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arXiv:2212.04389 · Physical Review Letters

Steady-State Ultracold Plasma Created by Continuous Photoionization of Laser Cooled Atoms

Boris B. Zelener, E V Vilshanskaya, N. V. Morozov, Sergey A. Saakyan, Andrey A. Bobrov, Vladimir A. Sautenkov, B. V. Zelener

Published Mar 15, 2024• 13 citations
arXivHTMLPDF

Abstract

In this Letter we discuss our approach that makes possible creation of the steady-state ultracold plasma having various densities and temperatures by means of continuous two-step optical excitation of calcium atoms in the magneto-optical trap. A strongly coupled ultracold plasma can be used as an excellent test platform for studying many-body interactions associated with various plasma phenomena. The parameters of the plasma are studied using laser-induced fluorescence of calcium ions. The experimental results are well described by a simple theoretical model involving equilibration of the continuous source of charged particles by the hydrodynamical ion outflux and three-body recombination. The ultracold plasma with the peak ion density of 2.7×10^{6} cm^{-3} and the minimum electron temperature near 2 K has been prepared. Our steady-state approach in combination with the strong magnetic confinement of the plasma will make it possible to reach extremely strong coupling in such system.

DOI
10.1103/physrevlett.132.115301

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In this Letter we discuss our approach that makes possible creation of the steady-state ultracold plasma having various densities and temperatures by means of continuous two-step optical excitation of calcium atoms in the magneto-optical trap. A strongly coupled ultracold plasma can be used as an excellent test platform for studying many-body interactions associated with various plasma phenomena. The parameters of the plasma are studied using laser-induced fluorescence of calcium ions. The experimental results are well described by a simple theoretical model involving equilibration of the continuous source of charged particles by the hydrodynamical ion outflux and three-body recombination. The ultracold plasma with the peak ion density of 2.7×10^{6} cm^{-3} and the minimum electron temperature near 2 K has been prepared. Our steady-state approach in combination with the strong magnetic confinement of the plasma will make it possible to reach extremely strong coupling in such system.
By photoionizing samples of laser-cooled atoms with laser light tuned just above the ionization limit, plasmas can be created with electron and ion temperatures below 10 K. These ultracold neutral plasmas have extended the temperature bounds of plasma physics by two orders of magnitude. Table-top experiments, using many of the tools from atomic physics, allow for the study of plasma phenomena in this new regime with independent control over the density and temperature of the plasma through the excitation process. Characteristic of these systems is an inhomogeneous density profile, inherited from the density distribution of the laser-cooled neutral atom sample. Most work has dealt with unconfined plasmas in vacuum, which expand outward at velocities of order 100 m/s, governed by electron pressure, and with lifetimes of order 100 μs, limited by stray electric fields. Using detection of charged particles and optical detection techniques, a wide variety of properties and phenomena have been observed, including expansion dynamics, collective excitations in both the electrons and ions, and collisional properties. Through three-body recombination collisions, the plasmas rapidly form Rydberg atoms, and clouds of cold Rydberg atoms have been observed to spontaneously avalanche ionize to form plasmas. Of particular interest is the possibility of the formation of strongly coupled plasmas, where Coulomb forces dominate thermal motion and correlations become important. The strongest impediment to strong coupling is disorder-induced heating, a process in which Coulomb energy from an initially disordered sample is converted into thermal energy. This restricts electrons to a weakly coupled regime and leaves the ions barely within the strongly coupled regime. This review will give an overview of the field of ultracold neutral plasmas, from its inception in 1999 to current work, including efforts to increase strong coupling and effects on plasma properties due to strong coupling.
Photoionizing laser-cooled atoms produces ultracold neutral plasmas with initial temperatures of 1–1000 K and densities as high as 10 10 cm −3 . Applied radio frequency fields can excite plasma oscillations that are used to monitor the expansion of the unconfined plasma. Significant three-body recombination of electrons and ions into Rydberg atoms takes place during the plasma expansion. Previous experiments have been done with xenon, but a new experiment is planned with laser-cooled strontium. The strontium ion has an optically allowed transition at a convenient blue wavelength. This will allow direct imaging of the plasma through fluorescence or absorption, and may enable laser cooling and trapping of the plasma.
We report the creation of an ultracold neutral plasma by photoionization of laser-cooled xenon atoms. The charge carrier density is as high as $2\ifmmode\times\else\texttimes\fi{}{10}^{9}{\mathrm{cm}}^{\ensuremath{-}3}$, and the temperatures of electrons and ions are as low as 100 mK and $10\ensuremath{\mu}\mathrm{K}$, respectively. Plasma behavior is evident in the trapping of electrons by the positive ion cloud when the Debye screening length becomes smaller than the size of the sample. We produce plasmas with parameters such that both electrons and ions are strongly coupled.
Ultracold neutral plasmas are created by photoionizing laser-cooled atoms in a magneto-optical trap (MOT). Due to their large electrical potential energies and comparatively small kinetic energies, ultracold plasmas fall into a regime of plasma systems which are called “strongly coupled.” A priority in the field of ultracold plasmas is to generate plasmas with higher values of the strong coupling parameter Γ, which is given as the ratio of the nearest-neighbor Coulomb potential energy to the average kinetic energy. The equilibrium strong coupling in ultracold plasmas is limited by the ultrafast relaxation of the ions due to spatial disorder in the initial system. This heating mechanism is called “disorder-induced heating” (DIH) and it limits the ion strong coupling in ultracold plasmas to order unity. This thesis describes experiments that explore ways to generate higher values of the strong coupling parameter in an ultracold neutral calcium plasma.One way to increase Γ is to mitigate the effects of DIH using electron screening. This thesis describes an experiment in which the initial electron temperature was systematically changed to determine the effect that electron screening has on the ion thermalization. At lower initial electron temperatures, corresponding to a higher degree of electron shielding, it was found that the screening slows the ion thermalization and reduces the equilibrium ion temperature by as much as a factor of two. However, electron screening also reduces the ion interaction strength by the same amount, which has the net effect of leaving the effective Γ unchanged.Another method for increasing the strong coupling of an ultracold plasma is to excite the plasma ions to a higher ionization state. Simulations predict that doubly ionizing the plasma ions can increase the strong coupling in an ultracold plasma by as much as a factor of 4, with the maximum value of Γ depending on the timing of the second ionization relative to the DIH process. This thesis describes an experiment designed to test these predictions in a Ca2+ plasma. Measurements of the change in the Ca+ ion temperature as a function of the timing of the second ionization pulses were made using laser-induced fluorescence. Results of these measurements show that the heating of the Ca+ ions due to the second ionization depends on the timing of the second ionization pulses, as predicted by MD simulations.
By photoionizing a sample of laser‐cooled xenon atoms, we create ultracold neutral plasmas with initial temperatures of 1–1000 K and densities as high as 1010 cm−3. The plasma is formed by the trapping of electrons by the residual positive charge that is left after some electrons initially leave the sample. We excite plasma oscillations with applied radio frequency fields and use this to monitor the expansion of the unconfined plasma. We have observed significant recombination of the plasma into Rydberg atoms (up to 20 %). At these low temperatures, the only traditional form of recombination that could be significant is three‐body recombination (TBR). Recent theoretical studies of ultracold plasmas, and prospects for future experiments, are discussed.
By photoionizing a sample of laser-cooled xenon atoms, we create ultracold neutral plasmas with initial temperatures of 1–1000 K and densities as high as 1010 cm−3. The plasma is formed by the trapping of electrons by the residual positive charge that is left after some electrons initially leave the sample. We excite plasma oscillations with applied radio frequency fields and use this to monitor the expansion of the unconfined plasma. We have observed significant recombination of the plasma into Rydberg atoms (up to 20%). At these low temperatures, the only traditional form of recombination that could be significant is three-body recombination (TBR), but we see a number of trends in direct contradiction to what one would expect from classical TBR theory.