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arXiv:2208.13548 · Physical Review Letters

Quantized Fields for Optimal Control in the Strong Coupling Regime

Frieder Lindel, Edoardo G. Carnio, Stefan Yoshi Buhmann, Andreas Buchleitner

Published Mar 28, 2023• 3 citations
arXivHTMLPDF

Abstract

We tailor the quantum statistics of a bosonic field to deterministically drive a quantum system into a target state. Experimentally accessible states of the field achieve good control of multilevel or multiqubit systems, notably also at coupling strengths beyond the rotating-wave approximation. This extends optimal control theory to the realm of fully quantized, strongly coupled control and target degrees of freedom.

DOI
10.1103/physrevlett.130.133601

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We tailor the quantum statistics of a bosonic field to deterministically drive a quantum system into a target state. Experimentally accessible states of the field achieve good control of multilevel or multiqubit systems, notably also at coupling strengths beyond the rotating-wave approximation. This extends optimal control theory to the realm of fully quantized, strongly coupled control and target degrees of freedom.
In conventional quantum optimal control theory, the parameters that determine an external field are optimised to maximise some predefined function of the trajectory, or of the final state, of a matter system. The situation changes in the case of quantum electrodynamics, where the degrees of freedom of the radiation field are now part of the system. In consequence, instead of optimising an external field, the optimal control question turns into a optimisation problem for the many-body initial state of the combined matter-photon system. In the present work, we develop such an optimal control theory for quantum electrodynamics. We derive the equation that provides the gradient of the target function, which is often the occupation of some given state or subspace, with respect to the control variables that define the initial state. We choose the well-known Dicke model to study the possibilities of this technique. In the weak coupling regime, we find that Dicke states are the optimal matter states to reach Fock number states of the cavity mode with large fidelity, and vice versa, that Fock number states of the photon modes are the optimal states to reach the Dicke states. This picture does not prevail in the strong coupling regime. We have also considered the extended case with more than one mode. In this case, we find that increasing the number of two-level systems allows reaching a larger occupation of entangled photon targets.
A Markovian master equation describing the evolution of open quantum systems in the presence of a time-dependent external field is derived within the Bloch-Redfield formalism. It leads to a system-bath interaction which depends on the control field. Optimal control theory is used to select control fields which allow accelerated or decelerated system relaxation, or suppression of relaxation (dissipation) altogether, depending on the dynamics we impose on the quantum system. The control-dissipation correlation and the nonperturbative treatment of the control field are essential for reaching this goal. The optimal control problem is formulated within Pontryagin's minimum principle and the resulting optimal differential system is solved numerically. As an application, we study the dynamics of a spin-boson model in the strong coupling regime under the influence of an external control field. We show how trapping the system in unstable quantum states and transfer of population can be achieved by optimized control of the dissipative quantum system. We also used optimal control theory to find the driving field that generates the quantum ZZZ gate. In several cases studied, we find that the selected optimal field which reduces the purity loss significantly is a multicomponent low-frequency field including higher harmonics, all of which lie below the phonon cutoff frequency. Finally, in the undriven case we present an analytic result for the Lamb shift at zero temperature.
In this article, we present an overview of theory and technique for optimal control of molecular dynamics using tailored light fields. The goal of this research is to design an optical field, which can drive a system to a desired target state with a fairly high probability and low power expenditure. For the laboratory implementation of the designed field, it is desirable that it has simple frequency structure and that the control outcome is robust in the presence of noise which will always accompany the field. The ability of the control field to cooperate with noise in the manipulation of quantum dynamics is also discussed.
The theory of optimal control of quantum systems is combined with a variational method for quantum-statistical dynamics to facilitate efficient nonperturbative calculations. The linear eigenfield approach is extended to the nonlinear regime to treat saturation and other higher-order effects. The application to a three-level \ensuremath{\Lambda} system generates, via an efficient iterative scheme, an eigenfield producing optimal constructive interference between direct and three-step excitation paths.
Driving quantum systems periodically in time plays an essential role in the coherent control of quantum states. The rotating-wave approximation (RWA) is a good approximation technique for weak and nearly resonance driven fields. However, these experiments sometimes require large detuning and strong driving fields, for which the RWA may not hold. In this work, we experimentally, numerically, and analytically explore strongly driven two-mode Josephson circuits in the regime of strong driving and large detuning. Specifically, we investigate beam-splitter and two-mode squeezing interaction between the two modes induced by driving a two-photon sideband transition. Using numerical simulations, we observe that the RWA is unable to correctly capture the amplitude of the sideband transition rates. We verify this finding using an analytical model that is based on perturbative corrections. We find that the breakdown of the RWA in the regime studied does not lead to qualitatively different dynamics, but gives the same results as the RWA theory at higher drive strengths, enhancing the coupling rates compared to what one would predict. This is an interesting consequence compared to the carrier transition case, where the breakdown of the RWA results in qualitatively different time evolution of the quantum state. Our work provides an insight into the behavior of time-periodically driven systems beyond the RWA. We also provide a robust theoretical framework for including these findings in the calculation and calibration of quantum protocols in circuit quantum electrodynamics.
Quantum optimal control, a toolbox for devising and implementing the shapes of external fields that accomplish given tasks in the operation of a quantum device in the best way possible, has evolved into one of the cornerstones for enabling quantum technologies. The last few years have seen a rapid evolution and expansion of the field. We review here recent progress in our understanding of the controllability of open quantum systems and in the development and application of quantum control techniques to quantum technologies. We also address key challenges and sketch a roadmap for future developments.