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arXiv:2210.10835 · Physical Review A

Pulse-area theorem in a single-mode waveguide and its application to photon echo and optical memory in Tm3+:Y3Al5O12

Sergey A. Moiseev, Mansur M. Minnegaliev, E. S. Moiseev, K. I. Gerasimov, A. V. Pavlov, Т.А. Рупасов, Nikolay N. Skryabin, Alexander A. Kalinkin, S. P. Kulik

Published Apr 20, 2023• 10 citations
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Abstract

We derive the area theorem for light pulses interacting with an inhomogeneously broadened ensemble of two-level atoms in a single-mode optical waveguide and present its analytical solution for Gaussian-type modes, which demonstrates the significant difference from the formation of $2\ensuremath{\pi}$ pulses by plane waves. We generalize this theorem to the description of photon echo and apply it to the two-pulse (primary) echo and the revival of silenced echo (ROSE) protocol of photon echo quantum memory. We implemented ROSE protocol in a single-mode laser-written waveguide made of an optically thin crystal ${\mathrm{Tm}}^{3+}$:${\mathrm{Y}}_{3}{\mathrm{Al}}_{5}{\mathrm{O}}_{12}$ . The experimental data obtained are satisfactorily explained by the developed theory. Finally, we discuss the obtained experimental results and possible applications of the derived pulse-area approach.

DOI
10.1103/physreva.107.043708

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The active use of resonators in quantum technologies increases the interest of their application in the creation of optical and microwave quantum memory. The use of photon and spin echoes opens up the possibility of storing a large number of light pulses in one such memory cell. High efficiency of such quantum memory is achieved in an optically dense resonant media, in which the formation of a photon (spin) echo can be accompanied by an increase in the nonlinear interaction of light with atoms causing the appearance of multiple echo signals. In this paper, we develop the pulse area approach to study general nonlinear properties of the primary and multi-pulse echo signals excited in a two-level atomic ensemble located in ring cavities with volumetric and surface modes. Conditions under which one or more echo pulses can be generated are analyzed. The solutions obtained are compared with recent experimental results. We show that the area theorem is one of the simplest and most powerful analytical tools for studying a highly nonlinear and dynamical process of the formation of the sequence of photon/spin echo signals in resonant media inside the resonator.
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We experimentally realize a quantum-memory protocol based on retrieval of silenced echo (ROSE) in Tm 3+ :Y 3 Al 5 O 12 crystal in an orthogonal geometry of the signal and control light fields. The silenced echo signal revival efficiency of ~13% with 36 μs storage time is demonstrated. To achieve that we implemented a high-precision atomic coherence control via amplitude- and phase-modulated laser pulses. We also discuss capabilities of this configuration, ways to increase quantum efficiency and to combine it with a single-mode optical cavity.
The protocol of optical quantum memory in the revival of silenced photon echo (ROSE) scheme is experimentally implemented in a Tm 3+ :Y 3 Al 5 O 12 crystal ( c = 0.1 at.%) placed in an impedance-matched optical Fabry–Perot resonator. The input signal recovery efficiency of ∼21 % is achieved for a light pulse with a storage time of 36 μs. The main sources of loss and their impact on the achieved quantum efficiency are discussed, as well as the advantages of the implemented scheme and the possibilities of the further improvement of the main parameters of quantum memory.