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arXiv:2209.01913

Spectral Properties of Transverse Laguerre-Gauss Modes in Parametric Down-Conversion

Carlos Sevilla-Gutiérrez, Varun Raj Kaipalath, Baghdasar Baghdasaryan, Markus Gräfe, S. Fritzsche, Fabian Steinlechner

Published Sep 5, 2022• 2 citations
arXivHTMLPDF

Abstract

The first color photos of the parametric down-conversion (PDC) emission cone illustrate the correlation of longitudinal- and transverse momentum in the process, i.e., wavelength-dependent emission angle of PDC photons. However, current experiments and applications are more conveniently described in terms of discrete mode sets, with the most suitable choice depending on the propagation symmetries of the experimental setting. Remarkably, despite the fact that experiments with PDC sources are becoming ever more demanding, e.g. in terms of brightness or state fidelity, a description of spectral-spatial coupling in parametric downconversion for the case of discrete modal decompositions remains elusive. We present a comprehensive study, in theory and experiment, of the spectral dependence of the transverse Laguerre-Gauss modes in parametric downconversion. Moreover, we show how the spectral and spatial coupling can be harnessed to tune the purity of the well-known orbital angular momentum entanglement. This work has implications for efficient collection of entangled photons in a transverse single mode, quantum imaging, and engineering pure states for high-dimensional quantum information processing.

DOI
10.48550/arxiv.2209.01913

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The first color photos of the parametric down-conversion (PDC) emission cone illustrate the correlation of longitudinal- and transverse momentum in the process, i.e., wavelength-dependent emission angle of PDC photons. However, current experiments and applications are more conveniently described in terms of discrete mode sets, with the most suitable choice depending on the propagation symmetries of the experimental setting. Remarkably, despite the fact that experiments with PDC sources are becoming ever more demanding, e.g. in terms of brightness or state fidelity, a description of spectral-spatial coupling in parametric downconversion for the case of discrete modal decompositions remains elusive. We present a comprehensive study, in theory and experiment, of the spectral dependence of the transverse Laguerre-Gauss modes in parametric downconversion. Moreover, we show how the spectral and spatial coupling can be harnessed to tune the purity of the well-known orbital angular momentum entanglement. This work has implications for efficient collection of entangled photons in a transverse single mode, quantum imaging, and engineering pure states for high-dimensional quantum information processing.
The first color photos of the parametric down-conversion (PDC) emission cone illustrate the correlation of longitudinal and transverse momentum in the process, i.e., wavelength-dependent emission angles of PDC photons. However, current experiments and applications are more conveniently described in terms of discrete mode sets, with the most suitable choice depending on the propagation symmetries of the experimental setting. Remarkably, despite the fact that experiments with PDC sources are becoming ever more demanding, e.g., in terms of brightness or state fidelity, a description of spectral-spatial coupling in parametric down-conversion for the case of discrete modal decompositions remains elusive. We present a comprehensive study, in theory and experiment, of the spectral dependence of the transverse Laguerre-Gauss modes in parametric down-conversion. Moreover, we show how the spectral and spatial coupling can be harnessed to tune the purity of the well-known orbital angular momentum entanglement. This paper has implications for efficient collection of entangled photons in a transverse single mode, quantum imaging, and engineering pure states for high-dimensional quantum information processing. Published by the American Physical Society 2024
High dimensional quantum states are of fundamental interest for quantum information processing. They give access to large Hilbert spaces and, in turn, enable the encoding of quantum information on multiple modes. One method to create such quantum states is parametric down-conversion (PDC) in waveguide arrays (WGAs) which allows for the creation of highly entangled photon pairs in controlled, easily accessible spatial modes, with unique spectral properties. In this paper we examine both theoretically and experimentally the PDC process in a lithium niobate WGA. We measure the spatial and spectral properties of the emitted photon pairs, revealing correlations between spectral and spatial degrees of freedom of the created photons. Our measurements show that, in contrast to prior theoretical approaches, spectrally dependent coupling effects have to be taken into account in the theory of PDC in WGAs. To interpret the results, we developed a theoretical model specifically taking into account spectrally dependent coupling effects, which further enables us to explore the capabilities and limitations for engineering the spatial correlations of the generated quantum states.
High dimensional quantum states are of fundamental interest for quantum information processing. They give access to large Hilbert spaces and, in turn, enable the encoding of quantum information on multiple modes. One method to create such quantum states is parametric down-conversion (PDC) in waveguide arrays (WGAs) which allows for the creation of highly entangled photon pairs in controlled, easily accessible spatial modes, with unique spectral properties. In this paper we examine both theoretically and experimentally the PDC process in a lithium niobate WGA. We measure the spatial and spectral properties of the emitted photon pairs, revealing correlations between spectral and spatial degrees of freedom of the created photons. Our measurements show that, in contrast to prior theoretical approaches, spectrally dependent coupling effects have to be taken into account in the theory of PDC in WGAs. To interpret the results, we developed a theoretical model specifically taking into account spectrally dependent coupling effects, which further enables us to explore the capabilities and limitations for engineering the spatial correlations of the generated quantum states.
Photon sources based on spontaneous parametric down-conversion (SPDC) are central to experimental quantum optics and quantum technologies. Their performance is commonly quantified by three metrics: pair-collection probability, heralding efficiency, and spectral purity. In bulk-crystal SPDC, these metrics are known to be mutually constrained, yet the physical origin of the resulting trade-offs is often obscured. We show that these trade-offs originate from the frequency-dependent population of discrete spatial modes in the SPDC emission. By performing a Laguerre-Gauss mode decomposition at each frequency component, we show how spectral-spatial non-separability impacts collection probability, heralding efficiency, and purity. We apply this framework to two widely used quasi-phase-matching configurations: collinear degenerate type-0 and type-II SPDC in periodically poled bulk crystals, and quantify how different phase-matching functions shape the spectral-spatial mode structure. In particular, for type-II SPDC we compare standard periodically poled and aperiodically poled Gaussian phase matching. We experimentally validate some of our theoretical results using spatial- and spectral-projection measurements. This spectral-spatial mode analysis provides a quantitative and predictive framework for understanding and engineering bulk-crystal photon sources, enabling systematic multi-parameter optimization beyond qualitative design guidelines.
We elucidate the paraxial orbital angular momentum of entangled photon pairs generated by spontaneous parametric down-conversion (SPDC) in different non-collinear geometries. To date, most investigations addressed SPDC in nearly collinear phase-matching geometries, where the pump, the signal and idler photons propagate coaxially almost along the same direction. However, non-collinear geometries introduce a variety of new features. The OAM of the entangled photons strongly depend on the propagation direction of the photons. Here we show that locally paraxial measurements of the OAM conducted with entangled photons generated in non collinear geometries, they do not comply with the known selection rules for the spiral index of the pump, signal and idler mode functions (Mair et al., Nature 412, 313 (2001)). In particular, we find the orbital angular momentum of entangled pairs generated in purely transverse-emitting configurations, where the entangled photons counter-propagate perpendicularly to the direction of propagation of the pump beam. In transverse emitting configurations, the spatial shape of the down converted in one transverse dimensions strongly depends on the corresponding spatial shape of the input pump beam, while in the other transverse dimension, the shape is tailored by the longitudinal phase matching. The spatial walk-off of all interacting waves in the parametric process also determines the OAM content of the down-converted photons, and here its influence is also revealed.