Atomic spectroscopy, an essential tool for frequency estimation, is widely used in quantum sensing. Atom-atom interaction can be used to generate entanglement for achieving quantum enhanced sensing. However, atom-atom interaction always induces collision shift, which brings systematic error in determining the resonance frequency. Contradiction between utilizing atom-atom interaction and suppressing collision shift generally exists in atomic spectroscopy. Here, we propose an antisymmetric Rabi spectroscopy protocol without collision shift in the presence of atom-atom interactions. We analytically find that the antisymmetric point can be used for determining the resonance frequency. For small Rabi frequency, our antisymmetric Rabi spectroscopy with slight atom-atom interaction can provide better measurement precision than the conventional Rabi spectroscopy. With stronger atom-atom interaction and Rabi frequency, the spectrum resolution can be dramatically improved and the measurement precision may even beat the standard quantum limit. Moreover, unlike the quantum-enhanced Ramsey interferometry via spin squeezing, our scheme is robust against detection noises. Our antisymmetric Rabi spectroscopy protocol has promising applications in various practical quantum sensors such as atomic clocks and atomic magnetometers.
Atomic spectroscopy, an essential tool for frequency estimation, is widely used in quantum sensing. Atom-atom interaction can be used to generate entanglement for achieving quantum enhanced sensing. However, atom-atom interaction always induces collision shift, which brings systematic error in determining the resonance frequency. Contradiction between utilizing atom-atom interaction and suppressing collision shift generally exists in atomic spectroscopy. Here, we propose an antisymmetric Rabi spectroscopy protocol without collision shift in the presence of atom-atom interactions. We analytically find that the antisymmetric point can be used for determining the resonance frequency. For small Rabi frequency, our antisymmetric Rabi spectroscopy with slight atom-atom interaction can provide better measurement precision than the conventional Rabi spectroscopy. With stronger atom-atom interaction and Rabi frequency, the spectrum resolution can be dramatically improved and the measurement precision may even beat the standard quantum limit. Moreover, unlike the quantum-enhanced Ramsey interferometry via spin squeezing, our scheme is robust against detection noises. Our antisymmetric Rabi spectroscopy protocol has promising applications in various practical quantum sensors such as atomic clocks and atomic magnetometers.
Ramsey spectroscopy serves as a key tool for frequency measurement. Although entanglement can enhance the measurement precision, the atom-atom interaction required for entanglement generation may lead to a frequency shift. In addition, the spectra also suffer from light shift caused by the interaction between light and atoms. Thus, it is difficult to achieve high precision without inducing additional systematic errors. Here, we propose to realize high-precision entanglement-enhanced Ramsey spectroscopy with composite pulses. First, we utilize spin-squeezed states generated by one-axis twisting (OAT) dynamics to enhance the measurement precision. We find that by applying a suitable pulse after OAT, the resonant frequency can be inferred and the light shift can be reduced by using composite pulses. To increase the signal slope, we use anti-OAT dynamics to perform interaction-based readout after interrogation. By designing suitable composite pulses, it can significantly increase the signal response and further improve the measurement precision. Although both schemes can mitigate the light shift, it cannot be entirely eliminated. Thus, we develop the autobalanced entanglement-enhanced Ramsey spectroscopy. By using combination of different sequences with short and long interrogation times and feedback control, the light shift of both our protocols can be completely suppressed, which increases the measurement accuracy. Besides, we also investigate the effects of background atom-atom interaction and find that it only reduces the measurement precision without introducing additional frequency shift. Our study offers an alternative method for achieving precise frequency measurement, which has the potential to be of significant application in quantum sensors such as atomic clocks.
Ramsey spectroscopy, a fundamental tool in both basic science and practical applications, is inevitably subject to several detrimental effects. % Here we propose a symmetry-protected destructive many-body interferometry (SPDMBI) for Ramsey spectroscopy, which successfully mitigates the spectral shift caused by interparticle interaction, noise, decoherence and experimental imperfection. % Through matching the symmetry of the input states and the Hamiltonian, the SPDMBI-based Ramsey spectroscopy yields an antisymmetric spectrum, whose antisymmetric point exactly determines the resonance frequency. % In such a Ramsey spectroscopy, the population difference under resonance is always zero, which is a result of destructive quantum interferometry. % To demonstrate its versatility, we showcase successful applications of symmetry-protected Ramsey spectroscopy in measuring both time-independent and time-dependent signals. % Our protocol can improve the performance of Ramsey spectroscopy, which offers a pathway for various high-precision quantum sensors.
Quantum entanglement is a powerful quantum resource for enhancing measurement precision beyond classical limit. % Here we propose an entanglement-enhanced symmetry-protected destructive many-body Ramsey interferometry for precise parameter estimation. % Through matching the symmetry of input states and Hamiltonian, the spectral shift of Ramsey spectroscopy caused by interparticle interaction, noise, decoherence and experimental imperfection can be mitigated for both time-independent and time-dependent signals, as explored in the companion Letter [S. Chen, et al., Ramsey Spectroscopy via Symmetry-Protected Destructive Many-Body Interferometry (submitted)]. % In this work, we show that symmetric entangled input states can further improve the measurement precision of symmetry-protected Ramsey spectroscopy without affecting the measurement accuracy. % Through inputting spin cat states and applying suitable interaction-based readout operations, the measurement precisions of time-independent and time-dependent signals can both approach the Heisenberg limit. % In particular, we systematically analyze how precision scaling and robustness depend on the input states, parameters, experimental imperfection and decoherence. % This work establishes a practical pathway to Heisenberg-limited quantum metrology with many-body Ramsey interferometry, offering resilience against realistic noise and imperfections.
Atomic projection noise limits the ultimate precision of all atomic sensors, including clocks, inertial sensors, magnetometers, etc. The independent quantum collapse of N atoms into a definite state (for example spin up or down) leads to an uncertainty ΔθSQL= 1/√N in the estimate of the quantum phase accumulated during a Ramsey sequence or its many generalizations. This phase uncertainty is referred to as the standard quantum limit. Creating quantum entanglement between the N atoms can allow the atoms to partially cancel each other's quantum noise, leading to reduced noise in the phase estimate below the standard quantum limit. Recent experiments have demonstrated up to 10 dB of phase noise reduction relative to the SQL by making collective spin measurements. This is achieved by trapping laser-cooled Rb atoms in an optical cavity and precisely measuring the shift of the cavity resonance frequency by an amount that depends on the number of atoms in spin up. Detecting the probe light with high total efficiency reduces excess classical and quantum back-action of the probe. Here we discuss recent progress and a technique for reducing the relative frequency noise between the probe light and the optical cavity, a key requirement for further advances.
Atomic clocks are crucial for fundamental science and practical technology, but their sensitivity is often constrained by the standard quantum limit. With a cold-atom coherent-population-trapping clock, the authors design and experimentally demonstrate an adaptive Bayesian quantum frequency estimation protocol that approaches the Heisenberg scaling with respect to total interrogation time. This atomic clock also yields improved fractional frequency stability and enhanced robustness against technical noises. This work provides a high-precision approach to atomic clock locking, and holds promising applications in various interferometry-based quantum sensors.
Ramsey interferometry is a widely used tool for precisely measuring transition frequencies between two energy levels of a quantum system, with applications in time keeping, precision spectroscopy, quantum optics, and quantum information. Often, the coherence time of the quantum system surpasses the one of the oscillator probing the system, thereby limiting the interrogation time and associated spectral resolution. Correlation spectroscopy overcomes this limitation by probing two quantum systems with the same noisy oscillator for a measurement of their transition frequency difference; this technique has enabled very precise comparisons of atomic clocks. Here, we extend correlation spectroscopy to the case of multiple quantum systems undergoing strong correlated dephasing. We model Ramsey correlation spectroscopy with N particles as a multiparameter phase estimation problem and demonstrate that multiparticle correlations can assist in reducing the measurement uncertainties even in the absence of entanglement. We derive precision limits and optimal sensing techniques for this problem and compare the performance of probe states and measurement with and without entanglement. Using one- and two-dimensional ion Coulomb crystals with up to 91 qubits, we experimentally demonstrate the advantage of measuring multiparticle correlations for reducing phase uncertainties and apply correlation spectroscopy to measure ion-ion distances, transition frequency shifts, laser-ion detunings, and path-length fluctuations. Our method can be straightforwardly implemented in experimental setups with globally coherent qubit control and qubit-resolved single-shot readout and is, thus, applicable to other physical systems such as neutral atoms in tweezer arrays. Published by the American Physical Society 2024