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arXiv:2210.06133

Rotational decoherence due to thermal photon scattering

Hamid Reza Naeij

Published Oct 12, 2022• 0 citations
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Abstract

The use of rotational degrees of freedom of quantum systems in quantum technologies is limited by environmental effects under decoherence mechanism. Here, we study the mechanism of decoherence based on a new formalism of elastic scattering for a nonspherical quantum system prepared in a superposition of rotational degrees of freedom. We show that for a dielectric ellipsoid immersed in an environment composed of thermal photons the rotational decoherence rate depends on the angular differences between the two configurations of the system and the seventh power of the temperature which is different from the translational one. Then we analyze the effect of different values of angular momentum quantum numbers of the environmental spherical harmonics on the rotational decoherence rate.

DOI
10.48550/arxiv.2210.06133

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The use of rotational degrees of freedom of quantum systems in quantum technologies is limited by environmental effects under decoherence mechanism. Here, we study the mechanism of decoherence based on a new formalism of elastic scattering for a nonspherical quantum system prepared in a superposition of rotational degrees of freedom. We show that for a dielectric ellipsoid immersed in an environment composed of thermal photons the rotational decoherence rate depends on the angular differences between the two configurations of the system and the seventh power of the temperature which is different from the translational one. Then we analyze the effect of different values of angular momentum quantum numbers of the environmental spherical harmonics on the rotational decoherence rate.
The mechanism of decoherence for a mesoscopic quantum system with rotational degrees of freedom is studied. From a simple model of elastic scattering, we show that the nondiagonal density-matrix elements of the system exponentially decay. The decay rate depends on the difference of scattering amplitudes for different rotational configurations, leading to the gradual loss of quantum coherence between the pointer states in the orientational space. For a dielectric ellipsoid immersed in a photon-gas environment (assuming no absorption), the decay rate is found to be proportional to the seventh power of the temperature. For an ellipsoidal object interacting with massive particles, the decay rate is proportional to the 5/2 power of the temperature. Both are different from the case of translational decoherence induced by the same environment scattering. For photon scattering, the coherence time in the rotational degrees of freedom is shown to be much shorter than that in the translational degrees of freedom.
Motivated by trapping and cooling experiments with nonspherical nanoparticles, we discuss how their combined rotational and translational quantum state is affected by the interaction with a gaseous environment. Based on the quantum master equation in terms of orientation-dependent scattering amplitudes, we evaluate the localization rate for gas collisions off an anisotropic van der Waals--type potential and for photon scattering off an anisotropic dielectric. We also show how pure angular momentum diffusion arises from these open quantum dynamics in the limit of weak anisotropies.
Recent advances in levitated optomechanics provide new perspectives for the use of rotational degrees of freedom for the development of quantum technologies as well as for testing fundamental physics. As for the translational case, their use, especially in the quantum regime, is limited by environmental noises, the characterization of which is fundamental in order to assess, control, and minimize their effect, in particular decoherence. Here, we present a general perturbative approach to compute decoherence for a quantum system in a superposition of its rotational degrees of freedom. The specific cases of the dipole-dipole and quadrupole-quadrupole interactions are solved explicitly, and we show that the rotational degrees of freedom decohere on a time scale that can be longer than the translational one.
We show how to describe the diffusion of the quantized angular momentum vector of an arbitrarily shaped rigid rotor as induced by its collisional interaction with an environment.We present the general form of the Lindblad-type master equation and relate it to the orientational decoherence of an asymmetric nanoparticle in the limit of small anisotropies.The corresponding diffusion coefficients are derived for gas particles scattering off large molecules and for ambient photons scattering off dielectric particles, using the elastic scattering amplitudes.
The effect induced by an environment on a composite quantum system is studied. The model considers the composite system as comprised by a subsystem A coupled to a subsystem B which is also coupled to an external environment. We studied all possible four combinations of subsystems A and B made up with a harmonic oscillator and an upside down oscillator. We analyzed the decoherence suffered by subsystem A due to an effective environment composed by subsystem B and the external reservoir. In all the cases we found that subsystem A decoheres even though it interacts with the environment only through its sole coupling to B. However, the effectiveness of the diffusion depends on the unstable nature of subsystem A and B. Therefore, the role of this degree of freedom in the effective environment is analyzed in detail. © World Scientific Publishing Company.
This paper presents a comprehensive model for quantum decoherence, grounded in the principles of quantum field theory (QFT) and statistical mechanics. The core argument is that traditional decoherence models often oversimplify the process, failing to adequately capture the intricate interactions arising from the quantum effects of the surrounding environment. This work introduces a framework that explicitly incorporates the scattering of quantum states by the environment, treated as a QFT system, and then analyzes the resultant impact using statistical mechanics. The model aims to provide a more accurate and nuanced understanding of decoherence, particularly in scenarios involving strong environmental interactions. Specifically, the model utilizes the formalism of quantum scattering theory to describe the interaction between a quantum system and its environment. The resulting dynamics are then analyzed using the framework of statistical mechanics, allowing for the calculation of decoherence rates as a function of environmental parameters such as temperature and density. The key contributions of this work include a detailed mathematical description of the decoherence process, a clear separation of the quantum and classical aspects of the problem, and a framework for extending the model to more complex systems. The model predicts that decoherence is not simply a loss of quantum information, but rather a fundamental process of state transformation driven by the statistical properties of the environment. This work offers a significant step forward in our ability to understand and potentially mitigate the effects of decoherence in quantum technologies.