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arXiv:2211.13249 · Physical Review Research

Identifying unbound strong bunching and the breakdown of the rotating wave approximation in the quantum Rabi model

Álvaro Nodar, Rubén Esteban, Unai Muniain, Michael J. Steel, Javier Aizpurua, Mikołaj K. Schmidt

Published Dec 7, 2023• 3 citations
arXivHTMLPDF

Abstract

We use a recently derived gauge-invariant formulation of the problem of a two-level system coupled to an optical cavity to explore the transition between the weak and the ultrastrong coupling regimes of light-matter interaction. We explore this transition using the intensity correlations ${g}^{(2)}(\ensuremath{\tau})$ of the emitted light, and we find strong, unbounded bunching of the emission from systems governed by the Rabi Hamiltonian. Surprisingly, this effect is observed not only in the ultrastrong coupling regime, but also for weakly coupled systems, where the Jaynes-Cummings Hamiltonian would predict the opposite, antibunched emission. This suggests that the higher-order correlations are a particularly sensitive probe of the divergence between the Jaynes-Cummings and Rabi Hamiltonians, and they can serve as an indicator of the breakdown of the rotating wave approximation. Our findings indicate also that the boundary between the weakly, strongly, and ultra-strongly-coupled dynamics is much richer than currently accepted.

DOI
10.1103/physrevresearch.5.043213

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We use a recently derived gauge-invariant formulation of the problem of a two-level system coupled to an optical cavity to explore the transition between the weak and the ultrastrong coupling regimes of light-matter interaction. We explore this transition using the intensity correlations g(2)(\ensuremathτ){g}^{(2)}(\ensuremath{\tau})g(2)(\ensuremathτ) of the emitted light, and we find strong, unbounded bunching of the emission from systems governed by the Rabi Hamiltonian. Surprisingly, this effect is observed not only in the ultrastrong coupling regime, but also for weakly coupled systems, where the Jaynes-Cummings Hamiltonian would predict the opposite, antibunched emission. This suggests that the higher-order correlations are a particularly sensitive probe of the divergence between the Jaynes-Cummings and Rabi Hamiltonians, and they can serve as an indicator of the breakdown of the rotating wave approximation. Our findings indicate also that the boundary between the weakly, strongly, and ultra-strongly-coupled dynamics is much richer than currently accepted.
Abstract Ultrastrong-coupling between two-level systems and radiation is important for both fundamental and applied quantum electrodynamics (QED). Such regimes are identified by the breakdown of the rotating-wave approximation, which applied to the quantum Rabi model (QRM) yields the apparently less fundamental Jaynes-Cummings model (JCM). We show that when truncating the material system to two levels, each gauge gives a different description whose predictions vary significantly for ultrastrong-coupling. QRMs are obtained through specific gauge choices, but so too is a JCM without needing the rotating-wave approximation. Analysing a circuit QED setup, we find that this JCM provides more accurate predictions than the QRM for the ground state, and often for the first excited state as well. Thus, Jaynes-Cummings physics is not restricted to light-matter coupling below the ultrastrong limit. Among the many implications is that the system’s ground state is not necessarily highly entangled, which is usually considered a hallmark of ultrastrong-coupling.
Ultrastrong-coupling between two-level systems and radiation is important for both fundamental and applied quantum electrodynamics (QED). Such regimes are identified by the breakdown of the rotating-wave approximation, which applied to the quantum Rabi model (QRM) yields the apparently less fundamental Jaynes-Cummings model (JCM). We show that when truncating the material system to two levels, each gauge gives a different description whose predictions vary significantly for ultrastrong-coupling. QRMs are obtained through specific gauge choices, but so too is a JCM without needing the rotating-wave approximation. Analysing a circuit QED setup, we find that this JCM provides more accurate predictions than the QRM for the ground state, and often for the first excited state as well. Thus, Jaynes-Cummings physics is not restricted to light-matter coupling below the ultrastrong limit. Among the many implications is that the system's ground state is not necessarily highly entangled, which is usually considered a hallmark of ultrastrong-coupling.
Ultrastrong-coupling between an effective two-level system and radiation offers immense potential for advancing both fundamental and applied quantum electrodynamics (QED). Such regimes cannot be treated using the rotating-wave approximation, which applied to the quantum Rabi model yields the apparently less fundamental Jaynes-Cummings model. However, the implications of gauge-freedom for ultrastrong-coupling QED are yet to be recognised. Here we show that when truncating the material system to only two levels, each gauge gives a different effective description whose predictions can vary significantly for ultrastrong-coupling. Rabi models are obtained through specific gauge choices, but so too is a Jaynes-Cummings model without needing the rotating-wave approximation. Analysing a circuit QED setup, we find that this Jaynes-Cummings model is not only valid well beyond the rotating-wave approximation, it is often more accurate than the Rabi model. Among the many implications of this finding is that the system's ground state is not necessarily highly entangled, which is usually considered a hallmark of ultrastrong-coupling light-matter physics.
We present a circuit-QED scheme which makes it possible to reach the ultrastrong-coupling regime of a nondipolar interaction between a single qubit and a quantum resonator. We show that the system Hamiltonian is well approximated by a two-photon quantum Rabi model and propose a simple scattering experiment to probe its fundamental properties. In particular, we identify a driving scheme that reveals the change in selection rules characterizing the breakdown of the rotating-wave approximation and the transition from strong to ultrastrong two-photon interactions. Finally, we show that a frequency crowding in a narrow spectral region is observable in the output fluorescence spectrum as the coupling strength approaches the collapse point, paving the way to the direct observation of the onset of the spectral collapse in a solid-state device.
The dissipative quantum phase transitions experienced by a driven optical system are studied in order to understand the underlying light-matter coupling. The primary system under study is composed of a cavity mode coupled to a two-level system with dissipation being introduced through the interaction with a surrounding environment; an external coherent field is included to drive the system out of the ground state. The coupling is given by a generalized Rabi Hamiltonian, where rotating, gr, and counter-rotating, ngr, couplings are both present and can be adjusted independently. A comprehensive study of the different phases the system can exhibit as gr and n are varied is presented. From this, we construct a bridge between two limiting scenarios: (i) the Jaynes-Cummings limit (n = 0), where the system undergoes a phase transition by means of the breakdown of the photon blockade, and (ii) the driven Dicke limit ( = 1 ), where the normal to super-radiant phase transition is found. Novel behaviour encountered in an intermediate regime (1 > n > 0) is discussed. Attention is drawn towards the strong coupling regime, where changes at the one-photon level induce nonlinear effects and behaviour reminiscent of phase transitions is encountered with just a few photons present. A comparison between weak and strong coupling regimes, and, thus, an exploration of the effect of fluctuations over quantum phase transitions of light, is given through a survey of the phases an auxiliary optical system exhibits. This system is composed of two coupled nonlinear cavities that are driven coherently and damped through the interaction with the environment; it is seen to exhibit three phases. Two phases present high-correlation between the cavities and are differentiated by the photon statistics, transitioning from classical to quantum. The third phase is characterized by a highly localized field in one of the cavities. The departure from mean-field results is highlighted and a new way to characterize the possible phases of the system is proposed. Finally, the crucial role of quantum fluctuations is quantified and used to define the phases at hand.
The prototypical system constituted by a two-level atom interacting with a quantized single-mode electromagnetic field is described by the quantum Rabi model (QRM). The QRM is potentially valid at any light-matter interaction regime, ranging from the weak (where the decay rates exceeds the coupling rate) to the deep strong coupling (where the interaction rate exceeds the bare transition frequencies of the subsystems). However, when reaching the ultrastrong coupling regime, several theoretical issues may prevent the correct description of the observable dynamics of such a system: (i) the standard quantum optics master equation fails to correctly describe the interaction of this system with the reservoirs; (ii) the correct output photon rate is no longer proportional to the intracavity photon number; and (iii) they appear to violate gauge invariance. Here, we study the photon flux emission rate of this system under the incoherent excitation of the two-level atom for any light-matter interaction strength and consider different effective temperatures. The dependence of the emission spectra on the coupling strength is the result of the interplay between energy levels, matrix elements of the observables, and the density of states of the reservoirs. Within this approach, we also study the occurrence of light-matter decoupling in the deep strong-coupling regime and show how all of the obtained results are gauge invariant.