartite entanglement in the Heisenberg chain diverges non-trivially as ∼log⁡(1/T)3/2\sim \log(1/T)^{3/2}∼log(1/T)3/2. We verify these predictions with calculations of the QFI using conformal field theory and matrix product state simulations. Finally we discuss the implications of our results for experiments to probe entanglement in quantum materials, comparing to neutron scattering data in KCuF3_33​, a material well-described by the Heisenberg chain.
Multipartite entanglement was thought to be intrinsically difficult to measure in solids, but recent work has established connections between multipartite entanglement, dynamic susceptibilities, and neutron scattering data, via the quantum Fisher information. This work focuses on the paradigmatic spin-half chain and shows that there are further simplifications: even static structure factors contain quantitative information about multipartite entanglement at low temperatures. Theory, numerics, and experiment then suggest that a high degree of multipartite entanglement is observable in Heisenberg chain compounds, including KCuF3{}_{3}3​.
Multipartite-entanglement tomography, namely the quantum Fisher information (QFI) calculated with respect to different collective operators, allows to fully characterize the phase diagram of the quantum Ising chain in a transverse field with variable-range interaction. In particular, it recognizes the phase stemming from long-range (LR) antiferromagnetic interaction, a capability also shared by the spin squeezing. Furthermore, the QFI locates the quantum critical points, both with vanishing and nonvanishing mass gap. In this case, we also relate the finite-size power-law exponent of the QFI to the critical exponents of the model, finding a signal for the breakdown of conformal invariance in the deep LR regime. Finally, the effect of a finite temperature on the multipartite entanglement, and ultimately on the phase stability, is considered. In light of the current realizations of the model with trapped ions and of the potential measurability of the QFI, our approach yields a promising strategy to probe LR physics in controllable quantum systems.
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The quantum Fisher information is of considerable interest not only for quantum metrology but also because it is a useful entanglement measure for finite temperature mixed states. In particular, it estimates the degree to which multipartite entanglement is present. Recent results have related the quantum Fisher information to experimentally measurable probes. While in principle possible, a direct evaluation of the quantum Fisher information at finite temperatures is technically challenging and here we show that a simple estimate can be obtained for materials where the single-mode approximation is valid. We focus on the S=1S=1S=1 antiferromagnetic Heisenberg model with uniaxial anisotropy. Quantum Monte Carlo techniques are used to determine low-temperature correlations from which the quantum Fisher information can be estimated within the single-mode approximation. The quantum Fisher information is compared to the quantum variance for the staggered magnetization operators in the transverse direction and inequalities between the quantum Fisher information, the quantum variance, and the full variance are discussed. Both the quantum and full variance as well as the quantum Fisher information are examined at finite temperatures above the isotropic point and at the quantum critical point for the Haldane-N\'eel transition. A finite size scaling study of the quantum Fisher information is performed at the quantum critical point and used to confirm the Ising nature of the Haldane-N\'eel transition.
Abstract We study the multipartite entanglement of a quantum many-body system undergoing a quantum quench. We quantify the multipartite entanglement through the quantum Fisher information (QFI) density, and we are able to express it after a quench in terms of a generalised response function. For pure state initial conditions and in the thermodynamic limit, we can express the QFI as the fluctuations of an observable computed in the so-called diagonal ensemble. We apply the formalism to the dynamics of a quantum Ising chain, after a quench in the transverse field. In this model the asymptotic state is, in almost all cases, more than two-partite entangled. Moreover, starting from the ferromagnetic phase, we find a divergence of multipartite entanglement for small quenches closely connected to a corresponding divergence of the correlation length.
Quantum Fisher information (QFI) is a measure of multipartite quantum entanglement that can be obtained from inelastic neutron scattering data on quantum magnets. In this work, we demonstrate that the QFI can distinguish an unconventional quantum critical point (QCP) with fractionalization and emergent gauge structure from conventional ones within the Landau paradigm. We compute the QFI, via large-scale quantum Monte Carlo (QMC) simulations and exact diagonalization, in a kagome lattice quantum spin liquid (QSL) model with an XY and a cluster-Ising interactions. When the XY interaction is ferromagetic, the QFI obtained by QMC reveals a large anomalous dimension, which is a fingerprint of the (2+1)d XY∗^\ast∗ universality class for the transition from the ferromagnetic phase to the Z2\mathbb{Z}_2Z2​ QSL. The investigation of thermal and dynamical properties of QFI is further extended to the case of antiferromagnetic XY interaction via exact diagonalization. In this regime, a transition to a possibly distinct QSL phase is suggested via both entanglement-based probes, such as QFI and genuine multipartite negativity, and analyses of the energy spectrum and structure factors. These results not only demonstrate the versatility of QFI in identifying QSL states and unconventional QCPs but also provide useful guidance for future theoretical and experimental studies of frustrated magnets.