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arXiv:2210.02322

Dichotomy of heavy and light pairs of holes in the $t-J$ model

Annabelle Bohrdt, Eugene Demler, Fabian Grusdt

Published Oct 5, 2022• 0 citations
arXivHTMLPDF

Abstract

A key step in unraveling the mysteries of materials exhibiting unconventional superconductivity is to understand the underlying pairing mechanism. While it is widely agreed upon that the pairing glue in many of these systems originates from antiferromagnetic spin correlations, a microscopic description of pairs of charge carriers remains lacking. Here we use state-of-the art numerical methods to probe the internal structure and dynamical properties of pairs of charge carriers in quantum antiferromagnets in four-legged cylinders. Exploiting the full momentum resolution in our simulations, we are able to distinguish two qualitatively different types of bound states: a highly mobile, meta-stable pair, which has a dispersion proportional to the hole hopping $t$, and a heavy pair, which can only move due to spin exchange processes and turns into a flat band in the Ising limit of the model. Understanding the pairing mechanism can on the one hand pave the way to boosting binding energies in related models, and on the other hand enable insights into the intricate competition of various phases of matter in strongly correlated electron systems.

DOI
10.3929/ethz-b-000646549

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Dichotomy of heavy and light pairs of holes in the t−Jt-Jt−J model
A key step in unraveling the mysteries of materials exhibiting unconventional superconductivity is to understand the underlying pairing mechanism. While it is widely agreed upon that the pairing glue in many of these systems originates from antiferromagnetic spin correlations, a microscopic description of pairs of charge carriers remains lacking. Here we use state-of-the art numerical methods to probe the internal structure and dynamical properties of pairs of charge carriers in quantum antiferromagnets in four-legged cylinders. Exploiting the full momentum resolution in our simulations, we are able to distinguish two qualitatively different types of bound states: a highly mobile, meta-stable pair, which has a dispersion proportional to the hole hopping ttt, and a heavy pair, which can only move due to spin exchange processes and turns into a flat band in the Ising limit of the model. Understanding the pairing mechanism can on the one hand pave the way to boosting binding energies in related models, and on the other hand enable insights into the intricate competition of various phases of matter in strongly correlated electron systems.
A key step in unraveling the mysteries of materials exhibiting unconventional superconductivity is to understand the underlying pairing mechanism. While it is widely agreed upon that the pairing glue in many of these systems originates from antiferromagnetic spin correlations, a microscopic description of pairs of charge carriers remains lacking. Here we use state-of-the art numerical methods to probe the internal structure and dynamical properties of pairs of charge carriers in quantum antiferromagnets in four-legged cylinders. Exploiting the full momentum resolution in our simulations, we are able to distinguish two qualitatively different types of bound states: a highly mobile, meta-stable pair, which has a dispersion proportional to the hole hopping t, and a heavy pair, which can only move due to spin exchange processes and turns into a flat band in the Ising limit of the model. Understanding the pairing mechanism can on the one hand pave the way to boosting binding energies in related models, and on the other hand enable insights into the intricate competition of various phases of matter in strongly correlated electron systems.
In strongly correlated quantum materials, the behavior of charge carriers is dominated by strong electron-electron interactions. These can lead to insulating states with spin order, and upon doping to competing ordered states including unconventional superconductivity. The underlying pairing mechanism remains poorly understood however, even in strongly simplified theoretical models. Recent advances in quantum simulation allow to study pairing in paradigmatic settings, e.g. in the t-J t − J and t-J_z t − J z Hamiltonians. Even there, the most basic properties of paired states of only two dopants, such as their dispersion relation and excitation spectra, remain poorly studied in many cases. Here we provide new analytical insights into a possible string-based pairing mechanism of mobile holes in an antiferromagnet. We analyze an effective model of partons connected by a confining string and calculate the spectral properties of bound states. Our model is equally relevant for understanding Hubbard-Mott excitons consisting of a bound doublon-hole pair or confined states of dynamical matter in lattice gauge theories, which motivates our study of different parton statistics. Although an accurate semi-analytic estimation of binding energies is challenging, our theory provides a detailed understanding of the internal structure of pairs. For example, in a range of settings we predict heavy states of immobile pairs with flat-band dispersions - including for the lowest-energy d d -wave pair of fermions. Our findings shed new light on the long-standing question about the origin of pairing and competing orders in high-temperature superconductors.
Understanding pairing in the strong-coupling regime of doped Mott insulators remains an open problem in the context of cuprate superconductors. We perform ultra-high resolution numerical simulations of spectral functions in the highly underdoped t−Jt-Jt−J model and discover two coupled branches of hole pairs emerging at low energies in the largely unexplored two-particle spectrum. As spin anisotropy is tuned from the Ising limit to the SU(2)SU(2)SU(2)-symmetric Heisenberg regime, the lowest ddd-wave pair evolves from a single bipolaronic branch into two hybridized branches separated by an avoided crossing. We explain this behaviour using an effective two-channel model involving a tightly bound bipolaronic state and a second channel associated with two magnetic polarons. The model reproduces the qualitative low-energy spectra and implies near-resonant ddd-wave interactions in the SU(2)SU(2)SU(2)-symmetric t−Jt-Jt−J model, consistent with proximity to an emergent Feshbach-type resonance. To probe these predictions experimentally, we propose a Raman spectroscopy scheme for the attractive Hubbard model that can be directly implemented using ultracold atoms in optical lattices. Our work establishes two-particle spectroscopy, beyond single-particle Green's functions, as a powerful tool for revealing the microscopic origins of unconventional superconductivity.
Abstract Conventional superconductivity emerges from pairing of charge carriers—electrons or holes—mediated by phonons 1 . In many unconventional superconductors, the pairing mechanism is conjectured to be mediated by magnetic correlations 2 , as captured by models of mobile charges in doped antiferromagnets 3 . However, a precise understanding of the underlying mechanism in real materials is still lacking and has been driving experimental and theoretical research for the past 40 years. Early theoretical studies predicted magnetic-mediated pairing of dopants in ladder systems 4–8 , in which idealized theoretical toy models explained how pairing can emerge despite repulsive interactions 9 . Here we experimentally observe this long-standing theoretical prediction, reporting hole pairing due to magnetic correlations in a quantum gas of ultracold atoms. By engineering doped antiferromagnetic ladders with mixed-dimensional couplings 10 , we suppress Pauli blocking of holes at short length scales. This results in a marked increase in binding energy and decrease in pair size, enabling us to observe pairs of holes predominantly occupying the same rung of the ladder. We find a hole–hole binding energy of the order of the superexchange energy and, upon increased doping, we observe spatial structures in the pair distribution, indicating repulsion between bound hole pairs. By engineering a configuration in which binding is strongly enhanced, we delineate a strategy to increase the critical temperature for superconductivity.
Understanding the physics of the two-dimensional Hubbard model is widely believed to be a key step in achieving a full understanding of high- T c cuprate superconductors. In recent years, progress has been made by large-scale numerical simulations at finite doping and, on the other hand, by microscopic theories able to capture the physics of individual charge carriers. In this work, we study single pairs of dopants in a cylindrical system using the density-matrix renormalization group algorithm. We identify two coexisting charge configurations that couple to the spin environment in different ways: a tightly bound configuration featuring (next-)nearest-neighbor pairs and a stripelike configuration of dopants on opposite sides of the cylinder, accompanied by a spin domain wall. Thus, we establish that the interplay between stripe order and uniform pairing, central to the models’ phases at finite doping, has its origin at the single-pair level. By interpolating between the Hubbard and the related t − J model, we are able to quantitatively understand discrepancies in the pairing properties of the two models through the three-site hopping term usually omitted from the t − J Hamiltonian. This term is closely related to a next-nearest-neighbor tunneling t ′ , which we observe to upset the balance between the competing stripe and pair states on the two-dopant level.
A single-hole ground state Ansatz for the two-dimensional t-J model has been recently studied by the variational Monte Carlo (VMC) method.Such a doped hole behaves like a "twisted" non-Landau quasiparticle characterized by an emergent quantum number in agreement with exact numerics.In this work, we further investigate the ground state of two holes by VMC.It is found that the two holes strongly attract each other to form a pairing state with a new quantum number the same as obtained by the numerical exact diagonalization and density matrix renormalization group (DMRG) calculations.A unique feature of this pairing state is a dichotomy in the pairing symmetry, i.e., a d wave in terms of the electron c operators and an s wave in terms of the new quasiparticles, as explicitly illustrated in the ground state wave function.A similar VMC study of a two-hole wave function for the t-J two-leg ladder also yields a good agreement with the DMRG result.We demonstrate that the pairing mechanism responsible for the strong binding here is not due to the long-range antiferromagnetic order nor the resonating-valence-bound pairing in the spin background but is the consequence of the quantum phase strings created by the hopping of holes.The resulting spin-current pattern mediating the pairing force is explicitly illustrated in the VMC calculation.Physical implications to superconductivity at finite doping are also discussed.