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arXiv:2208.09314 · Physical Review Letters

Spectroscopy of Spin-Split Andreev Levels in a Quantum Dot with Superconducting Leads

Arno Bargerbos, Marta Pita‐Vidal, Rok Žitko, Lukas Johannes Splitthoff, Lukas Grünhaupt, Jaap J. Wesdorp, Yu Liu, Leo P. Kouwenhoven, Ramón Aguado, Christian Kraglund Andersen, Angela Kou, Bernard van Heck

Published Aug 31, 2023• 51 citations
arXivHTMLPDF

Abstract

We use a hybrid superconductor-semiconductor transmon device to perform spectroscopy of a quantum dot Josephson junction tuned to be in a spin-1/2 ground state with an unpaired quasiparticle. Because of spin-orbit coupling, we resolve two flux-sensitive branches in the transmon spectrum, depending on the spin of the quasiparticle. A finite magnetic field shifts the two branches in energy, favoring one spin state and resulting in the anomalous Josephson effect. We demonstrate the excitation of the direct spin-flip transition using all-electrical control. Manipulation and control of the spin-flip transition enable the future implementation of charging energy protected Andreev spin qubits.

DOI
10.1103/physrevlett.131.097001

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We use a hybrid superconductor-semiconductor transmon device to perform spectroscopy of a quantum dot Josephson junction tuned to be in a spin-1/2 ground state with an unpaired quasiparticle. Because of spin-orbit coupling, we resolve two flux-sensitive branches in the transmon spectrum, depending on the spin of the quasiparticle. A finite magnetic field shifts the two branches in energy, favoring one spin state and resulting in the anomalous Josephson effect. We demonstrate the excitation of the direct spin-flip transition using all-electrical control. Manipulation and control of the spin-flip transition enable the future implementation of charging energy protected Andreev spin qubits.
We realize a hybrid superconductor-semiconductor transmon device in which the Josephson effect is controlled by a gate-defined quantum dot in an InAs-Al nanowire.Microwave spectroscopy of the transition spectrum of the transmon allows us to probe the ground-state parity of the quantum dot as a function of the gate voltages, the external magnetic flux, and the magnetic field applied parallel to the nanowire.The measured parity phase diagram is in agreement with that predicted by a single-impurity Anderson model with superconducting leads.Through continuous-time monitoring of the circuit, we furthermore resolve the quasiparticle dynamics of the quantum dot Josephson junction across the phase boundaries.Our results can facilitate the realization of semiconductor-based 0-π qubits and Andreev qubits.
We solve the problem of an interacting quantum dot embedded in a Josephson junction between two superconductors with finite charging energy described by the transmon (Cooper pair box) Hamiltonian. The approach is based on the flat-band approximation of the Richardson model, which reduces the Hilbert space to the point where exact diagonalization is possible while retaining all states that are necessary to describe the low-energy phenomena. The presented method accounts for the physics of the quantum dot, the Josephson effect, and the Coulomb repulsion (charging energy) at the same level. In particular, it captures the quantum fluctuations of the superconducting phase as well as the coupling between the superconducting phase and the quantum dot (spin) degrees of freedom. The method can be directly applied for modeling Andreev spin qubits embedded in transmon circuits in all parameter regimes, for describing time-dependent processes, and for the calculation of transition matrix elements for microwave-driven transmon, spin-flip, and mixed transitions that involve coupling to charge or current degrees of freedom.
We investigate the superconducting Anderson impurity model for interacting quantum dot Josephson junctions with spin-orbit coupling and a term accounting for tunnelling through higher-energy orbitals. These elements establish the conditions required for spin polarization in the absence of external magnetic field at finite superconducting phase bias. This Hamiltonian has been previously used to model the Andreev spin qubit, where quantum information is encoded in spinful odd-parity subgap states. Here we instead analyse the even-parity sector, i.e., the Andreev pair qubit based on Andreev bound states (ABS). The model is solved using the zero-bandwidth approximation and the numerical renormalization group, with further insight from variational calculations. Electron-electron interaction admixes single-occupancy Yu-Shiba-Rusinov (YSR) components into the ABS states, thereby strongly enhancing spin transitions in the presence of spin-orbit coupling. The ABS states can thus become sensitive to local magnetic field fluctuations, which has implications for decoherence in Andreev pair qubits. For strong interaction U U , especially in the cross-over region between the ABS and YSR regimes for U \sim 2\Delta U ∼ 2 Δ , charge, spin, and inductive transitions can all become strong, offering avenues for spin control and quantum transduction.
Abstract Josephson junctions based on semiconductor nanowires are potential building blocks for electrically tunable qubit structures, e.g., the gatemon or the Andreev qubit. However, an actual realization requires the thorough investigation of the intrinsic excitation spectrum. Here, we demonstrate the fabrication of low-loss superconducting microwave circuits that combine high quality factors with a well-controlled gate architecture by utilizing a flip-chip approach. This platform is then used to perform single-tone and two-tone experiments on Andreev states in in-situ grown InAs/Al core/half-shell nanowires with shadow mask defined Josephson junctions. In gate-controlled and flux-biased spectroscopic measurements we find clear signatures of single quasiparticle as well as quasiparticle pair transitions between discrete Andreev bound states mediated by photon-absorption. Our experimental findings are supported by simulations that show that the junction resides in the intermediate channel length regime.
Hybrid semiconductor-superconductor qubits have recently emerged as a promising alternative to traditional platforms, combining material advantages with device-level tunability. A defining feature is their gate-tunable Josephson coupling, enabling superconducting qubit architectures with full electric-field control and offering a path toward scalable, low-crosstalk quantum processors. This approach seeks to merge benefits of superconducting and semiconductor qubits, for instance by encoding quantum information in the spin of a quasiparticle occupying an Andreev bound state, thus combining long coherence times with fast, flexible control. Progress has accelerated through bottom-up engineering of Andreev states in coupled quantum dot arrays, leading to architectures such as minimal Kitaev chains hosting Majorana zero modes. In parallel, Hamiltonian-protected designs aim to enhance resilience against local noise and decoherence by exploiting superconducting phase dynamics and discrete charge or flux degrees of freedom. This article reviews recent theoretical and experimental advances in hybrid qubits, providing an overview of physical mechanisms, device implementations, and emerging architectures, with emphasis on their potential for (topologically) protected quantum information processing. While many designs remain at proof-of-concept stage, rapid progress suggests practical demonstrations may soon be achievable.
Andreev levels localized in a weak link between two superconductors can trap a superconducting quasiparticle. If there is a spin-orbit coupling in the link, the spin of the quasiparticle couples to the Josephson current. This effect can be leveraged to control and read out the spin of the quasiparticle, thus using it as a qubit. One of the factors limiting the performance of such an Andreev spin qubit is spin relaxation. Here, we theoretically demonstrate that the relaxation lifetime can be enhanced by utilizing the coupling between the Andreev spin and the supercurrent in a transmon circuit. The coupling ensures that the flip of the quasiparticle spin can only happen if it is accompanied by the excitation of multiple plasmons, as dictated by the Franck-Condon principle. This blocks spin relaxation at temperatures small compared to plasmon energy.