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arXiv:2209.06817 · Proceedings of the National Academy of Sciences

Diamagnetic response and phase stiffness for interacting isolated narrow bands

Dan Mao, Debanjan Chowdhury

Published Mar 10, 2023• 29 citations
arXivHTMLPDF

Abstract

Superconductivity is a macroscopic manifestation of a quantum phenomenon where pairs of electrons delocalize and develop phase coherence over a long distance. A long-standing quest has been to address the underlying microscopic mechanisms that fundamentally limit the superconducting transition temperature, T c . A platform which serves as an ideal playground for realizing “high”-temperature superconductors are materials where the electrons’ kinetic energy is quenched and interactions provide the only energy scale in the problem. However, when the noninteracting bandwidth for a set of isolated bands is small compared to the interactions, the problem is inherently nonperturbative. In two spatial dimensions, T c is controlled by superconducting phase stiffness. Here, we present a theoretical framework for computing the electromagnetic response for generic model Hamiltonians, which controls the maximum possible superconducting phase stiffness and thereby T c , without resorting to any mean-field approximation. Our explicit computations demonstrate that the contribution to the phase stiffness arises from i) “integrating out” the remote bands that couple to the microscopic current operator and ii) the density–density interactions projected on to the isolated narrow bands. Our framework can be used to obtain an upper bound on the phase stiffness and relatedly T c for a range of physically inspired models involving both topological and nontopological narrow bands with density–density interactions. We discuss a number of salient aspects of this formalism by applying it to a specific model of interacting flat bands and compare the upper bound against the known T c from independent numerically exact computations.

DOI
10.1073/pnas.2217816120

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Superconductivity is a macroscopic manifestation of a quantum phenomenon where pairs of electrons delocalize and develop phase coherence over a long distance. A long-standing quest has been to address the underlying microscopic mechanisms that fundamentally limit the superconducting transition temperature, T c . A platform which serves as an ideal playground for realizing “high”-temperature superconductors are materials where the electrons’ kinetic energy is quenched and interactions provide the only energy scale in the problem. However, when the noninteracting bandwidth for a set of isolated bands is small compared to the interactions, the problem is inherently nonperturbative. In two spatial dimensions, T c is controlled by superconducting phase stiffness. Here, we present a theoretical framework for computing the electromagnetic response for generic model Hamiltonians, which controls the maximum possible superconducting phase stiffness and thereby T c , without resorting to any mean-field approximation. Our explicit computations demonstrate that the contribution to the phase stiffness arises from i) “integrating out” the remote bands that couple to the microscopic current operator and ii) the density–density interactions projected on to the isolated narrow bands. Our framework can be used to obtain an upper bound on the phase stiffness and relatedly T c for a range of physically inspired models involving both topological and nontopological narrow bands with density–density interactions. We discuss a number of salient aspects of this formalism by applying it to a specific model of interacting flat bands and compare the upper bound against the known T c from independent numerically exact computations.
This work develops a systematic theoretical framework to determine the low-energy effective ``diamagnetic'' response associated with superconductivity and excitonic superfluidity in strongly interacting electronic models hosting isolated nearly flat bands. The results can be used to derive upper bounds on the transition temperatures for superconductivity and excitonic superfluidity without making any mean-field type approximations. The same theoretical framework can also be extended with very few modifications, to address questions related to ferromagnetism in flat bands and magnetic circular dichroism.
I summarize recent progress on obtaining rigorous upper bounds on superconducting transition temperature [Formula: see text] in two dimensions independent of pairing mechanism or interaction strength. These results are derived by finding a general upper bound for the superfluid stiffness for a multi-band system with arbitrary interactions, with the only assumption that the external vector potential couples to the kinetic energy and not to the interactions. This bound is then combined with the universal relation between the superfluid stiffness and the Berezinskii–Kosterlitz–Thouless [Formula: see text] in 2D. For parabolic dispersion, one obtains the simple result that [Formula: see text], which has been tested in recent experiments. More generally, the bounds are expressed in terms of the optical spectral weight and lead to stringent constraints for the [Formula: see text] of low-density, strongly correlated superconductors. Results for [Formula: see text] bounds for models of flat-band superconductors, where the kinetic energy vanishes and the vector potential must couple to interactions, are briefly summarized. Upper bounds on [Formula: see text] in 3D remains an open problem, and I describe how questions of universality underlie the challenges in 3D.
Understanding the material parameters that control the superconducting transition temperature T c is a problem of fundamental importance.In many novel superconductors phase fluctuations determine T c , rather than the collapse of the pairing amplitude.We derive rigorous upper bounds on the superfluid phase stiffness for multiband systems, valid in any dimension.This in turn leads to an upper bound on T c in two dimensions, which holds irrespective of pairing mechanism, interaction strength, or order-parameter symmetry.Our bound is particularly useful for the strongly correlated regime of low-density and narrowband systems, where mean-field theory fails.For a simple parabolic band in 2D with Fermi energy E F , we find that k B T c ≤ E F =8, an exact result that has direct implications for the 2D BCS-BEC crossover in ultracold Fermi gases.Applying our multiband bound to magic-angle twisted bilayer graphene, we find that band structure results constrain the maximum T c to be close to the experimentally observed value.Finally, we discuss the question of deriving rigorous upper bounds on T c in 3D.
Current theories of high-temperature superconductivity in flat-band systems predict a linear dependence of the transition temperature on the attractive interaction, Tc(U)=c∣U∣T_c(U) = c|U|Tc​(U)=c∣U∣. However, the value of ccc and the full nonlinear Tc(U)T_c(U)Tc​(U) curve---with a maximum at large ∣U∣|U|∣U∣---are known beyond mean-field and quantum geometry estimates only for systems with isolated flat bands. Using a controlled diagrammatic Monte Carlo technique, we trace the onset of superfluid response in the Lieb lattice with attractive Hubbard interaction. Focusing on the half-filled flat-band case, where the ordering mechanism differs fundamentally from both BCS and BEC (preformed Cooper pair) scenarios, we find that the pairing response diverges linearly with decreasing temperature over a broad range of UUU, leading to a sharp crossover to long-range correlations at a characteristic temperature T∗T_*T∗​, which provides a controlled upper bound on TcT_cTc​. The highest T∗T_*T∗​ occurs when all three bands touch at a single momentum point, potentially corresponding to high TcT_cTc​ values.
The superfluid stiffness fundamentally constrains the transition temperature of superconductors, especially in the strongly coupled regime. However, accurately determining this inherently quantum many-body property in microscopic models remains a significant challenge. In this Letter, we show how the quantum many-body bootstrap framework, specifically the reduced density matrix (RDM) bootstrap, can be leveraged to obtain rigorous lower bounds on the superfluid stiffness in frustration free interacting models with superconducting ground state. We numerically apply the method to a special class of frustration-free models, which are known as quantum geometric nesting models, for flatband superconductivity, where we uncover a general relation between the stiffness and the pair mass. Going beyond the familiar Hubbard case within this class, we find how additional interactions, notably simple magnetic couplings, can enhance the superfluid stiffness. Straightforward generalization of the method can lead to bounds on susceptibilities complementary to variational approaches. Our findings underscore the immense potential of the quantum many-body bootstrap as a powerful tool to derive rigorous bounds on physical quantities beyond energy.
We study the phase diagram of the Hubbard model in the limit where UUU, the onsite repulsive interaction, is much smaller than the bandwidth. We present an asymptotically exact expression for Tc{T}_{c}Tc​, the superconducting transition temperature, in terms of the correlation functions of the noninteracting system which is valid for arbitrary densities so long as the interactions are sufficiently small. Our strategy for computing Tc{T}_{c}Tc​ involves first integrating out all degrees of freedom having energy higher than an unphysical initial cutoff ${\ensuremath{\Omega}}_{0}$. Then, the renormalization group (RG) flows of the resulting effective action are computed and Tc{T}_{c}Tc​ is obtained by determining the scale below which the RG flows in the Cooper channel diverge. We prove that Tc{T}_{c}Tc​ is independent of ${\ensuremath{\Omega}}_{0}$. Using this method, we find a variety of unconventional superconducting ground states in two- and three-dimensional lattice systems, and present explicit results for Tc{T}_{c}Tc​ and pairing symmetries as a function of the electron concentration.