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arXiv:2209.10678 · APL Photonics

Spectrally shaped and pulse-by-pulse multiplexed multimode squeezed states of light

Tiphaine Kouadou, Francesca Sansavini, Matthieu Ansquer, Johan Henaff, Nicolas Treps, Valentina Parigi

Published Aug 1, 2023• 36 citations
arXivHTMLPDF

Abstract

Spectral- and time-multiplexing are currently explored to generate large multipartite quantum states of light for quantum technologies. In the continuous variable approach, the deterministic generation of scalable entangled states requires the generation of a scalable number of squeezed modes. Here, we demonstrate the simultaneous generation of 21 squeezed spectral modes at the repetition rate of our laser, i.e., 156 MHz. We exploit the full repetition rate and the pulse shaping of a femtosecond light source to combine, for the first time, frequency- and time-multiplexing in multimode squeezing. This paves the way for the implementation of multipartite entangled states that are both scalable and fully reconfigurable.

DOI
10.1063/5.0156331

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Spectral- and time-multiplexing are currently explored to generate large multipartite quantum states of light for quantum technologies. In the continuous variable approach, the deterministic generation of scalable entangled states requires the generation of a scalable number of squeezed modes. Here, we demonstrate the simultaneous generation of 21 squeezed spectral modes at the repetition rate of our laser, i.e., 156 MHz. We exploit the full repetition rate and the pulse shaping of a femtosecond light source to combine, for the first time, frequency- and time-multiplexing in multimode squeezing. This paves the way for the implementation of multipartite entangled states that are both scalable and fully reconfigurable.
Continuous variable encoding of quantum information requires the deterministic generation of highly correlated quantum states of light in the form of quantum networks, which, in turn, necessitates the controlled generation of a large number of squeezed modes. In this paper, we present an experimental source of multimode squeezed states of light at telecommunication wavelengths. Generation at such wavelengths is especially important as it can enable quantum information processing, communication, and sensing beyond the laboratory scale. We use a single-pass spontaneous parametric down-conversion process in a nonlinear waveguide pumped with the second harmonic of a femtosecond laser. Our measurements reveal significant squeezing in more than 21 frequency modes, with a maximum squeezing value exceeding 2.5 dB. We demonstrate multiparty entanglement by measuring the state's covariance matrix. Finally, we show the source reconfigurability by preparing few-node cluster states and measure their nullifier squeezing level. These results pave the way for a scalable implementation of continuous variable quantum information protocols at telecommunication wavelengths, particularly for multiparty, entanglement-based quantum communications. Moreover, the source is compatible with additional pulse-by-pulse multiplexing, which can be utilized to construct the necessary three-dimensional entangled structures for quantum computing protocols. Published by the American Physical Society 2024
Cluster states, in which entanglement is distributed amongst numerous parties, have attracted interest due to their role as a resource for measurement-based quantum computing. The traditional means for fabricating these highly-entangled states has been to sequentially combine the squeezed outputs from individual optical parametric oscillators (OPO) with a network of phase-shifters and beamsplitters. While successful, this approach demands an optical footprint commensurate with the dimensionality of the produced state. Within the continuous-variable regime, a promising alternative is to begin with a source that is intrinsically multimode. Toward that end, the frequency comb underlying femtosecond optical pulses contains upwards of ~ 105individual frequencies, which makes it an attractive starting point for the production of multipartite entanglement. This work demonstrates the ability of OPOs synchronously pumped by a femtosecond pulse train to create scalable, adaptable multipartite photonic states in a single beam while exploiting femtosecond pulse shaping to perform a complete state analysis.
Quantum optics has been, from its beginning, a driving force both for the exploration of fundamental limits of the quantum world and for conceiving seminal ideas and applications of the so-called quantum technologies. The last 20 years have seen a rapid development of ideas and proof-of-principle experiments involving the fields of quantum communication, quantum computation, quantum metrology and quantum simulation. The so called continuous variable (CV) approach to quantum optics, which uses many photon in collective states, and continuous observables like the quadratures of the electric field to encode information, has many interesting properties, especially from a communications perspective. It is inherently broadband and compatible with standard telecom infrastructures. Moreover, in CV, entanglement, one of the fundamental resource of quantum optics, can be generated deterministically. One of the main challenges for all quantum information technologies is scalability, being able to generate and manipulate a large number of quantum resources to achieve practical tasks efficiently. One approach to solve the issue of scalability is to use highly multimode quantum states. The quantum description of the electromagnetic field associate each photon (particle of light) with a mode (way for light to propagate). In a mutlimodal approach, we look at the quantum state bases and optical modes bases conjointly and tailor quantum fields not only in given modes, but also optimize the spatio-temporal shapes of the modes in which the state is defined. This opens wide perspectives for treating complex quantum states. In particular, using ultra-fast pulses of light which contain many temporal/spectral modes, we are able to generate large and complex entangled states of light using simple resources. In this thesis, we used an optical parametric oscillator pumped synchronously (SPOPO) with a frequency comb to generate multimode squeezed vacuum states which can be used to form cluster states: a large collection of modes (the nodes) entangled to each other in a certain way. These state are the basic resource for Measurement Based Quantum Computation (MBQC). This set-up has the advantage to generate entanglement in many mode with a single device. It is also highly tunable. Indeed, by tuning the spectrum of the OPO pump with a pulse shaper, one can tailor the properties of the generated quantum state. In this work, we focus on the optimization of the pump spectral shape to generate specific states. Using simulations based on Machine Learning Algorithms (MLA), we find optimal pump profile for typical target states. We then implement those shapes on the experimental set-up and measure the resulting states using multipixel homodyne detection. We also study intra-cavity dispersion effects. Dispersion inside the SPOPO cavity is indeed one of the main factor that limits the number of entangled modes in the generated quantum states. A systematic study of dispersion effects is therefore necessary to model the SPOPO output accurately. This works paves the way toward a fully tunable device that can be optimized in real time to generate specific quantum resources tailored for specific tasks.
Nowadays, the realization of quantum computations and communications based on continuous variables has attracted a significant attention due to a substantial expansion of the system dimensionality. The main progress in this area is attributed to the implementation of multimode systems based on squeezed states of light. One of the simplest ways to generate such states relies upon their producing in a single-pass optical parametric amplifier (OPA) using ultrafast pumping. However, for homodyne detection of such multimode states, the profile of the local oscillator (LO) must perfectly match the profile of the measured mode. Usually, this is not the case; therefore a proper treatment of multimode squeezing is required. In this work, we study both theoretically and experimentally the multimode squeezed light generated in type-0 and type-II OPA. We characterize such sources and investigate the degree of squeezing in dependence on the LO spectral profile, employing a pulse shaping technique. The theoretical analysis is performed using the Schmidt-mode theory. This work might have a significant impact on the realization of multimode quantum protocols
Continuous-variable quantum networks constitute a valuable resource for a wide range of quantum communication and information protocols. While frequency- and fast time-multiplexing enable the implementation of scalable quantum architectures, a precise characterization of multimode squeezed-light sources is essential. In this work, we increase both the spectral resolution and the measured squeezing values. Both parameters are relevant for the improved generation of so-called cluster states, a key resource for measurement-based quantum computing. Our source is based on parametric down-conversion in a periodically poled KTP waveguide pumped by a pulsed laser. The source produces squeezed states over a specific set of optical spectra. Increased spectral resolution in spectrally resolved homodyne detection allowed us to enhance the squeezing per spectral mode, increasing it from 1 dB to more than 2.4 dB in the first mode when measuring with a homodyne detector with a bandwidth of a few MHz. Secondly, we implemented a pulse-by-pulse characterization of the resource using a fast homodyne detector with an electronic bandwidth on the order of the laser repetition rate (100 MHz). Using this approach, the fast measurements revealed squeezing values of up to 1.5 dB in the first few spectral modes. To fully access the multimode quantum resource and ultimately improve the amount of squeezing, a high quantum efficiency is required. To avoid limitations imposed by poor spatial mode matching between the quantum resource and the local oscillator in homodyne detection, we implemented a wavefront-shaping scheme to characterize and control both the intensity profile and phase of the local oscillator. In preliminary tests this approach increased the mode-matching between the reference beam and the quantum signal by more than 8% while simultaneously providing a detailed characterization of the beam shape and of the influence of waveguide transmission on the beam profile. To achieve a genuine advantage in quantum information processing over classical protocols, the generation of non-Gaussian states is necessary. We therefore present a complete scheme for the creation of non-Gaussian states in a multimode system via mode-selective single-photon addition and subtraction, implemented through nonlinear optical processes in second-order nonlinear materials. We introduce a simulation framework applied to our squeezing source, which can be adapted to other regimes as well. Based on this framework, we are able to predict specific waveguide configurations that enable full control over the generated quantum states while maintaining high purity, with each process exhibiting a Schmidt number close to K=1, corresponding to effective single-mode addressing. generated quantum states while maintaining high purity, with each process exhibiting a Schmidt number close to K=1, corresponding to effective single-mode addressing.