Interactions between a source of light and atoms are ubiquitous in nature. The study of them is interesting on the fundamental level as well as for applications. They are at the core of quantum information processing tasks and quantum thermodynamics protocols. However, even for a two-level atom interacting with a field in rotating wave approximation there exists no exact solution. This touches upon a basic problem in quantum field theory, where we can only calculate the transitions in the time asymptotic limits (i.e., minus and plus infinity), while we are not able to trace the evolution. In this paper we want to get more insight into the time evolution of a total system of a two-level atom and a continuous-mode quantum field. We propose an approximation, which we are able to apply systematically to each order of Dyson expansion, resulting in a greatly simplified formula for the evolution of the combined system at any time. Our tools include a proposed non-Hermitian renormalization method. As a sanity check, by applying our framework, we derive the known optical Bloch equations.
Interactions between a source of light and atoms are ubiquitous in nature. The study of them is interesting on the fundamental level as well as for applications. They are at the core of quantum information processing tasks and quantum thermodynamics protocols. However, even for a two-level atom interacting with a field in rotating wave approximation there exists no exact solution. This touches upon a basic problem in quantum field theory, where we can only calculate the transitions in the time asymptotic limits (i.e., minus and plus infinity), while we are not able to trace the evolution. In this paper we want to get more insight into the time evolution of a total system of a two-level atom and a continuous-mode quantum field. We propose an approximation, which we are able to apply systematically to each order of Dyson expansion, resulting in a greatly simplified formula for the evolution of the combined system at any time. Our tools include a proposed non-Hermitian renormalization method. As a sanity check, by applying our framework, we derive the known optical Bloch equations.
We introduce a non-Hermitian approximation of Bloch optical equations. This approximation provides a complete description of the excitation, relaxation, and decoherence dynamics of ensembles of coupled quantum systems in weak laser fields, taking into account collective effects and dephasing. In the proposed method, one propagates the wave function of the system instead of a complete density matrix. Relaxation and dephasing are taken into account via automatically adjusted time-dependent gain and decay rates. As an application, we compute the numerical wave packet solution of a time-dependent non-Hermitian Schrödinger equation describing the interaction of electromagnetic radiation with a quantum nano-structure, and compare the calculated transmission, reflection, and absorption spectra with those obtained from the numerical solution of the Liouville-von Neumann equation. It is shown that the proposed wave packet scheme is significantly faster than the propagation of the full density matrix while maintaining small error. We provide the key ingredients for easy-to-use implementation of the proposed scheme and identify the limits and error scaling of this approximation.
The dual Dyson series [M. Frasca, Phys. Rev. A 58 3439 (1998)] is used to develop a general perturbative method for the study of atom-field interaction in quantum optics. In fact, both the Dyson series and its dual, by renormalization-group methods to remove secular terms from the perturbation series, give the opportunity for a full study of the solution of the Schr\"odinger equation in different ranges of the parameters of the given Hamiltonian. In view of recent experiments with strong laser fields, this approach seems well-suited to give a clarification and an improvement of the applications of the dressed states as currently done through the eigenstates of the atom-field interaction, showing that these are just the leading order of the dual Dyson series when the Hamiltonian is expressed in the interaction picture. In order to best exploit the method, a study is accomplished of the well-known Jaynes-Cummings model in the rotating-wave approximation, whose exact solution is known, comparing the perturbative solutions obtained by the Dyson series and its dual with the same approximations obtained by Taylor expanding the exact solution. Finally, a full perturbative study of high-order harmonic generation is given, obtaining, through analytical expressions, a clear account of the power spectrum using a two-level model, even if the method can be successfully applied to a more general model that can account for ionization too. The analysis shows that to account for the power spectrum it is necessary to go to first order in the perturbative analysis. The spectrum obtained gives a way to measure experimentally the shift of the energy levels of the atom interacting with the laser field by looking at the shifting of hyper-Raman lines.
We introduce a non-Hermitian Schrödinger-type approximation of optical Bloch equations for two-level systems. This approximation provides a complete and accurate description of the coherence and decoherence dynamics in both weak and strong laser fields at the cost of losing accuracy in the description of populations. In this approach, it is sufficient to propagate the wave function of the quantum system instead of the density matrix, providing that relaxation and dephasing are taken into account via automatically adjusted time-dependent gain and decay rates. The developed formalism is applied to the problem of scattering and absorption of electromagnetic radiation by a thin layer comprised of interacting two-level emitters.
In this work we shall study the interaction of matter and light. In so doing we shall rely heavily on the description of such processes provided by quantum mechanics. This appears on a number of levels: firstly, a quantum description of matter is indispensable if one wants to understand on the microscopic scale the different kinds of interaction processes that can occur. Secondly, a quantum description of light often turns out to be useful, sometimes necessary, to better understand these processes. We shall study phenomena such as spontaneous emission, which can only be properly treated by a theory taking into account the quantum nature of both light and matter. In the following chapters we shall address, amongst others, the following question: ‘given an atom prepared at a given time in a particular state and subjected from this time onwards to electromagnetic radiation, what is the state of the atom and radiation at any later moment in time?’ In order to be able to answer this question it will be necessary for us to know how to calculate the evolution of a quantum system in a small number of typical situations. These methods we shall demonstrate in the first chapter. The evolution of the coupled atom–light system depends on the temporal dependence of the applied light field, which could, for example, be applied from a given moment and thereafter remain unchanged in intensity, or, perhaps, be appreciable only for a finite period of time (pulsed excitation).
We derive the stochastic equations and consider the non-Markovian dynamics of a system of multiple two-level atoms in a common quantum field. We make only the dipole approximation for the atoms and assume weak atom–field interactions. From these assumptions, we use a combination of non-secular open- and closed-system perturbation theory, and we abstain from any additional approximation schemes. These more accurate solutions are necessary to explore several regimes: in particular, near-resonance dynamics and low-temperature behavior. In detuned atomic systems, small variations in the system energy levels engender timescales which, in general, cannot be safely ignored, as would be the case in the rotating-wave approximation (RWA). More problematic are the second-order solutions, which, as has been recently pointed out (Fleming and Cummings 2011 Phys. Rev. E 83 031117), cannot be accurately calculated using any second-order perturbative master equation, such as RWA, Born–Markov, Redfield, etc. The latter problem, which applies to all perturbative open-system master equations, has a profound effect upon calculation of entanglement at low temperatures. We find that even at zero temperature all initial states will undergo finite-time disentanglement (sometimes termed ‘sudden death’), in contrast to the previous work. We also use our solution, without invoking the RWA, to characterize the necessary conditions for Dicke subradiance at finite temperature. We find that the sub-radiant states fall into two categories at finite temperature: one that is temperature independent and one that acquires temperature dependence. With the RWA, there is no temperature dependence in any case.
In this paper, the general optical Bloch equation describing interaction between intensive fields and two level system is obtained without using rotating wave approximation. The first-order solution of this equation is obtained by iterative method and analytic formulas of transition probability as a function of time, perturbation frequency and strength are presented. These results are in agreement with those obtained by an iterative step-wise power series and numerical integration solution for the time dependent Schr(?)dinger equation. And these simplified and clear mathmatical formulas facilitate the application of physics.