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arXiv:2209.09853 · Physical review. B./Physical review. B

Detecting symmetry fractionalization in gapped quantum spin liquids by magnetic impurities

Shuangyuan Lu, Yuan-Ming Lu

Published Sep 3, 2024• 2 citations
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Abstract

Abstract We study the Kondo effect of spin-1/2 magnetic impurities in gapped Z2 spin liquids on two-dimensional lattices. We find that if the impurity is placed at a high-symmetry location, a nontrivial spinon fractionalization class of the impurity site symmetry group will necessarily lead to a non-Kramers doublet in the Kondo screening regime, protected by associated crystalline symmetries. This is in sharp contrast to a featureless screening phase in the usual Kondo effect. We demonstrate this symmetry-protected topological degeneracy by an exactly solvable model and by the large-N theory. Based on this effect, we discuss how thermodynamic measurements in the limit of dilute magnetic impurities can be used to detect symmetry fractionalization in gapped Z2 spin liquids.

DOI
10.1103/physrevb.110.l100401

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Abstract We study the Kondo effect of spin-1/2 magnetic impurities in gapped Z2 spin liquids on two-dimensional lattices. We find that if the impurity is placed at a high-symmetry location, a nontrivial spinon fractionalization class of the impurity site symmetry group will necessarily lead to a non-Kramers doublet in the Kondo screening regime, protected by associated crystalline symmetries. This is in sharp contrast to a featureless screening phase in the usual Kondo effect. We demonstrate this symmetry-protected topological degeneracy by an exactly solvable model and by the large-N theory. Based on this effect, we discuss how thermodynamic measurements in the limit of dilute magnetic impurities can be used to detect symmetry fractionalization in gapped Z2 spin liquids.
Despite rapid progress in understanding gapped topological states, much less is known about gapless topological phases of matter, especially in strongly correlated electrons. In this work, we discuss a large class of robust gapless quantum spin liquids in frustrated magnets made of half-integer spins, which are described by gapless fermionic spinons coupled to dynamical Z2{\mathbb{Z}}_{2}Z2​ gauge fields. Requiring U(1)\text{U}(1)U(1) spin conservation, time-reversal, and certain space-group symmetries, we show that certain spinon symmetry fractionalization class necessarily leads to a gapless spectrum. These gapless excitations are stable against any perturbations, as long as the required symmetries are preserved. Applying these gapless criteria to spin-12\frac{1}{2}21​ systems on square, triangular, and kagome lattices, we show that all gapped symmetric Z2{\mathbb{Z}}_{2}Z2​ spin liquids in Abrikosov-fermion representation can also be realized in Schwinger-boson representation. This leads to 64 gapped Z2{\mathbb{Z}}_{2}Z2​ spin liquids on square lattice, and 8 gapped states on both kagome and triangular lattices.
In this thesis, we study the topological phases of quantum spin systems. One project is to investigate a class of anti-ferromagnetic SU(N) Heisenberg models, describing Mott insulators of fermionic ultra-cold alkaline earth atoms on the three-dimensional simple cubic lattice. Our large-N analysis maps a rich phase diagram. One particularly striking state we found spontaneously breaks lattice rotation symmetry, where the cubic lattice breaks up into bilayers, each of which forms a two-dimensional chiral spin liquid state. In the other projects, we study the phenomenon of symmetry fractionalization on anyons as a tool to characterize two-dimensional symmetry enriched topological phases. In particular, we focus on how crystalline symmetries may fractionalize in gapped Z2 spin liquids. If the system has the symmetry of the square lattice, then there are 2080 symmetry fractionalization patterns possible. With exactly solvable models, we realize 487 of these in strictly two-dimensional systems. In addition, we succeed to understand why the remaining patterns cannot be found in the family of models we construct. Some can only appear on the surface of three-dimensional systems with non-trivial point group symmetry protected topological (pgSPT) order, whose boundary degrees of freedom transform non-locally under the symmetries. We construct a simple toy model to show this anomalous crystalline symmetry fractionalization phenomenon associated with a reflection. Moreover, our approach establishes the connection between the pgSPT phases and the topological phases with on-site symmetries in lower dimensions. This insight is very useful for classification of pgSPT orders in general.
We classify distinct types of quantum number fractionalization occurring in two-dimensional topologically ordered phases, focusing in particular on phases with Z2{\mathbb{Z}}_{2}Z2​ topological order, that is, on gapped Z2{\mathbb{Z}}_{2}Z2​ spin liquids. We find that the fractionalization class of each anyon is an equivalence class of projective representations of the symmetry group, corresponding to elements of the cohomology group H2(G,Z2){H}^{2}(G,{\mathbb{Z}}_{2})H2(G,Z2​). This result leads us to a symmetry classification of gapped Z2{\mathbb{Z}}_{2}Z2​ spin liquids, such that two phases in different symmetry classes cannot be connected without breaking symmetry or crossing a phase transition. Symmetry classes are defined by specifying a fractionalization class for each type of anyon. The fusion rules of anyons play a crucial role in determining the symmetry classes. For translation and internal symmetries, braiding statistics plays no role, but can affect the classification when point group symmetries are present. For square lattice space group, time-reversal, and SO(3)\mathrm{SO}(3)SO(3) spin rotation symmetries, we find $2\phantom{\rule{0.16em}{0ex}}098\phantom{\rule{0.16em}{0ex}}176\ensuremath{\approx}{2}^{21}$ distinct symmetry classes. Our symmetry classification is not complete, as we exclude, by assumption, permutation of the different types of anyons by symmetry operations. We give an explicit construction of symmetry classes for square lattice space group symmetry in the toric code model. Via simple examples, we illustrate how information about fractionalization classes can, in principle, be obtained from the spectrum and quantum numbers of excited states. Moreover, the symmetry class can be partially determined from the quantum numbers of the four degenerate ground states on the torus. We also extend our results to arbitrary Abelian topological orders (limited, though, to translations and internal symmetries), and compare our classification with the related projective symmetry group classification of parton mean-field theories. Our results provide a framework for understanding and probing the sharp distinctions among symmetric Z2{\mathbb{Z}}_{2}Z2​ spin liquids and are a first step toward a full classification of symmetric topologically ordered phases.
Using a one-dimensional spin-orbital model as a typical example of quantum spin systems with richer symmetries, we study the effect of an isolated impurity on its low-energy dynamics in the gapless phase through bosonization and renormalization-group methods. In the case of internal impurities, depending on the symmetry, the boundary fixed points can be either an open chain with a residual spin or (and) orbital triplet left behind, or a periodic chain. However, these two fixed points are indistinguishable in the sense that in both cases, the lead-correction-to-scaling boundary operators (LCBO) only show Fermi-liquid-like corrections to thermodynamical quantities (except the possible Curie-like contributions from the residual moments in the former cases). In the case of external (Kondo) impurities, the boundary fixed points, depending on the sign of orbital couplings, can be either an open chain with an isolated orbital doublet due to Kondo screening or an intermediate fixed point with the same LCBO as that of the two-channel Kondo problem. Comparison with the Kondo effect in one-dimensional Heisenberg spin chain and multiband Hubbard models is also made.
We consider gapped Z2{\mathbb{Z}}_{2}Z2​ spin liquids, where spinon quasiparticles may carry fractional quantum numbers of space-group symmetry. In particular, spinons can carry fractional crystal momentum. We show that such quantum number fractionalization has dramatic, spectroscopically accessible consequences, namely, enhanced periodicity of the two-spinon density of states in the Brillouin zone, which can be detected via inelastic neutron scattering. This effect is a sharp signature of certain topologically ordered spin liquids and other symmetry-enriched topological phases. Considering square lattice space-group and time-reversal symmetry, we show that exactly four distinct types of spectral periodicity are possible.
Paramagnetic impurities in a quantum spin liquid give rise to Kondo effects with highly unusual properties. We have studied the effect of locally coupling a paramagnetic impurity with the spin-12\frac{1}{2}21​ honeycomb Kitaev model in its gapless spin-liquid phase. The (impurity) scaling equations are found to be insensitive to the sign of the coupling. The weak and strong coupling fixed points are stable, with the latter corresponding to a noninteracting vacancy and an interacting, spin-1 defect for the antiferromagnetic and ferromagnetic cases, respectively. The ground state in the strong coupling limit in both cases has a nontrivial topology associated with a finite Z2{Z}_{2}Z2​ flux at the impurity site. For the antiferromagnetic case, this result has been obtained straightforwardly owing to the integrability of the Kitaev model with a vacancy. The strong-coupling limit of the ferromagnetic case is, however, nonintegrable, and we address this problem through exact-diagonalization calculations with finite Kitaev fragments. Our exact diagonalization calculations indicate that the weak-to-strong coupling transition and the topological phase transition occur rather close to each other and are possibly coincident. We also find an intriguing similarity between the magnetic response of the defect and the impurity susceptibility in the two-channel Kondo problem.